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We report on strong dipole transitions to 3d orbitals of neighboring Co atoms in the Co 1s x-ray absorption pre-edge. They are revealed by applying high-resolution resonant x-ray emission spectroscopy (RXES) to compounds containing CoO6…

Strongly Correlated Electrons · Physics 2008-02-21 György Vankó , Frank M. F. de Groot , Simo Huotari , R. J. Cava , Thomas Lorenz , M. Reuther

Spectroscopic properties, useful for plasma diagnostics and astrophysics, of a few rubidium-like ions are studied here. We choose one of the simplest, but correlationally challenging series where $d-$ and $f-$ orbitals are present in the…

Atomic Physics · Physics 2018-01-17 Arghya Das , Anal Bhowmik , Narendra Nath Dutta , Sonjoy Majumder

Charge transfer between metal nanoparticles and the supported TiO2 surface is primarily important for catalytic applications as it greatly affects the catalytic activity and the thermal stability of the deposited nanoparticles on the…

Materials Science · Physics 2013-12-24 Cai Yongqing , Bai Zhaoqiang , Chintalapati Sandhya , Zeng Qingfeng , Feng Yuan Ping

The lifting of degenerate electronic states, in which multiple electronic states share the same energy, is a fundamental issue in the physics of crystalline solids. In real materials, this problem has been extensively studied in transition…

The electronic structure and magnetic properties of the 2H-NbS$_2$ compound intercalated by Cr, Mn and Fe, have been investigated by means of the Korringa-Kohn-Rostoker (KKR) method. The calculations demonstrate easy plane…

Materials Science · Physics 2016-11-30 S. Mankovsky , S. Polesya , H. Ebert , W. Bensch

Ilmenites $AB$O$_3$ provide a platform for electron correlation and magnetism on alternatively stacked honeycomb layers of edge-sharing $A$O$_6$ or $B$O$_6$ octahedra. When $A$ and $B$ are $3d$ transition metals, strong electron correlation…

Strongly Correlated Electrons · Physics 2024-02-12 Seong-Hoon Jang , Yukitoshi Motome

Metal insulator transitions driven by local Coulomb interactions are among the most fascinating phenomena in condensed matter physics. They occur in a large variety of transition metal compounds. Most of these strongly correlated materials…

Strongly Correlated Electrons · Physics 2007-05-23 A. Liebsch

Transition metals (TMs) implanted in oxides with rock-salt crystal structures (for example MgO and BaO) are assumed to substitute cations (Mg in case of MgO) from the lattice sites. We show that not all implanted TMs substitute cations but…

Materials Science · Physics 2019-03-14 Debolina Misra , Satyesh K. Yadav

Local structural measurements have been performed on hexagonal HoMnO3 in order to ascertain the specific changes in bond distances which accompany magnetic ordering transitions. The transition from paramagnetic to the antiferromagetic…

Strongly Correlated Electrons · Physics 2015-05-14 T. A. Tyson , T. Wu , K. H. Ahn , S. Kim , S. -W. Cheong

We studied the mechanism of half-metallicity (HM) formation in transition metal doped (TM) conjugated carbon based structures by first-principles electronic structure simulations. It is found that the HM is a rather complex phenomenon,…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Lida Pan , Boqun Song , Jiatao Sun , Lizhi Zhang , Werner Hofer , Shixuan Du , Hong-jun Gao

Several layered transition metal borides can now be realized by a simple and general fabrication method [Fokwa et al.,Adv. Mater. 2018, 30, 1704181],inspiring our interest to transition metal borides monolayer. Here, we predict a new…

Materials Science · Physics 2019-11-05 Yipeng An , Shijing Gong , Yusheng Hou , Jie Li , Ruqian Wu , Zhaoyong Jiao , Tianxing Wang , Jutao Jiao

MAB phases (MABs) are atomically-thin laminates of ceramic/metallic-like layers, having made a breakthrough in the development of 2D materials. Though theoretically offering a vast chemical and phase space, relatively few MABs have yet been…

Materials Science · Physics 2024-06-21 Nikola Koutná , Lars Hultman , Paul H. Mayrhofer , Davide G. Sangiovanni

The low and high-temperature phases of V$_4$O$_7$ have been studied by \textit{ab initio} calculations. At high temperature, all V atoms are electronically equivalent and the material is metallic. Charge and orbital ordering, associated…

Strongly Correlated Electrons · Physics 2011-12-06 A. S. Botana , V. Pardo , D. Baldomir , A. V. Ushakov , D. I. Khomskii

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

Strongly Correlated Electrons · Physics 2015-12-23 F. Wallington , A. M. Arevalo-Lopez , J. W. Taylor , J. R. Stewart , V. Garcia-Sakai , J. P. Attfield , C. Stock

X-ray resonant scattering at the K-edge of transition metal oxides is shown to measure the orbital order parameter, supposed to accompany magnetic ordering in some cases. Virtual transitions to the 3d-orbitals are quadrupolar in general. In…

Strongly Correlated Electrons · Physics 2009-10-30 Michele Fabrizio , Massimo Altarelli , Maurizio Benfatto

Electronic structures of MC where M is the alkali and alkaline earth metals with the rocksalt structure are calculated by full potential density functional codes. We find that the spin magnetic moment in the compounds is mainly contributed…

Materials Science · Physics 2012-11-02 Wenxu Zhang , Zhida Song , Bin Peng , Wanli Zhang

I give a brief overview of a polaron formation in three distinct transition metal oxides: (i) spin polaron when a hole is added to the antiferromagnetic (AF) ordered plane in La$_2$CuO$_4$, (ii) orbital polaron when a hole is added to the…

Strongly Correlated Electrons · Physics 2015-05-13 Krzysztof Wohlfeld

Magnetic and transport properties of (Pr1/3Sm2/3)2/3A1/3MnO3 (A = Ca, Sr and Ba) compounds, prepared by the citrate gel route, have been investigated. These compounds are found to crystallize in the orthorhombic structure. Charge ordering…

Materials Science · Physics 2009-11-10 Saket Asthana , D. Bahadur , A. K. Nigam , S. K. Malik

The metal-insulator transition of the Magneli phase Ti4O7 is studied by means of augmented spherical wave (ASW) electronic structure calculations as based on density functional theory and the local density approximation. The results show…

Strongly Correlated Electrons · Physics 2009-11-10 V. Eyert , U. Schwingenschloegl , U. Eckern

In this paper we propose a tight-binding molecular dynamics with parameters fitted to first-principles calculations on the smaller clusters and with an environment correction, to be a powerful technique for studying large transition/noble…

Atomic and Molecular Clusters · Physics 2009-11-10 Mukul Kabir , Abhijit Mookerjee , A. K. Bhattacharya