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We study the dynamics of excitonic insulators coupled to phonons. Without phonon couplings, the linear response is given by the damped amplitude oscillations of the order parameter with frequency equal to the minimum band gap. A phonon…

Strongly Correlated Electrons · Physics 2017-12-19 Yuta Murakami , Denis Golež , Martin Eckstein , Philipp Werner

We consider a two-band spinless model describing an excitonic insulator (EI) on the two-dimensional square lattice with anisotropic hopping parameters and electron-phonon (el-ph) coupling, inspired by the EI candidate Ta$_2$NiSe$_5$. We…

Strongly Correlated Electrons · Physics 2020-05-20 Yuta Murakami , Denis Golež , Tatsuya Kaneko , Akihisa Koga , Andrew J. Millis , Philipp Werner

The elementary optical excitations in two dimensional semiconductors hosting itinerant electrons are attractive and repulsive polarons -- excitons that are dynamically screened by electrons. Exciton-polarons have hitherto been studied in…

Motivated by recent interests in exploring excitonic condensate as the ground state of some narrow-bandgap semiconductors such as transition metal dichalcogenides and layered chalcogenide material Ta$_2$NiSe$_5$, in this work we…

Strongly Correlated Electrons · Physics 2023-11-09 Elahe Davari , S. Samaneh Ataei , Mehdi Kargarian

We show that the nonlinear optical response probed by two-dimensional coherent spectroscopy (2DCS) can discriminate between excitonic and lattice driven order. In the excitonic regime of a realistic model of Ta$_2$NiSe$_5$, the third order…

Strongly Correlated Electrons · Physics 2025-12-23 Jiyu Chen , Jernej Mravlje , Denis Golež , Philipp Werner

The recent observation of a transmitted Thz pulse oscillating at three times the frequency of the incident light paves the way to a new protocol to access resonant excitations in a superconductor. Here we show that this non-linear optical…

Superconductivity · Physics 2016-06-01 T. Cea , C. Castellani , L. Benfatto

We explore the collective response in an excitonic insulator phase in Ta$_2$NiSe$_5$ using a semirealistic model including relevant lattice and electronic instabilities. We calculate order-parameter susceptibility and Raman response within…

Strongly Correlated Electrons · Physics 2025-08-19 Banhi Chatterjee , Jernej Mravlje , Denis Golež

We consider nonlinear effects in scattering of light by a periodic structure supporting optical bound states in the continuum. In the spectral vicinity of the bound states the scattered electromagnetic field is resonantly enhanced…

Optics · Physics 2019-02-18 Evgeny N. Bulgakov , Dmitrii N. Maksimov

The strong-field induced generation of nonclassical states of light is not only a subject of fundamental research but also has potential usage in quantum information science and technology. The emerging field of strong-field quantum optics…

Quantum Physics · Physics 2025-03-21 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

Optical responses of atomically thin 2D materials are greatly influenced by electron-hole interactions. It is by far established that exciton signatures can be well-identified in the optical absorption spectrum of quasi-2D materials.…

Mesoscale and Nanoscale Physics · Physics 2023-10-30 Yu-Tzu Chang , Yang-Hao Chan

Excitonic insulator is a coherent electronic phase that results from the formation of a macroscopic population of bound particle-hole pairs - excitons. With only a few candidate materials known, the collective excitonic behavior is…

Strongly Correlated Electrons · Physics 2021-05-27 Pavel A. Volkov , Mai Ye , Himanshu Lohani , Irena Feldman , Amit Kanigel , Girsh Blumberg

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

Mesoscale and Nanoscale Physics · Physics 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice systems. The magnitude of the THG at the 10 percent doping increases by the factor about 10^2 from that of the neutral…

Condensed Matter · Physics 2016-08-31 Kikuo Harigaya

Nonlinear light propagation in a single-mode micron-size waveguide made of semiconducting excitonic material has been theoretically studied in terms of exciton-polaritons by using an analysis based on macroscopic fields. When a light pulse…

Materials Science · Physics 2011-05-24 Oleksii A. Smyrnov , Fabio Biancalana , Stefan Malzer

We employ time-resolved resonant x-ray diffraction to study the melting of charge order and the associated insulator-metal transition in the doped manganite Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ after resonant excitation of a high-frequency…

Strongly Correlated Electrons · Physics 2017-06-21 V. Esposito , R. Mankowsky , M. Fechner , H. Lemke , M. Chollet , J. M. Glownia , M. Nakamura , M. Kawasaki , Y. Tokura , U. Staub , P. Beaud , M. Först

We predict a non-thermal magneto-optical effect for magnetic insulators subject to intense light carrying orbital angular momentum (OAM). Using a classical approach to second harmonic generation in non-linear media with specific symmetry…

Mesoscale and Nanoscale Physics · Physics 2014-10-17 Thomas Bose , Jamal Berakdar

We theoretically investigate the nonlinear optical pulse responses of excitons in a thin film where the excitonic center-of-mass motion is confined. A large interaction volume between excitons and radiation yields particular coupled states…

Materials Science · Physics 2017-04-19 Takashi Kinoshita , Hajime Ishihara

Excitonic effects in the linear optical response of semiconductors are well-known and the subject of countless experimental and theoretical studies. For the technologically important second order nonlinear response, however, description of…

Strongly Correlated Electrons · Physics 2007-05-23 Thomas G. Pedersen , Horia D. Cornean

The amplitude and phase of a material's nonlinear optical response provide insight into the underlying electronic dynamics that determine its optical properties. Phase-sensitive nonlinear spectroscopy techniques are widely implemented to…

Mesoscale and Nanoscale Physics · Physics 2018-07-12 Galan Moody , Corey McDonald , Ari Feldman , Todd Harvey , Richard P. Mirin , Kevin L. Silverman

Optical responses in an excitonic insulating (EI) system with strong electron correlation are studied. We adopt the two-orbital Hubbard model with a finite energy difference between the two orbitals where the spin state degree of freedom…

Strongly Correlated Electrons · Physics 2020-03-25 Hengyue Li , Junya Otsuki , Makoto Naka , Sumio Ishihara
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