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Detailed information on the electronic states of both V and Mn 3d electrons in the ferrimagnet Mn2VAl is obtained by the bulk sensitive resonant inelastic soft x-ray scattering (SX-RIXS) excited with the circularly polarized light under an…

We show that, contrary to common lore, in resonant inelastic x-ray scattering (RIXS) at the copper L- and M-edge direct spin-flip scattering is in principle allowed. We demonstrate how this possibility can be exploited to probe the momentum…

Strongly Correlated Electrons · Physics 2015-05-13 L. J. P. Ament , G. Ghiringhelli , M. Moretti Sala , L. Braicovich , J. van den Brink

Core hole resonance is used in X-ray spectroscopy to incisively probe the local electronic states of many-body systems. Here, resonant inelastic X-ray scattering (RIXS) is studied as a function of incident photon energy on Mott insulators…

Strongly Correlated Electrons · Physics 2016-12-14 L. Andrew Wray , Shih-Wen Huang , Yuqi Xia , M. Zahid Hasan , Charles Mathy , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

We have performed a resonant x-ray scattering (RXS) study near the Co K edge on a single crystal of Ca3Co2O6. In the magnetically ordered phase a new class of weak reflections appears at the magnetic propagation vector tau (1/3,1/3,1/3).…

Strongly Correlated Electrons · Physics 2009-11-13 A. Bombardi , C. Mazzoli , S. Agrestini , M. R. Lees

In the high spin-orbit coupled Sr2IrO4, the high sensitivity of the ground state to the details of the local lattice structure shows a large potential for the manipulation of the functional properties by inducing local lattice distortions.…

Chromium tri-halides Cr$X_3$ ($X$ = Cl, Br, and I) have recently become a focal point of research due to their intriguing low-temperature,layer-dependent magnetism that can be manipulated by an electric field. This makes them essential…

The strongly correlated insulator Ca$_{2}$RuO$_4$ is considered as a paradigmatic realization of both spin-orbital physics and a band-Mott insulating phase, characterized by orbitally selective coexistence of a band and a Mott gap. We…

X-ray absorption is the standard method to probe the unoccupied density of states at a given edge. Here we show that polarized Resonant Inelastic X-Ray Scattering in La2CuO4 at the Cu K-edge is extremely sensitive to the environment of the…

Strongly Correlated Electrons · Physics 2009-11-11 A. Shukla , M. Calandra , M. Taguchi , A. Kotani , G. Vanko , S-W. Cheong

We compute the K-edge indirect resonant inelastic x-ray scattering (RIXS) spectrum of a triangular lattice antiferromagnet in its ordered coplanar 3- sublattice 120 degree magnetic state. By considering the first order self$-$energy…

Materials Science · Physics 2015-07-07 Cheng Luo , Trinanjan Datta , Zengye Huang , Dao-Xin Yao

We have investigated the excitation spectra of $j_{eff}$=$\frac{1}{2}$ Mott insulator Na$_2$IrO$_3$. Taking into account a relativistic multiplet structure of Ir ions, we have calculated the optical conductivity $\sigma(\omega)$ and…

Strongly Correlated Electrons · Physics 2014-02-25 Beom Hyun Kim , G. Khaliullin , B. I. Min

We report empirical comparisons of Cu K-edge indirect resonant inelastic x-ray scattering (RIXS) spectra, taken at the Brillouin zone center, with optical dielectric loss functions measured in a number of copper oxides. The RIXS data are…

Strongly Correlated Electrons · Physics 2010-04-02 Jungho Kim , D. S. Ellis , H. Zhang , J. P. Hill , F. C. Chou , T. Gog , D. Casa , Young-June Kim

The results of investigations of intercalated compounds Cr_xTiSe_2 and Co_xTiSe_2 by X-ray photoelectron spectroscopy (XPS) and X-ray emission spectroscopy (XES) are presented. The data obtained are compared with theoretical results of…

We present a microscopic theory of resonant soft x-ray scattering (RSXS) that accounts for the delocalized character of valence electrons. Unlike past approaches defined in terms of form factors for atoms or clusters, we develop a…

Strongly Correlated Electrons · Physics 2013-04-08 David Benjamin , Dmitry Abanin , Peter Abbamonte , Eugene Demler

We study the magnetic excitation spectra of L-edge resonant inelastic x-ray scattering (RIXS) from the spin singlet ground state in one-dimensional undoped cuprates. Analyzing the transition amplitudes of the magnetic excitations in the…

Strongly Correlated Electrons · Physics 2013-05-30 Jun-ichi Igarashi , Tatsuya Nagao

The development of high-brightness free-electron lasers (FEL) has revolutionised our ability to create and study matter in the high-energy-density (HED) regime. Current diagnostic techniques have been very successful in yielding information…

We have studied the local electronic structure of LaMn0.5Co0.5O3 using soft-x-ray absorption spectroscopy at the Co-L_3,2 and Mn-L_3,2 edges. We found a high-spin Co^{2+}--Mn^{4+} valence state for samples with the optimal Curie…

Strongly Correlated Electrons · Physics 2008-03-18 T. Burnus , Z. Hu , H. H. Hsieh , V. L. J. Joly , P. A. Joy , M. W. Haverkort , Hua Wu , A. Tanaka , H. -J. Lin , C. T. Chen , L. H. Tjeng

Resonant inelastic x-ray scattering (RIXS) has become an important tool for studying elementary excitations in correlated materials. Here, we present a systematic theoretical investigation of the Cu L-edge RIXS spectra of undoped and doped…

Strongly Correlated Electrons · Physics 2019-05-22 Umesh Kumar , Alberto Nocera , Elbio Dagotto , Steven Johnston

The low energy excitations in Na2IrO3 have been investigated using resonant inelastic x-ray scattering (RIXS). A magnetic excitation branch can be resolved, whose dispersion reaches a maximum energy of about 35 meV at the \Gamma-point. The…

Strongly Correlated Electrons · Physics 2013-07-08 H. Gretarsson , J. P. Clancy , Yogesh Singh , P. Gegenwart , J. P. Hill , Jungho Kim , M. H. Upton , A. H. Said , D. Casa , T. Gog , Young-June Kim

Soft X-ray resonant scattering (XRS) has been used to observe directly, for the first time, the ordering of localized electronic states on both the Mn and Tb sites in multiferroic TbMnO$_3$. Large resonant enhancement of the X-ray…

Resonant-magnetic x-ray scattering (RMXS) near the vanadium $L_{2,3}$-absorption edges has been used to investigate the low temperature magnetic structure of high quality \bvs\ single crystals. Below $T_N$ = 31 K, the strong resonance…

Strongly Correlated Electrons · Physics 2011-04-27 Ph. Leininger , V. Ilakovac , Y. Joly , E. Schierle , E. Weschke , O. Bunau , H. Berger , J. -P. Pouget , P. Foury-Leylekian