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Electron energy loss spectroscopy (EELS) is often utilized to characterize localized surface plasmon modes supported by plasmonic antennas. However, the spectral resolution of this technique is only mediocre, and it can be rather difficult…

Recent developments in experiments with vibrational electron energy loss spectroscopy (EELS) have revealed spectral shape variations at spatial resolutions down to sub-atomic scale. Interpretation in terms of local phonon density of states…

Materials Science · Physics 2021-09-15 Paul M. Zeiger , Ján Rusz

A fully relativistic description of the electron energy loss and the induced radiation emission in arbitrary arrays of non-overlapping metallic cylinders is presented in terms of the multiple scattering method on the basis of vector…

Materials Science · Physics 2009-11-10 T. Ochiai , K. Ohtaka

Direct measurement of local phonon dispersion in individual nanostructures can greatly advance our understanding of their electrical, thermal, and mechanical properties. However, such experimental measurements require extremely high…

Mesoscale and Nanoscale Physics · Physics 2021-03-02 Ruishi Qi , Ning Li , Jinlong Du , Ruochen Shi , Yang Huang , Xiaoxia Yang , Lei Liu , Zhi Xu , Qing Dai , Dapeng Yu , Peng Gao

Noble metal nanoparticles have been utilized for a vast amount of optical applications. For the applications that used metal nanoparticles as nanosensors and optical labeling, larger radiation damping is preferred (higher optical signal).…

Optics · Physics 2022-03-02 Yanhe Yang , Weihai Ni , Hao Xie , Jian You , Weixiang Ye

Engineering nanophotonic mode dispersions in ultrathin, planar structures enables significant control over infrared perfect absorption (PA) and thermal emission characteristics. Here, using simulations, the wavelength and angular ranges…

Optics · Physics 2022-01-14 Ben Johns , Shashwata Chattopadhyay , Joy Mitra

Scanning transmission electron microscopy (STEM) combined with electron energy loss spectroscopy (EELS) has become a standard technique to map localized surface plasmon resonances with a nanometer spatial and a sufficient energy resolution…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 Michal Horák , Tomáš Šikola

Swift electrons passing near or through metallic structures have proven to be an excellent tool for studying plasmons and other types of confined optical modes involving collective charge oscillations in the materials hybridized with…

Electron energy-loss spectroscopy (EELS) performed in transmission electron microscopes is shown to directly render the photonic local density of states (LDOS) with unprecedented spatial resolution, currently below the nanometer. Two…

Materials Science · Physics 2012-11-13 F. J. Garcia de Abajo , M. Kociak

Measuring nanoscale local temperatures, particularly in vertically integrated and multi-component systems, remains challenging. Spectroscopic techniques like X-ray absorption and core-loss electron energy-loss spectroscopy (EELS) are…

Orientation dependent electronic properties of wurtzite zinc oxide nanorods are characterized by aloof beam electron energy-loss spectroscopy (EELS) carried out in a scanning transmission electron microscope (STEM). The two key crystal…

Materials Science · Physics 2021-10-06 Yao-Wen Yeh , Sobhit Singh , David Vanderbilt , Philip E. Batson

A periodic arrangement of 2D conducting planes is known to host a (bulk) plasmon dispersion that interpolates between the typical, gapped behavior of 3D metals and a gapless, acoustic regime as a function of the out-of-plane wavevector. The…

Strongly Correlated Electrons · Physics 2022-11-09 Christian Boyd , Luke Yeo , Philip W. Phillips

The polarization- and angle- resolved optical response of the anapole mode in silicon nano-disks array have been experimentally and theoretically investigated. The good agreement betweenmeasured data and simulations yields to a consistent…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Lucia Fornasari , Marco Passoni , Franco Marabelli , Yuyao Chen , Yu Wang , Luca Dal Negro

We report a novel behavior of the surface plasmon linewidth in sodium nanospheres Na$_{1760}$ changing with the electron temperature, which monotonically decreases and bears a discontinuous sudden drop at high electron temperatures. Our…

Mesoscale and Nanoscale Physics · Physics 2014-08-15 Guozhong Wang , Yizhuang Zheng , Jian Zi

Versatile quantum modes emerge for plasmon describing the collective oscillations of free electrons in metallic nanoparticles when the particle sizes are greatly reduced. Rather than traditional nanoscale study, the understanding of quantum…

Over the last two decades, Electron Energy Loss Spectroscopy (EELS) imaging with a scanning transmission electron microscope (STEM) has emerged as a technique of choice for visualizing complex chemical, electronic, plasmonic, and phononic…

The electronic structure and optical properties of metallic nanoshells are investigated using a jellium model and the Time Dependent Local Density Approximation (TDLDA). An efficient numerical implementation enables applications to…

Materials Science · Physics 2009-11-10 P. Nordlander , E. Prodan

We propose a setup enabling electron energy loss spectroscopy to determine the density of the electrons accumulated by an electro-positive dielectric in contact with a plasma. It is based on a two-layer structure inserted into a recess of…

Applied Physics · Physics 2020-01-08 E. Thiessen , F. X. Bronold , H. Fehske

We provide a self-consistent electromagnetic theory of the coupling between dipole emitters and dissipative nanoresonators. The theory that relies on the concept of quasi-normal modes with complex frequencies provides an accurate…

Mesoscale and Nanoscale Physics · Physics 2017-05-25 C. Sauvan , J. P. Hugonin , I. S. Maksymov , P. Lalanne

Within the MNPBEM toolbox, we show how to simulate electron energy loss spectroscopy (EELS) of plasmonic nanoparticles using a boundary element method approach. The methodology underlying our approach closely follows the concepts developed…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Ulrich Hohenester