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We investigate excitonic transitions in a h-BN encapsulated monolayer $\textrm{MoS}_2$ phototransistor by photocurrent spectroscopy at cryogenic temperature (T = 5 K). The spectra presents excitonic peaks with linewidths as low as 8 meV,…

We have studied the low-energy electronic excitations of solid picene at 20 K using momentum dependent electron energy-loss spectroscopy. Our results demonstrate the presence of five excitonic features below the transport energy gap of…

Materials Science · Physics 2011-04-28 Friedrich Roth , Benjamin Mahns , Bernd Büchner , Martin Knupfer

Several theoretical predictions have claimed that the neutral exciton of TMDCs splits into a transversal and longitudinal exciton branch, with the longitudinal one, which is the upper branch, exhibiting an extraordinary strong dispersion in…

Mesoscale and Nanoscale Physics · Physics 2020-05-29 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Atomistically detailed computational studies of nanocrystals, such as those derived from the promising lead-halide perovskites, are challenging due to the large number of atoms and lack of symmetries to exploit. Here, focusing on…

Materials Science · Physics 2022-10-05 Giulia Biffi , Yeongsu Cho , Roman Krahne , Timothy C. Berkelbach

We report an experimental study of excitons in a double quantum well van der Waals heterostructure made of atomically thin layers of \Mo* and hexagonal boron nitride (hBN). The emission of neutral and charged excitons is controlled by gate…

Mesoscale and Nanoscale Physics · Physics 2016-03-14 E. V. Calman , C. J. Dorow , M. M. Fogler , L. V. Butov , S. Hu , A. Mishchenko , A. K. Geim

Monolayer C$_3$N is an emerging two-dimensional indirect band gap semiconductor with interesting mechanical, thermal, and electronic properties. In this work we present a description of C$_3$N electronic and dielectric properties, focusing…

Mesoscale and Nanoscale Physics · Physics 2022-04-26 Miki Bonacci , Matteo Zanfrognini , Elisa Molinari , Alice Ruini , Marilia J. Caldas , Andrea Ferretti , Daniele Varsano

Optical properties of transition metal dichalcogenides monolayers are controlled by the Wannier-Mott excitons forming a series of $1s$, $2s$, $2p$,... hydrogen-like states. We develop the theory of the excited excitonic states energy…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 M. M. Glazov , L. E. Golub , G. Wang , X. Marie , T. Amand , B. Urbaszek

The photoluminescence spectra of spherical CdTe nanocrystals with zincblende structure are studied by size-selective spectroscopic techniques. We observe a resonant Stokes shift of 15 meV when the excitation laser energy is tuned to the red…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee , M. Chamarro , P. Lavallard , V. D. Petrikov , A. A. Lipovskii

The excitonic behavior of anisotropic two-dimensional crystals is investigated using numerical methods. We employ a screened potential arising due to the system polarizability to solve the central-potential problem using the Numerov…

Mesoscale and Nanoscale Physics · Physics 2014-08-28 A. S. Rodin , A. Carvalho , A. H. Castro Neto

Controlling interlayer excitons in van der Waals heterostructures holds promise for exploring Bose-Einstein condensates and developing novel optoelectronic applications, such as excitonic integrated circuits. Despite intensive studies,…

Mesoscale and Nanoscale Physics · Physics 2024-04-09 Lifu Zhang , Ruihao Ni , Liuxin Gu , Ming Xie , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , You Zhou

We present experimental and theoretical results on the high-quality single-layer MoS$_{2}$ which reveal the fine structure of charged excitons, i.e., trions. In the emission spectra we resolve and identify two trion peaks, T$_{1}$ and…

We examine the excitonic nature of high-lying optical transitions in single-walled carbon nanotubes by means of Rayleigh scattering spectroscopy. A careful analysis of the principal transitions of individual semiconducting and metallic…

Mesoscale and Nanoscale Physics · Physics 2010-01-27 Stephane Berciaud , Christophe Voisin , Hugen Yan , Bhupesh Chandra , Robert Caldwell , Yuyao Shan , Louis E. Brus , James Hone , Tony F. Heinz

van der Waals stacking of two-dimensional (2D) materials offers a powerful platform for engineering material interfaces with tailored electronic and optical properties. While most van der Waals multilayers have featured inorganic…

Excitons in monolayer transition-metal dichalcogenides (TMDs) have garnered significant attention because of their large binding energies due to weakly screened Coulomb interaction, and direct bandgap at the K/K$^\prime$ point in the…

We report first-principles calculations of the effects of quasiparticle self-energy and electron-hole interaction on the optical properties of single-walled BN nanotubes. Excitonic effects are shown to be even more important in BN nanotubes…

Materials Science · Physics 2007-08-23 Cheol-Hwan Park , Catalin D. Spataru , Steven G. Louie

The measurement and manipulation of the coherent dynamics of excitonic states constitute a forefront research challenge in semiconductor optics and in quantum coherence-based protocols for optoelectronic technologies. Layered semiconductors…

The peculiar crystal structure of one-dimensional molecular solids originates from packing of an array of molecules in which intermolecular interactions are dominantly dispersive, including hydrogen-bond, van der Waals and London-type…

Mesoscale and Nanoscale Physics · Physics 2019-05-06 E. Nji Nde Aboringong , Alain M. Dikandé

Composite quasi-particles with emergent functionalities in spintronic and quantum information science can be realized in correlated materials due to entangled charge, spin, orbital, and lattice degrees of freedom. Here we show that by…

Boron nitride single layer belongs to the family of 2D materials whose optical properties are currently receiving considerable attention. Strong excitonic effects have already been observed in the bulk and still stronger effects are…

We propose a robust and efficient way of controlling the optical spectra of two-dimensional materials and van der Waals heterostructures by quantum cavity embedding. The cavity light-matter coupling leads to the formation of…

Mesoscale and Nanoscale Physics · Physics 2019-06-19 Simone Latini , Enrico Ronca , Umberto de Giovannini , Hannes Hübener , Angel Rubio