Related papers: Photodissociation of long-range Rydberg molecules
Divalent atoms provide excellent means for advancing control in Rydberg atom-based quantum simulation and computing, due to the second optically active valence electron available. Particularly promising in this context are circular Rydberg…
We report on measurements of the binding energies of several weakly bound vibrational states of the paramagnetic $^{174}$Yb$^{6}$Li molecule in the electronic ground state using two-photon spectroscopy in an ultracold atomic mixture…
Photoionization of atoms immersed in an environment such as an ultracold gas is investigated. We show that the interference of two ionization pathways, one passing directly to the continuum and one accounting for scattering processes…
We predict that ultralong-range Rydberg bi-molecules form in collisions between polar molecules in cold and ultracold settings. The collision of $\Lambda$-doublet nitric oxide (NO) with long-lived Rydberg NO($nf$, $ng$) molecules forms…
We present fast Rydberg-mediated entanglement involving nuclear spins of divalent atoms with $^{171}$Yb as an example. First, we show a nuclear-spin controlled phase gate of an arbitrary phase realizable either with two laser pulses when…
Photonic molecules - particular systems composed of coupled optical resonators - emulate the behavior of complex physical systems exhibiting discrete energy levels. In this work, we present a novel photonic molecule composed of two strongly…
Arrays of highly excited Rydberg atoms can be used as powerful quantum simulation platforms. Here, we introduce an approach that makes it possible to implement fully controllable effective spin interactions in such systems. We show that…
We demonstrate a multiphoton Rydberg dark resonance where a Lambda-system is coupled to a Rydberg state. This N-type level scheme combines the ability to slow and store light pulses associated with long lived ground state superpositions,…
Coupling photons to Rydberg excitations in a cold atomic gas yields unprecedentedly large optical nonlinearities at the level of individual light quanta, where the formation of nearby dark-state polaritons is blocked by the strong…
Applicability of Rydberg atoms to quantum computers is examined from experimental point of view. In many theoretical proposals appeared recently, excitation of atoms into highly excited Rydberg states was considered as a way to achieve…
A theory of Rydberg atom interactions is used to derive analytical forms for the spin wave pair correlation function in laser-excited cold-atom vapors. This function controls the quantum statistics of light emission from dense,…
Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…
We report the generation of entanglement between two individual $^{87}$Rb atoms in hyperfine ground states $|F=1,M=1>$ and $|F=2,M=2>$ which are held in two optical tweezers separated by 4 $\mu$m. Our scheme relies on the Rydberg blockade…
A fascinating aspect of Rydberg atoms is their ability to form huge but very weakly bound molecules with a ground state atom, only held together by a scattering process between the latter and the Rydberg electron. Beyond the usual way of…
Here, we explore the combination of sub-wavelength, two-dimensional atomic arrays and Rydberg interactions as a powerful platform to realize strong, coherent interactions between individual photons with high fidelity. In particular, the…
Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between…
The long-range interaction between Rydberg-excited atoms endows a medium with large optical nonlinearity. Here, we demonstrate an optical switch to operate on a single photon from an entangled photon pair under a Rydberg electromagnetically…
Inhomogeneous electric fields generated above two-dimensional electrode structures have been used to transversely split beams of helium Rydberg atoms into pairs of spatially separated components. The atomic beams had initial longitudinal…
Recent developments in the study of ultracold Rydberg gases demand an advanced level of experimental sophistication, in which high atomic and optical densities must be combined with excellent control of external fields and sensitive Rydberg…
Over the past few years we have built an apparatus to demonstrate the entanglement of neutral Rb atoms at optically resolvable distances using the strong interactions between Rydberg atoms. Here we review the basic physics involved in this…