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We study the low-frequency properties of the bulk photovoltaic effect in topological semimetals. The bulk photovoltaic effect is a nonlinear optical effect that generates DC photocurrents under uniform irradiation, allowed by…

Mesoscale and Nanoscale Physics · Physics 2021-07-12 Junyeong Ahn , Guang-Yu Guo , Naoto Nagaosa

Dirac materials have unique transport properties, partly due to the presence of surface states. A new type of Dirac materials, protected by non-symmorphic symmetries was recently proposed by Young and Kane [1]. By breaking of time reversal…

Mesoscale and Nanoscale Physics · Physics 2019-02-13 P. G. Matveeva , D. N. Aristov , D. Meidan , D. B. Gutman

The interplay between magnetism and light can create abundant optical phenomena. Here, we demonstrate the emergence of an unconventional magnetization-induced second-harmonic generation (MSHG) stemming from vector spin chirality, denoted as…

Materials Science · Physics 2025-04-08 Dezhao Wu , Yong Xu , Meng Ye , Wenhui Duan

We extend image scanning microscopy to second harmonic generation (SHG) by extracting the complex field amplitude of the second-harmonic beam. While the theory behind coherent image scanning microscopy (ISM) is known, an experimental…

Optics · Physics 2022-03-14 Dekel Raanan , Man Suk Song , William A Tisdale , Dan Oron

We present a first principles theoretical study employing nonlinear response theory to investigate the d.c. photocurrent generated by linearly polarized light in the type-II Weyl semimetal TaIrTe4. We report the low energy spectrum of…

Mesoscale and Nanoscale Physics · Physics 2023-05-30 Álvaro R. Puente-Uriona , Stepan S. Tsirkin , Ivo Souza , Julen Ibañez-Azpiroz

We report calculated substantial enhancement of the second harmonic generation (SHG) in cuprous oxide crystals resonantly hybridized with an appropriate organic material (DCM2:CA:PS 'solid-state solvent'). The quadrupole origin of the…

Materials Science · Physics 2009-11-13 Oleksiy Roslyak , Joseph L. Birman

Nonlinear frequency conversion plays a crucial role in advancing the functionality of next-generation optical systems. Portable metrology references and quantum networks will demand highly efficient second-order nonlinear devices, and the…

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

Experimental insight into the elementary processes underlying charge transfer across interfaces has blossomed with the wide-spread availability of ultra-high vacuum set-ups that allow the preparation and characterization of solid surfaces…

Chemical Physics · Physics 2024-02-27 Zhipeng Huang , Tobias Roos , Yujin Tong , R. Kramer Campen

High-harmonic spectroscopy in solids gives insight into the inner workings of solids, such as reconstructing band structures or probing the topological phase of materials. High-harmonic generation (HHG) is a highly non-linear phenomena and…

Quantum Physics · Physics 2025-12-16 Asger Weeth , Lars Bojer Madsen

We report the observation of second harmonic generation with high conversion efficiency $\sim 0.005\%$ in the terahertz regime from thin films of the topological insulator Bi$_2$Se$_3$ that exhibit the linear photogalvanic effect, measured…

Strongly Correlated Electrons · Physics 2024-06-11 Jonathan Stensberg , Xingyue Han , Zhuoliang Ni , Xiong Yao , Xiaoyu Yuan , Debarghya Mallick , Akshat Gandhi , Seongshik Oh , Liang Wu

We investigate the dependence of the photogalvanic response of a multi-Weyl semimetal on its topological charge, tilt, and chemical potential. We derive analytical expressions for the shift and injection conductivities for tilted charge-$n$…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Arpit Raj , Swati Chaudhary , Gregory A. Fiete

Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…

Materials Science · Physics 2022-05-12 Zhuoliang Ni , Nan Huang , Amanda V. Haglund , David G. Mandrus , Liang Wu

The unprecedented brilliance of X-ray free-electron lasers (XFELs) [1, 2] has enabled first studies of nonlinear interactions in the hard X-ray range. In particular, X-ray-optical mixing [3], X-ray second harmonic generation (XSHG) [4] and…

Symmetry plays a central role in conventional and topological phases of matter, making the ability to optically drive symmetry change a critical step in developing future technologies that rely on such control. Topological materials, like…

This study presents an investigation of second harmonic generation (SHG) resulting from interaction of radially polarized laser beam propagating in homogeneous, unmagnetized plasma. Lorentz force and continuity equations have been used to…

Plasma Physics · Physics 2025-09-30 Shivani Aggarwal , Saumya Singh , Dinkar Mishra , Bhupesh Kumar , Pallavi Jha

Polarized and azimuthal dependencies of optical second harmonics generation (SHG) at the surface of noncentrosymmetric semiconductor crystals have been measured on polished surfaces of ZnSe(100), using a fundamental wavelength of 1.06$\mu…

Optics · Physics 2007-05-23 Xiangyang Song , Arnold Neumann , Rein Maripuu , Kai Siegbahn

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

Inversion symmetry eliminates the second-order nonlinear responses in materials commonly used in silicon photonics with electric-dipole approximation. The lack of effective methods to induce the second-order nonlinearity in silicon photonic…

Optics · Physics 2024-05-22 Ru Wang , Yue Dai , Jinsong Cheng , Ruoyu Wang , Xiaoqin Shen

We have studied second harmonic generation (SHG) in a polar ferrimagnet GaFeO_3, employing a FeO_6 cluster model in which the Fe atom is slightly shifted from the center of the octahedron. The electric-dipole transition could take place…

Strongly Correlated Electrons · Physics 2015-05-19 Jun-ichi Igarashi , Tatsuya Nagao