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In order to fully exploit the potential of transition metal dichalcogenide monolayers (TMD-MLs), the well-controlled creation of atomically sharp lateral heterojunctions within these materials is highly desirable. A promising approach to…

Mesoscale and Nanoscale Physics · Physics 2017-10-11 Sven Borghardt , Jhih-Sian Tu , Florian Winkler , Jürgen Schubert , Willi Zander , Kristján Lesson , Beata E. Kardynał

Monolayers of transition metal dichalcogenides (TMDC) became one of the most studied nanostructures in the last decade. Combining two different TMDC monolayers results in a heterostructure whose properties can be individually tuned by the…

Mesoscale and Nanoscale Physics · Physics 2024-03-29 Marten Richter

Two-dimensional group-VI transition metal dichalcogenide semiconductors, such as MoS2, WSe2 and others, exhibit strong light-matter coupling and possess direct band gaps in the infrared and visible spectral regimes, making them potentially…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Thomas Mueller , Ermin Malic

The geometry and binding energy of excitons, set by electron-hole wavefunction distributions, are fundamental factors that underpin their many-body interactions and determine optoelectronic properties of semiconductors. However, in typical…

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang

Moir\'e superlattices open an unprecedented opportunity for tailoring interactions between quantum particles and their coupling to electromagnetic fields. Strong superlattice potential generates moir\'e minibands of excitons -- bound pairs…

Materials Science · Physics 2020-02-25 Yanhao Tang , Jie Gu , Song Liu , Kenji Watanabe , Takashi Taniguchi , James Hone , Kin Fai Mak , Jie Shan

Moir\'e superlattices of transition-metal dichalcogenide bilayers host strong Coulomb interactions residing in narrow electron bands, leading to correlated insulating states at fractional carrier doping densities, known as generalized…

We present theoretical results for the radiative rates and doping-dependent photoluminescence spectrum of interlayer excitonic complexes localized by donor impurities in MoSe$_2$/WSe$_2$ twisted heterobilayers, supported by quantum Monte…

Mesoscale and Nanoscale Physics · Physics 2018-06-04 Mark Danovich , David A. Ruiz-Tijerina , Ryan J. Hunt , Marcin Szyniszewski , Neil D. Drummond , Vladimir I. Fal'ko

Transition-metal dichalcogenide bilayers exhibit a rich exciton landscape including layer-hybridized excitons, i.e. excitons which are of partly intra- and interlayer nature. In this work, we study hybrid exciton-exciton interactions in…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Daniel Erkensten , Samuel Brem , Raul Perea-Causin , Joakim Hagel , Fedele Tagarelli , Edoardo Lopriore , Andras Kis , Ermin Malic

Moir\'e excitons are emergent optical excitations in 2D semiconductors with deep moir\'e superlattice potentials. While these excitations have been realized in several platforms, a system with dynamically tunable moir\'e potential to tailor…

In atomically thin transition metal dichalcogenides (TMDs), reduced dielectric screening of the Coulomb interaction leads to strongly correlated many-body states, including excitons and trions, that dominate the optical properties.…

Moir\'e superlattices serve as a playground for emerging phenomena, such as localization of band states, superconductivity, and localization of excitons. These superlattices are large and are often modeled in the zero angle limit, which…

Materials Science · Physics 2022-06-01 Christopher Linderälv , Joakim Hagel , Samuel Brem , Ermin Malic , Paul Erhart

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

Exciton-polaritons formed inside optical cavities offer a highly tunable platform for exploring novel quantum phenomena. Here, we introduce and theoretically characterize a light-matter moir\'e effect (LMME) that arises when a 2D material…

We studied the exciton properties in double layers of transition metal dichalcogenides (TMDs) with a dielectric spacer between the layers. We developed a method based on an expansion of Chebyshev polynomials to solve the Wannier equation…

Mesoscale and Nanoscale Physics · Physics 2023-08-09 Luiz G. M. Tenório , Teldo A. S. Pereira , K. Mohseni , T. Frederico , M. R. Hadizadeh , Diego R. da Costa , André J. Chaves

The quest for platforms to generate and control exotic excitonic states has greatly benefited from the advent of transition metal dichalcogenide (TMD) monolayers and their heterostructures. Among the unconventional excitonic states,…

Moir\'e superlattices in transition-metal dichalcogenide semiconductor heterobilayers enable the quantum confinement of interlayer excitons with large out-of-plane permanent electric dipoles and spin-valley control. Here, we report a novel…

Moir\'e potential acts as periodic quantum confinement for optically generated exciton, generating spatially ordered zero-dimensional quantum system. However, broad emission spectrum arising from inhomogeneity among moir\'e potential…

The giant exciton binding energy and the richness of degrees of freedom make monolayer transition metal dichalcogenide an unprecedented playground for exploring exciton physics in 2D systems. Thanks to the well energetically separated…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Bairen Zhu , Ke Xiao , Siyuan Yang , Kenji Watanabe , Takashi Taniguchi , Xiaodong Cui

Rydberg excitons, the solid-state counterparts of Rydberg atoms, have sparked considerable interest in harnessing their quantum application potentials, whereas a major challenge is realizing their spatial confinement and manipulation.…

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