Related papers: Crossover of dynamical instability and chaos in th…
Recent research suggests that the supercritical state consists of liquidlike and gaslike states where particle dynamics and key system properties are qualitatively different. We report experimental evidence of the structural crossover in…
Physics of supercritical state is understood to a much lesser degree compared to subcritical liquids. Carbon dioxide in particular has been intensely studied, yet little is known about the supercritical part of its phase diagram. Here, we…
Dusty plasmas represent a powerful playground to study the collective dynamics of strongly coupled systems with important interdisciplinary connections to condensed matter physics. Due to the pure Yukawa repulsive interaction between dust…
We calculate the Lyapunov exponents in a classical molecular dynamics framework. The system is composed of few hundreds particles interacting either through Yukawa (Nuclear) or Slater-Kirkwood (Atomic) forces. The forces are chosen to give…
We calculate the maximal Lyapunov exponent, the generalized entropies, the asymptotic distance between nearby trajectories and the fractal dimensions for a finite two dimensional system at different initial excitation energies. We show that…
An upper bound on Lyapunov exponent of a thermal many body quantum system has been conjectured recently. In this work, we attempt to achieve a physical understanding of what prevents a system from violating this bound. To this end, we…
Many physical systems, including classical fluids, present in their phase diagram the competition between two phases that are separated by a line of first-order phase transitions which terminates at a so-called critical point. Despite…
There have been ample studies of the many phases of H2O in both its solid and low pressure liquid states, and the transitions between them. Using molecular dynamics simulations we address the hitherto unexplored deeply supercritical…
A general indicator of the presence of chaos in a dynamical system is the largest Lyapunov exponent. This quantity provides a measure of the mean exponential rate of divergence of nearby orbits. In this paper, we show that the so-called…
Can liquid-like and gas-like states be distinguished beyond the critical point, where the liquid-gas phase transition no longer exists and conventionally only a single supercritical fluid phase is defined? Recent experiments and simulations…
The dynamics of inertial particles in $2-d$ incompressible flows can be modeled by $4-d$ bailout embedding maps. The density of the inertial particles, relative to the density of the fluid, is a crucial parameter which controls the…
We calculate the maximal Lyapunov exponent in constant-energy molecular dynamics simulations at the melting transition for finite clusters of 6 to 13 particles (model rare-gas and metallic systems) as well as for bulk rare-gas solid. For…
Dynamical instability is studied in a deterministic dynamical system of Hamiltonian type composed of a tracer particle in a fluid of many particles. The tracer and fluid particles are hard balls (disks, in two dimensions, or spheres, in…
The dynamics of supercritical fluids, a state of matter beyond the gas-liquid critical point, changes from diffusive to oscillatory motions at high pressure. This transition is believed to occur across a locus of thermodynamic states called…
A new dynamic line, the Frenkel line, has recently been proposed to separate the supercritical state into rigid-liquid and non-rigid gas-like uid. The location of Frenkel line on the phase diagram is unknown for real uids. Here, we map the…
Fluids cooled to the liquid-vapor critical point develop system-spanning fluctuations in density that transform their visual appearance. Despite the rich phenomenology of this critical point, there is not currently an explanation of the…
We report experimental evidence for a crossover between a liquid-like state and a gas-like state in fluid methane (CH4). This crossover is observed in all of our experiments, up to 397 K temperature; 2.1 times the critical temperature of…
Random neural networks are dynamical descriptions of randomly interconnected neural units. These show a phase transition to chaos as a disorder parameter is increased. The microscopic mechanisms underlying this phase transition are unknown,…
The phase space trajectories of many body systems charateristic of simple fluids are highly unstable. We quantify this instability by a set of Lyapunov exponents, which are the rates of exponential divergence, or convergence, of initial…
It is demonstrated that the crossover between gas- and liquid-like regions on the phase diagram of the Lennard-Jones system occurs at a fixed value of the density divided by its value at the freezing point, $\rho/\rho_{\rm fr}\simeq 0.35$.…