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Related papers: Liquid-liquid Phase transitions in silicon

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First principles molecular dynamics simulations reveal a liquid-liquid phase transition in supercooled elemental silicon. Two phases coexist below $T_c\approx 1232K$. The low density phase is nearly tetra-coordinated, with a pseudogap at…

Materials Science · Physics 2009-11-13 P. Ganesh , M. Widom

A novel liquid-liquid phase transition has been proposed and investigated in a wide variety of pure substances recently, including water, silica and silicon. From computer simulations using the Stillinger-Weber classical empirical…

Statistical Mechanics · Physics 2015-05-27 Vishwas V Vasisht , Shibu Saw , Srikanth Sastry

Carbon, the fourth most abundant element in the Universe forms a metallic fluid with transient covalent bonds on melting. Its liquid-liquid phase transitions, intensely sought using simulations had been elusive. Here we use density…

Statistical Mechanics · Physics 2022-03-02 M. W. C. Dharma-wardana , Dennis D. Klug

Recent cutting-edge experiments have provided {\it in situ} structure characterization and measurements of the pressure ($P$), density ($\bar{\rho}$) and temperature ($T$) of shock compressed silicon in the 100 GPa range of pressures and…

Materials Science · Physics 2024-12-12 M. W. C. Dharma-wardana , Dennis D. Klug , Hannah Poole , G. Gregori

The existence of a 'crossover region' in glass-forming liquids has long been considered as a general phenomenon that is as important as the glass transition. One potential origin for the crossover behavior is a liquid-to-liquid phase…

Materials Science · Physics 2015-09-14 S. Lan , M. Blodgett , K. F. Kelton , X. -L. Wang

A recent experiment [K. H. Kim, et al., Science 370, 978 (2020)] showed that it may be possible to detect a liquid-liquid phase transition (LLPT) in supercooled water by subjecting high density amorphous ice (HDA) to ultrafast heating,…

Statistical Mechanics · Physics 2021-06-24 Nicolas Giovambattista , Peter H. Poole

We present a review on the study of metastable silicon, primarily focusing mainly on the aspects of liquid-liquid transition, critical point and phase behaviour, structural and dynamic properties of liquid phase as well as crystal…

Materials Science · Physics 2021-09-01 Vishwas V. Vasisht , Srikanth Sastry

Liquid-liquid and liquid-vapor coexistence regions of various water models were determined by MC simulations of isotherms of density fluctuation restricted systems and by Gibbs ensemble MC simulations. All studied water models show multiple…

Statistical Mechanics · Physics 2009-11-11 Ivan Brovchenko , Alfons Geiger , Alla Oleinikova

We simulate high-pressure hydrogen in its liquid phase close to molecular dissociation using a machine-learned interatomic potential. The model is trained with density functional theory (DFT) forces and energies, with the…

Statistical Mechanics · Physics 2024-12-20 Mathieu Istas , Scott Jensen , Yubo Yang , Markus Holzmann , Carlo Pierleoni , David M. Ceperley

Liquid-liquid phase transition (LLPT) in supercooled water has been a long-standing controversial issue. We show simulation results of real stable first-order phase transitions between high and low density liquid (HDL and LDL)-like…

Soft Condensed Matter · Physics 2020-06-30 Saeed Pourasad , Amir Hajibabaei , Chang Woo Myung , Kwang S. Kim

The existence of a phase transition between two distinct liquid phases in single-component network-forming liquids (e.g., water, silica, silicon) has elicited considerable scientific interest. The challenge, both for experiments and…

Soft Condensed Matter · Physics 2022-05-30 Yagyik Goswami , Srikanth Sastry

We use numerical simulation to examine the possibility of a reversible liquid-liquid transition in supercooled water and related systems. In particular, for two atomistic models of water, we have computed free energies as functions of…

Statistical Mechanics · Physics 2012-05-11 David T. Limmer , David Chandler

A longstanding question in water research is the possibility that supercooled liquid water can undergo a liquid-liquid phase transition (LLT) into high- and low-density liquids. We used several complementary molecular simulation techniques…

A quantum phase transition that was recently observed in a high-mobility silicon MOSFET is analyzed in terms of a scaling theory. The most striking characteristic of the transition is a divergence of the thermopower, according to an inverse…

Strongly Correlated Electrons · Physics 2013-10-01 T. R. Kirkpatrick , D. Belitz

We present strong theoretical evidence that a Larkin-Ovchinnikov (LOFF/FFLO) pairing phase is favoured over the homogeneous superfluid and normal phases in three-dimensional unitary Fermi systems. Using a Density Functional Theory (DFT)…

Superconductivity · Physics 2009-01-19 Aurel Bulgac , Michael McNeil Forbes

For a long time, there have been huge discrepancies between different models and experiments concerning the liquid-liquid phase transition (LLPT) in dense hydrogen. In this work, we present the results of extensive calculations of the LLPT…

Computational Physics · Physics 2019-12-10 Binbin Lu , Dongdong Kang , Dan Wang , Tianyu Gao , Jiayu Dai

The striking anomalies in physical properties of supercooled water that were discovered in the 1960-70s, remain incompletely understood and so provide both a source of controversy amongst theoreticians, and a stimulus to experimentalists…

Chemical Physics · Physics 2016-05-31 Sander Woutersen , Michiel Hilbers , Zuofeng Zhao , C. Austen Angell

Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

Disordered Systems and Neural Networks · Physics 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

We studied dielectric properties of nano-sized liquid water samples confined in polymerized silicates MCM-41 characterized by the porous sizes \sim 3-10nm. We report the direct measurements of the dielectric constant by the dielectric…

Soft Condensed Matter · Physics 2015-05-27 P. O. Fedichev , L. I. Menshikov , G. S. Bordonskiy , A. O. Orlov

We present theoretical and experimental studies of superconductivity and low temperature structural phase boundaries in lithium. We mapped the structural phase diagram of 6Li and 7Li under hydrostatic conditions between 5 top 55GPa and…

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