English
Related papers

Related papers: Recent developments in MAS DNP-NMR of materials

200 papers

Nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) are well-established techniques that provide valuable information in a diverse set of disciplines but are currently limited to macroscopic sample volumes. Here we…

Dynamic Nuclear Polarization (DNP) presently stands as the preferred strategy to enhance the sensitivity of nuclear magnetic resonance measurements, but its application relies on the use of high-frequency microwave to manipulate electron…

Mesoscale and Nanoscale Physics · Physics 2022-02-02 Carlos A. Meriles , Pablo R. Zangara

We report measurements of enhanced tensor polarization on solid-state targets. The results here represent an increase in tensor polarization over that previously achieved in high energy and nuclear scattering experiments that focused on the…

Instrumentation and Detectors · Physics 2020-08-24 Dustin Keller , Don Crabb , Donal Day

Dynamic nuclear polarization (DNP) is an important method to enhance the limited sensitivity of nuclear magnetic resonance (NMR). Using the existing mechanisms such as Overhauser DNP (ODNP) is still difficult to achieve significant…

Chemical Physics · Physics 2025-03-31 Maria Grazia Concilio , Yiwen Wang , Linjun Wang , Xueqian Kong

Resistively-detected NMR (RDNMR) is a unique characterization method enabling highly-sensitive NMR detection for a single quantum nanostructure, such as a quantum point contact (QPC). In many studies, we use dynamic nuclear polarization and…

Mesoscale and Nanoscale Physics · Physics 2022-03-09 M. H. Fauzi , T. Sobue , A. Noorhidayati , K. Sato , K. Hashimoto , Y. Hirayama

NMR is the technique of election to probe the local properties of materials. Herein we present the results of density functional theory (DFT) \textit{ab initio} calculations of the NMR parameters for fluorapatite (FAp), a calcium…

Materials Science · Physics 2012-07-27 Barbara Pavan , Davide Ceresoli , Mary M. J. Tecklenburg , Marco Fornari

Much new solid state technology for single-photon sources, detectors, photovoltaics and quantum computation relies on the fabrication of strained semiconductor nanostructures. Successful development of these devices depends strongly on…

Conventional nuclear magnetic resonance (NMR) spectroscopy relies on acquiring signal from a macroscopic ensemble of molecules to gain information about molecular structure and dynamics. Transferring this technique to nanoscale sample sizes…

Mesoscale and Nanoscale Physics · Physics 2019-02-06 Jeffrey Holzgrafe , Qiushi Gu , Jan Beitner , Dhiren Kara , Helena S. Knowles , Mete Atatüre

We present the architecture of the versatile NMR spectrometer with software-defined radio (SDR) technology and its application to the dynamically controlled pulsed magnetic fields. The pulse-field technology is the only solution to access…

Strongly Correlated Electrons · Physics 2021-11-24 Yoshihiko Ihara , Kaoru Hayashi , Tomoki Kanda , Kazuki Matsui , Koichi Kindo , Yoshimitsu Kohama

Characterizing ion adsorption and diffusion in porous carbons is essential to understand the performance of such materials in a range of key technologies such as energy storage and capacitive deionisation. Nuclear Magnetic Resonance (NMR)…

Materials Science · Physics 2023-05-08 Anagha Sasikumar , Céline Merlet

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

Nuclear Magnetic Resonance (NMR) spectroscopy is a central characterization method for molecular structure elucidation, yet interpreting NMR spectra to deduce molecular structures remains challenging due to the complexity of spectral data…

Chemical Physics · Physics 2025-07-15 Qingsong Yang , Binglan Wu , Xuwei Liu , Bo Chen , Wei Li , Gen Long , Xin Chen , Mingjun Xiao

We present a new method for high-resolution nanoscale magnetic resonance imaging (nano-MRI) that combines the high spin sensitivity of nanowire-based magnetic resonance detection with high spectral resolution nuclear magnetic resonance…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 William Rose , Holger Haas , Angela Q. Chen , Nari Jeon , Lincoln J. Lauhon , David G. Cory , Raffi Budakian

Magnetic resonance imaging at microtesla fields is a promising imaging method that combines the pre-polarization technique and broadband signal reception by SQUID sensors to enable in vivo MRI at microtesla-range magnetic fields. Despite…

Medical Physics · Physics 2010-10-18 V. S. Zotev , T. Owens , A. N. Matlashov , I. M. Savukov , J. J. Gomez , M. A. Espy

Hyperpolarized nuclear magnetic resonance and lab-on-a-chip microfluidics are two dynamic, but until recently quite distinct, fields of research. Recent developments in both areas increased their synergistic overlap. By microfluidic…

Chemical Physics · Physics 2021-09-29 James Eills , William Hale , Marcel Utz

We use dynamic nuclear polarization (DNP) enhanced nuclear magnetic resonance (NMR) at liquid helium temperatures to directly detect hydrogen attached to the surface of silicon microparticles. The proton NMR spectrum from a dry sample of…

Materials Science · Physics 2017-06-08 Mallory L. Guy , Kipp J. van Schooten , Lihuang Zhu , Chandrasekhar Ramanathan

Nuclear magnetic resonance (NMR) spectroscopy is a powerful technique to study local magnetism in a variety of materials. However, the inherently low sensitivity of conventional inductively detected solid state NMR typically requires a…

Mesoscale and Nanoscale Physics · Physics 2025-12-16 Louis Beaudoin , Aimé Verrier , Youcef A. Bioud , Mathieu Massicotte , Bertrand Reulet , Jeffrey A. Quilliam

Magnetic nanoparticles (MNPs) form the foundation of many technologies, frequently serving to purify proteins or cells from a biological sample or to remove environmental contaminants. Their success relies on their magnetic response, which…

Instrumentation and Detectors · Physics 2025-06-18 Alexis Scholtz , Jack Paulson , Victoria Nunez , Andrea M. Armani

The past 15 years have seen an astonishing increase in Nuclear Magnetic Resonance (NMR) sensitivity and accessible pressure range in high-pressure NMR experiments, owing to a series of new developments of NMR spectroscopy applied to the…

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be…