Related papers: A spectrally bright wavelength-switchable vacuum u…
Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do…
Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies…
The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…
Although supercontinuum sources are readily available for the visible and near infrared, and recently also for the mid-IR, many areas of biology, chemistry and physics would benefit greatly from the availability of compact, stable and…
Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent…
Frequency-modulation (FM) spectroscopy has been extended to the vacuum-ultraviolet (VUV) range of the electromagnetic spectrum. Coherent VUV laser radiation is produced by resonance-enhanced sum-frequency mixing…
Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…
Recent demonstrations of high-harmonic generation (HHG) at very high repetition frequencies (~100 MHz) may allow for the revolutionary transfer of frequency combs to the vacuum ultraviolet (VUV). This advance necessitates unifying optical…
We present a source of coherent extreme ultraviolet (XUV) radiation with a flux of 10$^{13}$ photons per second at 26.5 eV. The source is based on high-harmonic generation (HHG) in argon and pumped by a frequency-doubled 100 kHz repetition…
We report the generation of a purely vibrational Raman comb, extending from the vacuum ultraviolet (184 nm) to the visible (478 nm), in hydrogen-filled kagom\'e-style photonic crystal fiber pumped at 266 nm. Stimulated Raman scattering and…
The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…
Extreme ultraviolet (XUV) light sources allow for the probing of bound electron dynamics on attosecond scales, interrogation of high-energy-density matter, and access to novel regimes of strong-field quantum electrodynamics. Despite the…
Coherent supercontinuum radiation in the extreme-ultraviolet (XUV) range is indispensable for synthesizing attosecond light pulses and for exploring transient atomic structures. Here, we report the striking observations of coherent XUV…
When a laser pump beam of sufficient intensity is incident on a Raman-active medium such as hydrogen gas, a strong Stokes signal, red-shifted by the Raman transition frequency {\Omega}$_R$, is generated. This is accompanied by the creation…
The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear…
We introduce a novel ultra-broadband ultraviolet and visible frequency comb light source covering more than 240 THz by resonant dispersive wave emission in a gas-filled hollow-core fiber waveguide. The light source allows tuning from ~340…
Laser spectroscopy of the $^{\mathrm{229m}}$Th nuclear clock transition is necessary for the future construction of a nuclear-based optical clock. Precision laser sources with broad spectral coverage in the vacuum ultraviolet are needed for…
Ultrafast electron dynamics drive phenomena such as photochemical reactions, catalysis, and light harvesting. To capture such dynamics in real-time, femtosecond to attosecond light sources are extensively used. However, an exact match…
Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of…
We report on two types of Raman laser sources emitting in the near and middle ultraviolet spectral ranges by the use of a solarization-resilient gas-filled inhibited-coupling (IC) hollow-core photonic-crystal fiber (HCPCF) with record low…