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We analyze the resonant inelastic x-ray scattering (RIXS) spectra at the K edge of Mn in the antiferromagnetic insulating manganite LaMnO3. We make use of the Keldysh-type Green-function formalism, in which the RIXS intensity is described…

Strongly Correlated Electrons · Physics 2009-11-13 Taeko Semba , Manabu Takahashi , Junichi Igarashi

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

We investigate electronic excitations in La2-x(Br,Sr)xCuO4 using resonant inelastic x-ray scattering (RIXS) at the oxygen K edge. RIXS spectra of the hole-doped cuprates show clear momentum dependence below 1 eV. The spectral weight…

Strongly Correlated Electrons · Physics 2017-09-26 K. Ishii , T. Tohyama , S. Asano , K. Sato , M. Fujita , S. Wakimoto , K. Tustsui , S. Sota , J. Miyawaki , H. Niwa , Y. Harada , J. Pelliciari , Y. Huang , T. Schmitt , Y. Yamamoto , J. Mizuki

We study the magnetic resonant x-ray scattering (RXS) spectra around the $K$ edge of Cu in KCuF$_3$ on the basis of an {\em ab initio} calculation. We use the full-potential linearlized augmented plane wave method in the LDA$+U$ scheme, and…

Strongly Correlated Electrons · Physics 2009-11-07 M. Takahashi , M. Usuda , J. Igarashi

We have performed neutron inelastic scattering and resonant inelastic X-ray scattering (RIXS) at the Cu-$L_3$ edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La$_{2-x}$Sr$_{x}$CuO$_{4}$…

We report on the Cu 1s resonant inelastic X-ray scattering (RIXS) of Cu-O one-dimensional (1D) strongly correlated insulator systems with contrasting atomic arrangements, namely edge-sharing CuGeO3 and corner-sharing Sr2CuO3. Owing to good…

Strongly Correlated Electrons · Physics 2009-11-11 S. Suga , S. Imada , A. Higashiya , A. Shigemoto , S. Kasai , M. Sing , H. Fujiwara , A. Sekiyama , A. Yamasaki , C. Kim , T. Nomura , J. Igarashi , M. Yabashi , T. Ishikawa

We report on a combined soft x-ray absorption and magnetic circular dichroism (XMCD) study at the Co-$L_{3,2}$ on the hybrid 3$d$/5$d$ solid state oxide Sr$_2$Co$_{0.5}$Ir$_{0.5}$O$_4$ with the K$_2$NiF$_4$ structure. Our data indicate…

Strongly Correlated Electrons · Physics 2017-06-28 S. Agrestini , C. -Y. Kuo , D. Mikhailova , K. Chen , P. Ohresser , T. W. Pi , H. Guo , A. C. Komarek , A. Tanaka , Z. Hu , L. H. Tjeng

The structural, magnetic and electronic properties of transition metal oxides reflect in atomic charge, spin and orbital degrees of freedom. Resonant x-ray scattering (RXS) allows us to perform an accurate investigation of all these…

Strongly Correlated Electrons · Physics 2015-05-14 G. Subías , Joaquín García , Blasco Javier , Javier Herrero-Martin , María Concepción Sanchez

Several nonlinear spectroscopy experiments which employ broadband x-ray pulses to probe the coupling between localized core and delocalized valence excitation are simulated for the amino acid cysteine at the K-edges of oxygen and nitrogen…

Chemical Physics · Physics 2015-06-15 Jason D. Biggs , Yu Zhang , Daniel Healion , Shaul Mukamel

The manifestation of skyrmions in the Mott-insulator Cu$_2$OSeO$_3$ originates from a delicate balance between magnetic and electronic energy scales. As a result of these intertwined couplings, the two symmetry-inequivalent magnetic ions,…

For the Sr2-xIrO4 system, recent work pointed out the abnormal electronic and magnetic properties around the critical point. Here, to understand Sr-vacancy effect on spin-orbit coupled Mott insulator Sr2IrO4, the electronic structure and…

Strongly Correlated Electrons · Physics 2019-01-07 Jie Cheng , Shengli Liu , Bin Li , Haiyun Wang , Yu Wang , Wei Xu

In a recent publication Larson \textit{et al.} reported remarkably clear $d$-$d$ excitations for NiO and CoO measured with x-ray energies well below the transition metal $K$ edge. In this letter we demonstrate that we can obtain an accurate…

Strongly Correlated Electrons · Physics 2008-01-09 M. W. Haverkort , A. Tanaka , L. H. Tjeng , G. A. Sawatzky

We present a temperature and doping dependent resonant inelastic X-ray scattering experiment at the V L$_{2,3}$ and O K edges in La$_{1-x}$Sr$_x$VO$_3$ for $x=0$ and $x=0.1$. This material is a canonical example of a compound that exhibits…

We performed a resonant inelastic X-ray scattering (RIXS) study of La$_{2-x}$Sr$_{x}$NiO$_{4+{\delta}}$ (LSNO) at the oxygen $K$ edge to investigate the nature of the doped holes with regard to charge excitations. Charge excitations of the…

Resonant inelastic x-ray scattering (RIXS) experiment was performed at the Mn $L_3$ edge. A 10 $\%$ Mn-doped Sr$_{3}$Ru$_{2}$O$_{7}$ compound, where the Mn$^{3+}$ ions are in the 3$d^4$ state, were probed for $dd$ excitations. The dilute…

We present a detailed study of the Ti 3$d$ carriers at the interface of LaAlO$_3$/SrTiO$_3$ heterostructures by high-resolution resonant inelastic soft x-ray scattering (RIXS), with special focus on the roles of overlayer thickness and…

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

Strongly Correlated Electrons · Physics 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

Resonant inelastic x-ray scattering at the N K edge reveals clearly resolved harmonics of the anion plane vibrations in the kappa-(BEDT-TTF)2Cu2(CN)3 spin-liquid insulator. Tuning the incoming light energy at the K edge of two distinct N…

We have investigated the valence, spin, and orbital state of the Co ions in the one-dimensional cobaltate Ca3Co2O6 using x-ray absorption and x-ray magnetic circular dichroism at the Co-L2,3 edges. The Co ions at both the octahedral Co_oct…

Strongly Correlated Electrons · Physics 2007-05-23 T. Burnus , Z. Hu , M. W. Haverkort , J. C. Cezar , D. Flahaut , V. Hardy , A. Maignan , N. B. Brookes , A. Tanaka , H. -H. Hsieh , H. -J. Lin , C. -T. Chen , L. H. Tjeng

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

Strongly Correlated Electrons · Physics 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov
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