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We present an implementation and benchmark of new approximations in multireference algebraic diagrammatic construction theory for simulations of neutral electronic excitations and UV/Vis spectra of strongly correlated molecular systems…

Chemical Physics · Physics 2021-12-02 Ilia M. Mazin , Alexander Yu. Sokolov

We present a second-order formulation of multi-reference algebraic diagrammatic construction theory [Sokolov, A. Yu. J. Chem. Phys. 2018, 149, 204113] for simulating photoelectron spectra of strongly correlated systems (MR-ADC(2)). The…

Chemical Physics · Physics 2020-07-28 Koushik Chatterjee , Alexander Yu. Sokolov

We present algebraic diagrammatic construction theory for simulating spin-orbit coupling and electron correlation in charged electronic states and photoelectron spectra. Our implementation supports Hartree-Fock and multiconfigurational…

Chemical Physics · Physics 2025-05-12 Rajat Majumder , Alexander Yu. Sokolov

We present a multi-reference generalization of the algebraic diagrammatic construction theory (ADC) [J. Schirmer, Phys. Rev. A 26, 2395 (1982)] for excited electronic states. The resulting multi-reference ADC approach (MR-ADC) can be…

Chemical Physics · Physics 2018-12-27 Alexander Yu. Sokolov

We report the development and benchmark of multireference algebraic diagrammatic construction theory (MR-ADC) for the simulations of core-excited states and X-ray absorption spectra (XAS). Our work features an implementation that…

Chemical Physics · Physics 2024-01-23 Ilia M. Mazin , Alexander Yu. Sokolov

We present an efficient implementation of multireference algebraic diagrammatic construction theory (MR-ADC) for simulating core-ionized states and X-ray photoelectron spectra (XPS). Taking advantage of spin adaptation, automatic code…

Chemical Physics · Physics 2024-11-19 Carlos E. V. de Moura , Alexander Yu. Sokolov

We present an efficient implementation of the second- and third-order single-reference algebraic diagrammatic construction theory for electron attachment (EA) and ionization (IP) energies and spectra (EA/IP-ADC(n), n = 2, 3). Our new…

Chemical Physics · Physics 2021-07-12 Samragni Banerjee , Alexander Yu. Sokolov

We present implementation of second- and third-order algebraic diagrammatic construction theory for efficient and accurate computations of molecular electron affinities (EA), ionization potentials (IP), and densities of states…

Chemical Physics · Physics 2020-07-28 Samragni Banerjee , Alexander Yu. Sokolov

We present a new theoretical approach for the simulations of X-ray photoelectron spectra of strongly correlated molecular systems that combines multireference algebraic diagrammatic construction theory (MR-ADC) [J. Chem. Phys., 2018, 149,…

Chemical Physics · Physics 2022-05-31 Carlos E. V. de Moura , Alexander Yu. Sokolov

We present the theory and implementation of a highly efficient relativistic third-order algebraic diagrammatic construction [ADC(3)] method based on a four-component (4c) Dirac-Coulomb (DC) Hamiltonian for the calculation of ionization…

Chemical Physics · Physics 2024-11-01 Sudipta Chakraborty , Tamoghna Mukhopadhyay , Malaya K. Nayak , Achintya Kumar Dutta

We present the first implementation and applications of non-Dyson algebraic diagrammatic construction theory for charged excitations in three-dimensional periodic solids (EA/IP-ADC). The EA/IP-ADC approach has a computational cost similar…

Materials Science · Physics 2022-11-15 Samragni Banerjee , Alexander Yu. Sokolov

We report internally contracted relativistic multireference configuration interaction (ic-MRCI), complete active space second-order perturbation (CASPT2), and strongly contracted n-electron valence state perturbation theory (NEVPT2) on the…

Chemical Physics · Physics 2015-12-31 Toru Shiozaki , Wataru Mizukami

We present an efficient relativistic implementation of algebraic diagrammatic construction (ADC) theory up to third order for the treatment of electronic ionization potentials (IP), electron affinities (EA), and excitation energies (EE) in…

Chemical Physics · Physics 2026-01-27 Sudipta Chakraborty , Kamal Majee , Achintya Kumar Dutta

We have developed a reduced-cost non-Dyson third-order algebraic diagrammatic construction theory for the electron-attachment problem based on state-specific frozen natural orbitals. Density fitting and truncated natural auxiliary functions…

Chemical Physics · Physics 2026-03-13 Tamoghna Mukhopadhyay , Kamal Majee , Achintya Kumar Dutta

Charged excitations are electronic transitions that involve a change in the total charge of a molecule or material. Understanding the properties and reactivity of charged species requires insights from theoretical calculations that can…

Chemical Physics · Physics 2023-06-16 Samragni Banerjee , Alexander Yu. Sokolov

Algebraic diagrammatic construction (ADC) theory is a computationally efficient and accurate approach for simulating electronic excitations in chemical systems. However, for the simulations of excited states in molecules with unpaired…

Chemical Physics · Physics 2022-11-15 Terrence L. Stahl , Samragni Banerjee , Alexander Yu. Sokolov

Theoretical simulations of electron detachment processes are vital for understanding chemical redox reactions, semiconductor and electrochemical properties, and high-energy radiation damage. However, accurate calculations of ionized…

Chemical Physics · Physics 2025-02-06 James D. Serna , Alexander Yu. Sokolov

A multiconfigurational adiabatic connection (AC) formalism is an attractive approach to computing dynamic correlation within CASSCF and DMRG models. Practical realizations of AC have been based on two approximations: i) fixing one- and…

Chemical Physics · Physics 2023-02-15 Mikuláš Matoušek , Michał Hapka , Libor Veis , Katarzyna Pernal

We present the first-ever implementation and benchmark of periodic algebraic diagrammatic construction theory (ADC) for core-ionized states and X-ray photoelectron spectra (XPS) in crystalline materials. Using a triple-zeta Gaussian basis…

Materials Science · Physics 2026-02-24 Abdelrahman M. Ahmed , Alexander Yu. Sokolov

We have studied electron correlations in the doped two-dimensional (2D) Hubbard model by using the coupled-cluster method (CCM) to investigate whether or not the method can be applied to correct the independent particle approximations…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshihiro Asai , Hideki Katagiri
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