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We have performed multicanonical computer simulations of a small system of short protein-like heteropolymers and found that their aggregation transition possesses similarities to first-order phase separation processes. Not being a phase…

Soft Condensed Matter · Physics 2024-05-22 Christoph Junghans , Michael Bachmann , Wolfhard Janke

Thermoresponsive microgels are polymeric colloidal networks that can change their size in response to a temperature variation. This peculiar feature is driven by the nature of the solvent-polymer interactions, which triggers the so-called…

Soft Condensed Matter · Physics 2019-02-08 Fabrizio Camerin , Nicoletta Gnan , Lorenzo Rovigatti , Emanuela Zaccarelli

We present results from extensive molecular dynamics simulations of collapse transitions of hydrophobic polymers in explicit water focused on understanding effects of lengthscale of the hydrophobic surface and of attractive interactions on…

Statistical Mechanics · Physics 2007-05-23 Manoj V. Athawale , Gaurav Goel , Tuhin Ghosh , Thomas M. Truskett , Shekhar Garde

Results of torsional oscillation tests are reported that were performed at the temperature T=230C on melts of a hybrid nanocomposite consisting of isotactic polypropylene reinforced with 5 wt.% of montmorillonite clay. Prior to mechanical…

Materials Science · Physics 2007-05-23 A. D. Drozdov , A. Al-Mulla , D. A. Drozdov , R. K. Gupta

A high level polarizable force field is used to study the temperature dependence of hydrophobic hydration of small-sized molecules from computer simulations. Molecular dynamics (MD) simulations of liquid water at various temperatures form…

Biological Physics · Physics 2007-11-27 R. Mahajan , D. Krazmueller , U. H. E. Hansmann , J. Volkert , S. Hoefinger

Laser-based metal processing including welding and three dimensional printing, involves localized melting of solid or granular raw material, surface tension-driven melt flow and significant evaporation of melt due to the applied very high…

Computational Engineering, Finance, and Science · Computer Science 2021-05-05 Christoph Meier , Sebastian L. Fuchs , A. John Hart , Wolfgang A. Wall

By means of atomistic molecular dynamics simulations we investigate the behaviour of poly(N-isopropylacrylamide), PNIPAM, in water at temperatures below and above the lower critical solution temperature (LCST), including the undercooled…

Soft Condensed Matter · Physics 2019-02-11 L. Tavagnacco , E. Zaccarelli , E. Chiessi

Recent cutting-edge experiments have provided {\it in situ} structure characterization and measurements of the pressure ($P$), density ($\bar{\rho}$) and temperature ($T$) of shock compressed silicon in the 100 GPa range of pressures and…

Materials Science · Physics 2024-12-12 M. W. C. Dharma-wardana , Dennis D. Klug , Hannah Poole , G. Gregori

Temperature dependence of the capacitance of the electrical double layer (EDL) in concentrated electrolytes/ionic liquids has been under debates for decades. To rationalise the capacitance vs temperature dependence, we run molecular…

Soft Condensed Matter · Physics 2020-05-26 Vladislav B Ivaništšev , Kathleen Kirchner , Maxim V. Fedorov

We study the aggregation of peptides using the discrete molecular dynamics simulations. At temperatures above the alpha-helix melting temperature of a single peptide, the model peptides aggregate into a multi-layer parallel beta-sheet…

Soft Condensed Matter · Physics 2009-11-10 S. Peng , F. Ding , B. Urbanc , S. V. Buldyrev , L. Cruz , H. E. Stanley , N. V. Dokholyan

Electrostatic interactions in polymeric systems are responsible for a wide range of liquid-liquid phase transitions that are of importance for biology and materials science. Such transitions are referred to as complex coacervation, and…

Soft Condensed Matter · Physics 2023-09-29 Boyuan Yu , Heyi Liang , Paul F. Nealey , Matthew Tirrell , Artem M. Rumyantsev , Juan J. de Pablo

We present a multiscale modeling approach that integrates molecular dynamics simulations, machine learning, and the Elastically Collective Nonlinear Langevin Equation (ECNLE) theory to investigate the glass transition dynamics of polymer…

Soft Condensed Matter · Physics 2026-01-21 Nguyen T. T. Duyen , Ngo T. Que , Anh D. Phan

Linearly-sloped or `ramp' potentials belong to a class of core-softened models which possess a liquid-liquid critical point (LLCP) in addition to the usual liquid-gas critical point. Furthermore they exhibit thermodynamic anomalies in the…

Statistical Mechanics · Physics 2009-11-11 Helen M. Gibson , Nigel B. Wilding

For warm and hot dense plasma (WHDP), the ionization potential depression (IPD) is a key physical parameter in determining its ionization balance, therefore a reliable and universal IPD model is highly required to understand its microscopic…

Plasma Physics · Physics 2023-05-17 Chensheng Wu , Fuyang Zhou , Yong Wu , Jun Yan , Xiang Gao , Jianguo Wang

We simulate high-pressure hydrogen in its liquid phase close to molecular dissociation using a machine-learned interatomic potential. The model is trained with density functional theory (DFT) forces and energies, with the…

Statistical Mechanics · Physics 2024-12-20 Mathieu Istas , Scott Jensen , Yubo Yang , Markus Holzmann , Carlo Pierleoni , David M. Ceperley

We present the exact solution of a microscopic statistical mechanical model for the transformation of a long polypeptide between an unstructured coil conformation and an $\alpha$-helix conformation. The polypeptide is assumed to be adsorbed…

Soft Condensed Matter · Physics 2015-01-30 Ganga P. Sharma , Yana K. Reshetnyak , Oleg A. Andreev , Michael Karbach , Gerhard Müller

Computer simulations can provide mechanistic insight into ionic liquids (ILs) and predict the properties of experimentally unrealized ion combinations. However, ILs suffer from a particularly large disparity in the time scales of atomistic…

The ground states of noninteracting fermions in one-dimension with chiral symmetry form a class of topological band insulators, described by a topological invariant that can be related to the Zak phase. Recently, a generalization of this…

Strongly Correlated Electrons · Physics 2023-04-05 Paolo Molignini , Nigel Cooper

Solid-solid collapse transition in open framework structures is ubiquitous in nature. The real difficulty in understanding detailed microscopic aspects of such transitions in molecular systems arises from the interplay between different…

Soft Condensed Matter · Physics 2015-06-15 Rakesh S. Singh , Biman Bagchi

We consider the thermodynamics of a homogeneous superfluid dilute Bose gas in the presence of weak quenched disorder. Following the zero-temperature approach of Huang and Meng, we diagonalize the Hamiltonian of a dilute Bose gas in an…

Other Condensed Matter · Physics 2010-02-05 G. M. Falco , A. Pelster , R. Graham