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We explore the quantum dynamics of nuclear spin relaxation in cold collisions of $^1\Sigma^+$ molecules with structureless atoms in an external magnetic field. To this end, we develop a rigorous coupled-channel methodology, which accounts…

Chemical Physics · Physics 2023-06-29 Rebekah Hermsmeier , Xiaodong Xing , Timur V. Tscherbul

The low temperature relaxation of the magnetization in magnetic molecular solids such as Fe$_8$ is studied using Monte Carlo simulations. A set of rate equations is developed to understand the simulations, and the results are compared. The…

Statistical Mechanics · Physics 2015-10-14 Avinash Vijayaraghavan , Anupam Garg

A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. Morello , A. Millán , L. J. de Jongh

We model magnetization processes that take place through tunneling in crystals of single-molecule magnets, such as Mn_12 and Fe_8. These processes take place when a field H is applied after quenching to very low temperatures. Magnetic…

Statistical Mechanics · Physics 2007-05-23 J. F. Fernandez , J. J. Alonso

A kinetic Ising model is analyzed where spin variables correspond to lattice cells with mobile or immobile particles. Introducing additional restrictions for the flip processes according to the n-spin facilitated kinetic Ising model and…

Disordered Systems and Neural Networks · Physics 2009-10-31 B. Zheng , M. Schulz , S. Trimper

Single molecule magnets (SMMs) with single-ion anisotropies $\mathbf d$, comparable to exchange interactions J, between spins have recently been synthesized. In this paper, we provide theoretical insights into the magnetism of such systems.…

Strongly Correlated Electrons · Physics 2017-11-22 Sumit Haldar , Rajamani Raghunathan , Jean-Pascal Sutter , S. Ramasesha

The prospects of sympathetic cooling of polar molecules with magnetically co-trapped alkali-metal atoms are generally considered poor due to strongly anisotropic atom-molecule interactions leading to large spin relaxation rates. Using…

Atomic Physics · Physics 2012-02-06 T. V. Tscherbul , J. Klos , A. A. Buchachenko

The three-dimensional anisotropic classical XY ferromagnet has been investigated by extensive Monte Carlo simulation using the Metropolis single spin flip algorithm. The magnetization ($M$) and the susceptibility ($\chi$) are measured and…

Statistical Mechanics · Physics 2023-09-26 Olivia Mallick , Muktish Acharyya

Magnetic properties of the intermetallic compound NdCo$_2$Si$_2$ are investigated by using the Monte Carlo simulation (MCs) under Metropolis algorithm. The magnetism of the compound is caused by the existence of the rare earth (Nd3+) ions…

Materials Science · Physics 2019-12-10 R. Khalladi , S. Idrissi , S. Mtougui , I. El Housni , S. Ziti , H. Labrim , N. El Mekkaoui , L. Bahmad

We report that the major features in the temperature dependence of dc and ac magnetization of a well-known spin-chain compound, Ca3Co2O6, which has been known to exhibit two complex magnetic transitions due to geometrical frustration (one…

Strongly Correlated Electrons · Physics 2015-05-13 Niharika Mohapatra , Kartik K Iyer , Sitikantha D Das , B. A. Chalke , S. C. Purandare , E. V. Sampathkumaran

We present an accurate quantum mechanical study of molecule-molecule collisions in the presence of a magnetic field. The work focusses on the analysis of elastic scattering and spin relaxation in collisions of O2(3Sigma_g) molecules at cold…

Atomic Physics · Physics 2012-02-06 T. V. Tscherbul , Yu. V. Suleimanov , V. Aquilanti , R. V. Krems

Artificial Spin Ice (ASI), consisting of a two dimensional array of nanoscale magnetic elements, provides a fascinating opportunity to observe the physics of out of equilibrium systems. Initial studies concentrated on the static, frozen…

The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…

Mesoscale and Nanoscale Physics · Physics 2009-07-21 P. Maletinsky , M. Kroner , A. Imamoglu

A quantum mechanical close coupling theory of spin relaxation in the stretched hyperfine level of sodium is presented. We calculate the dipolar relaxation rate of magnetically trapped cold sodium atoms in the magnetic field. The influence…

Atomic Physics · Physics 2007-05-23 B. Zygelman

We study the magnetisation dynamics of a bulk single crystal Cr$_2$Ge$_2$Te$_6$ (CGT), by means of broadband ferromagnetic resonance (FMR), for temperatures from 60 K down to 2 K. We determine the Kittel relations of the fundamental FMR…

Materials Science · Physics 2019-11-05 S. Khan , C. W. Zollitsch , D. M. Arroo , H. Cheng , I. Verzhbitskiy , A. Sud , Y. P. Feng , G. Eda , H. Kurebayashi

We consider a simple model of maghemite nanoparticles and study their magnetic properties using Monte Carlo methods. The particles have a spherical geometry with diameters ranging from 3 nm to 8 nm. The interior of the particles consists of…

Statistical Mechanics · Physics 2015-03-13 K. Adebayo , B. W. Southern

Motivated by the recent suggestion of anisotropic effective exchange interactions between Mn spins in Ga$_{1-x}$Mn$_x$As (arising as a result of spin-orbit coupling), we study their effects in diluted Heisenberg spin systems. We perform…

Disordered Systems and Neural Networks · Physics 2007-05-23 Chenggang Zhou , Malcolm P. Kennett , Xin Wan , Mona Berciu , R. N. Bhatt

This article takes a broad view of the understanding of magnetic bistability and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on three families of relatively simple, low-nuclearity transition metal clusters: spin S…

A cluster Monte Carlo method for systems of classical spins with purely dipolar couplings is presented. It is tested and applied for finite arrays of perpendicular Ising dipoles on the triangular lattice. This model is a modification with…

Statistical Mechanics · Physics 2009-11-07 Ulrich K. Roessler

We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. J. Graf , A. Lascialfari , F. Borsa , A. M. Tkachuk , B. Barbara