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We show that the highly conductive polymer poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate) (PEDOT:PSS) can successfully be applied as a hole selective front contact in silicon heterojunction (SHJ) solar cells. In combination with a…

Other Condensed Matter · Physics 2017-01-20 Sara Jäckle , Martin Liebhaber , Clemens Gersmann , Mathias Mews , Klaus Jäger , Silke Christiansen , Klaus Lips

Antiperovskites are a rich family of compounds with applications in battery cathodes, superconductors, solid-state lighting, and catalysis. Recently, a novel series of antimonide phosphide antiperovskites (A$_3$SbP, where A = Ca, Sr, Ba)…

Materials Science · Physics 2023-12-05 Ruiqi Wu , Alex M. Ganose

Previously, we proposed that the polarization and capacitive charge in \ce{CH3NH3PbI3} screens the external electric field that hinders charge transport. We argue here that this screening effect is in significant part responsible for the…

Mesoscale and Nanoscale Physics · Physics 2016-09-28 Yecheng Zhou , Fuzhi Huang , Yi-Bing Cheng , Angus Gray-Weale

Perovskite/Si tandem solar cells have the potential to considerably out-perform conventional solar cells. Under standard test conditions, perovskite/Si tandem solar cells already outperform the Si single junction. Under realistic…

Materials Science · Physics 2017-08-23 Moritz H. Futscher , Bruno Ehrler

Lead-halide perovskites have demonstrated astonishing increases in power conversion efficiency in photovoltaics over the last decade. The most efficient perovskite devices now outperform industry-standard multi-crystalline silicon solar…

Applied Physics · Physics 2023-02-20 Yi-Teng Huang , Sean R. Kavanagh , David O. Scanlon , Aron Walsh , Robert L. Z. Hoye

The efficiency and stability of halide perovskite-based solar cells and light-emitting diodes directly depend on the intricate dynamics of solid-solid crystallization[1-23]. In this study, we employ a multi-scale approach using random phase…

Materials Science · Physics 2024-04-09 Paramvir Ahlawat

Perovskite-based optoelectronic devices have gained significant attention due to their remarkable performance and low processing cost, particularly for solar cells. However, for perovskite light-emitting diodes (LEDs), non-radiative charge…

Thin-film solar cells suffer from various types of recombination, of which leakage current usually dominates at lower voltages. Herein, we demonstrate first a three-order reduction of the shunt loss mechanism in planar methylammonium lead…

Singlet fission process has gained considerable attention because of its potential to enhance photovoltaic efficiency and break the Shockley Queisser limit. In photovoltaic devices perovskite materials have shown tremendous progress in the…

Materials Science · Physics 2022-04-07 Tejasvini Sharma , Saurav Saini , Naveen Kumar Tailor , Mahesh Kumar , Soumitra Satapathi

Ion and metal diffusion in metal halide perovskites, charge-transporting layers, and electrodes are detrimental to the performance and stability of perovskite-based photovoltaic devices. As a result, there is an intense research interest in…

Herein, we report on the synthesis and investigation of two triazino-isoquinoline tetrafluoroborate electrolytes as hole-blocking layers in methylammonium triiodide perovskite photovoltaic devices with fullerene electron extraction layer.…

Lead poisoning and notorious ambient instability in lead-based halide perovskites pave the way for the exploration of alternative materials for affordable and efficient solar cell fabrication. An important prerequisite to this end is the…

Next-generation low-cost semiconductors such as halide perovskites exhibit optoelectronic properties dominated by nanoscale variations in their structure, composition and photophysics. While microscopy provides a proxy for ultimate device…

Increasing evidence suggests that the presence of mobile ions in perovskite solar cells can cause a current-voltage curve hysteresis. Steady state and transient current-voltage characteristics of a planar metal halide CH$_3$NH$_3$PbI$_3$…

Applied Physics · Physics 2018-04-24 N. E. Courtier , J. M. Foster , S. E. J. O'Kane , A. B. Walker , G. Richardson

Light fusion increases the efficiency of solar cells by converting photons with lower energy than the bandgap into higher energy photons. The solar cell converts the product photons to current. We use Monte Carlo simulation to predict that…

Mesoscale and Nanoscale Physics · Physics 2021-12-20 Benedicta Sherrie , Alison M. Funston , Laszlo Frazer

Two-dimensional (2D) perovskites show higher stability in comparison to their three-dimensional (3D) counterparts. Therefore, 2D perovskites have invoked remarkable attention in basic understanding of their physical properties and…

Materials Science · Physics 2025-07-01 Deepika Gill , Gunjana Yadav , Saswata Bhattacharya

Recent research on perovskite solar cells has caught much attention for the application in renewable energy materials. However, the effect of external dopants on the performance of perovskite solar cell is yet to be understood properly.…

Materials Science · Physics 2024-01-18 Chongyao Yang , Wei Wu , Kwang-Leong Choy

Chemically prepared colloidal semiconductor quantum dots have long been proposed as scalable and color-tunable single emitters in quantum optics, but they have typically suffered from prohibitively incoherent emission. We now demonstrate…

One of the most significant features of lead-halide perovskites are their ability to have comparably slow recombination despite the fact that these materials are mostly processed from solution at room temperature. The slow recombination…

Applied Physics · Physics 2019-07-26 Thomas Kirchartz

In perovskite solar cells (PSCs) energy levels alignment and charge extraction at the interfaces are the essential factors directly affecting the device performance. In this work, we present a modified interface between all-inorganic…

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