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With the increasing interest in twisted bilayer graphene (tBLG) of the past years, fast, reliable, and non-destructive methods to precisely determine the twist angle are required. Raman spectroscopy potentially provides such method, given…

Materials Science · Physics 2022-07-14 Pablo Solís-Fernández , Hiroki Ago

Twisted bilayer graphene (TBLG) has emerged as an exciting new material with tunable electronic properties ranging from superconductivity to correlated insulating phases. But current methods of fabrication and identification of TBLG are…

Materials Science · Physics 2022-10-07 Tom Vincent , Kenji Kawahara , Vladimir Antonov , Hiroki Ago , Olga Kazakova

Twisted 2D layered materials have garnered a lot of attention recently as a class of 2D materials whose interlayer interactions and electronic properties are dictated by the relative rotation / twist angle between the adjacent layers. In…

Twisted bilayer graphene (tBLG) provides us with a large rotational freedom to explore new physics and novel device applications, but many of its basic properties remain unresolved. Here we report the synthesis and systematic Raman study of…

We present a comprehensive first-principles study of twisted bilayer graphene (tBLG) for a wide range of twist angles, with a focus on structural and electronic properties. By employing density functional theory (DFT) with an optimized…

Mesoscale and Nanoscale Physics · Physics 2026-05-13 Albert Zhu , Daniel Bennett , Daniel T. Larson , Mohammed M. Al Ezzi , Efstratios Manousakis , Efthimios Kaxiras

We develop a theoretical framework for probing moir\'e phonon modes using Raman spectroscopy, and illustrate it with the example of twisted bilayer graphene (TBG). These moir\'e phonons arise from interlayer sliding motion in twisted 2D…

Strongly Correlated Electrons · Physics 2025-06-24 Vitor Dantas , Héctor Ochoa , Rafael M. Fernandes , Natalia B. Perkins

Tailoring the interlayer twist angle of bilayer graphene (BLG) has a significant influence on its electronic properties, including superconductivity, topological transitions, ferromagnetic states and correlated insulating states. These…

In this study, we introduce an innovative methodology for robust twist angle identification in bilayer graphene using Raman spectroscopy, featuring the integration of generative adversarial network and convolutional neural network…

Applied Physics · Physics 2024-01-09 Dan Hu , Ting-Fung Chung , Yong P. Chen , Yaping Qi

Twisted bilayer graphene displays many fascinating properties that can be tuned by varying the relative angle (also called twist angle) between its monolayers. As a remarkable feature, both the electronic flat bands and the corresponding…

Materials Science · Physics 2022-05-06 V. Hung Nguyen , Trinh X. Hoang , J. -C. Charlier

Twisted bilayer graphene (TBG) represents a highly tunable, strongly correlated electron system owed to its unique flat electronic bands. However, understanding the single-particle band structure alone has been challenging due to complex…

The role of twist angle ($\theta_t$) in tailoring the physical properties of heterostructures is emerging as a new paradigm in two-dimensional materials. The influence of flat electronic bands near the magic angle ($\sim$1.1$^{\circ}$) on…

Mesoscale and Nanoscale Physics · Physics 2025-07-14 Darshit Solanki , Kenji Watanabe , Takashi Taniguchi , A. K. Sood , Anindya Das

Van der Waals layered materials with well-defined twist angles between the crystal lattices of individual layers have attracted increasing attention due to the emergence of unexpected material properties. As many properties critically…

Twisted bilayer graphene (tBLG) forms a quasicrystal whose structural and electronic properties depend on the angle of rotation between its layers. Here we present a scanning tunneling microscopy study of gate-tunable tBLG devices supported…

Twisted bilayer graphene (tBLG) provides a fascinating platform for engineering flat bands and inducing correlated phenomena. By designing the stacking architecture of graphene layers, twisted multilayer graphene can exhibit different…

We compare the main feature of the measured Raman scattering spectra from single layer graphene with a bilayer in which the two layers are arbitrarily misoriented. The profiles of the 2D bands are very similar having only one component,…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Philippe Poncharal , Anthony Ayari , Thierry Michel , Jean-Louis Sauvajol

In this work, we study the Raman spectra of twisted bilayer graphene samples as a function of their twist-angles ($\theta$), ranging from 0.03$^\circ$ to 3.40$^\circ$, where local $\theta$ are determined by analysis of their associated…

Focusing on the twist angle for the minimal commensurate structure, we perform nonperturbative calculations of electron dynamics in the twisted bilayer graphene (TBG) under intense laser fields. We show that the TBG exhibits enriched…

Strongly Correlated Electrons · Physics 2020-07-22 Tatsuhiko N. Ikeda

Several numerical studies have shown that the electronic properties of twisted bilayers of graphene (TBLG) and transition metal dichalcogenides (TMDs) are tunable by strain engineering of the stacking layers. In particular, the flatness of…

Mesoscale and Nanoscale Physics · Physics 2023-07-24 Marwa Mannaï , Sonia Haddad

Two new Raman modes below 100 cm^-1 are observed in twisted bilayer graphene grown by chemical vapor deposition. The two modes are observed in a small range of twisting angle at which the intensity of the G Raman peak is strongly enhanced,…

Mesoscale and Nanoscale Physics · Physics 2013-08-16 Rui He , Ting-Fung Chung , Conor Delaney , Courtney Keiser , Luis A. Jauregui , Paul M. Shand , C. C. Chancey , Yanan Wang , Jiming Bao , Yong P. Chen

If we stack up two layers of graphene while changing their respective orientation by some twisting angle, we end up with a system that has striking differences when compared to single-layer graphene. For a very specific value of this twist…

Mesoscale and Nanoscale Physics · Physics 2024-09-18 Eduardo B. Molinero , Anushree Datta , María J. Calderón , Elena Bascones , Rui E. F. Silva
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