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Advances in light sources and time resolved spectroscopy have made it possible to excite specific atomic vibrations in solids and to observe the resulting changes in electronic properties but the mechanism by which phonon excitation causes…

Superconductivity · Physics 2017-05-05 Dante M. Kennes , Eli Y. Wilner , David R. Reichman , Andrew J. Millis

In stimulated Raman scattering, two incident optical waves induce a force oscillating at the difference of the two light frequencies. This process has enabled important applications such as the excitation and coherent control of phonons and…

Materials Science · Physics 2017-09-27 Sebastian Maehrlein , Alexander Paarmann , Martin Wolf , Tobias Kampfrath

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

Photo-induced phase transitions have been intensively studied owing to the ability to control a material of interest in the ultrafast manner, which can induce exotic phases unable to be attained at equilibrium. However, the key mechanisms…

We demonstrate dynamic control of the lattice by THz light by exploiting the coupling of phonon modes. The low-energy sliding phonon modes in the spin-ladder system, Sr$_{14}$Cu$_{24}$O$_{41}$, are excited using THz radiation with high…

Strongly Correlated Electrons · Physics 2023-11-10 S. J. Sreerag , N. Malathi , Shahla Yasmin Mathengattil , Rabindranath Bag , Surjeet Singh , Rajeev N. Kini

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high frequency vibrational mode is driven resonantly by…

The interaction of a single-cycle THz electric field with the topological insulator $\mathrm{MnBi}_2\mathrm{Te}_4$ triggers strongly anharmonic lattice dynamics, promoting fully coherent energy transfer between the otherwise non-interacting…

Coherent phonons describe the collective, ultrafast motion of atoms and play a central role in light-induced structural dynamics. Here, we employ terahertz scanning tunneling microscopy (THz-STM) to excite and detect coherent phonons in…

Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…

Strongly Correlated Electrons · Physics 2016-08-22 Daniele Nicoletti , Andrea Cavalleri

Phononic engineering at gigahertz (GHz) frequencies form the foundation of microwave acoustic filters, acousto-optic modulators, and quantum transducers. Terahertz (THz) phononic engineering could lead to acoustic filters and modulators at…

Femtosecond core-level transient absorption spectroscopy is utilized to investigate photoinduced dynamics of the charge density wave in 1T-TiSe2 at the Ti M2,3 edge (30-50 eV). Photoexcited carriers and phonons are found to primarily induce…

Materials Science · Physics 2022-11-08 Tobias Heinrich , Hung-Tzu Chang , Sergey Zayko , Kai Rossnagel , Murat Sivis , Claus Ropers

The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of…

We propose an experimental technique to generate large amplitude coherent phonons with irradiation of THz-rate pump pulses and to study the dynamics of phase transition in GeTe ferroelectrics. When a single pump pulse irradiates the sample…

Materials Science · Physics 2011-02-01 Muneaki Hase , Masahiro Kitajima , Shin-ichi Nakashima , Kohji Mizoguchi

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

Materials Science · Physics 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

The coherent modulation of electronic and vibrational nonlinearities in atoms and molecular gases by intense few-cycle pulses has been used for high-harmonic generation in the soft X-ray and attosecond regime, as well as for Raman frequency…

Materials Science · Physics 2013-09-16 Muneaki Hase , Masayuki Katsuragawa , Anca Monia Constantinescu , Hrvoje Petek

We investigate the out-of-equilibrium lattice dynamics in the spin-ladder system $\alpha'$-NaV$_2$O$_5$ using intense terahertz (THz) pump and near-infrared (NIR) probe spectroscopy. When quasi-single-cycle THz pulses interact with…

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , J. Bowlan , S. A. Trugman , R. Valdes Aguilar , J. Qi , X. Liu , J. Furdyna , M. Dobrowolska , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

The aim of this work is to describe the behavior of a device capable to generate high frequency (~THz) acoustic phonons. This device consists in a GaAs-AlGaAs double barrier heterostructure that, when an external bias is applied, produces a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 I. Camps , S. S. Makler , H. M. Pastawski , L. E. F. Foa Torres

Ultrashort light pulses can selectively excite charges, spins and phonons in materials, providing a powerful approach for manipulating their properties. Here we use femtosecond laser pulses to coherently manipulate the electron and phonon…

Driving coherent lattice motion with THz pulses has emerged as a novel pathway for achieving dynamic stabilization of exotic phases that are inaccessible in equilibrium quantum materials. In this work, we present a previously unexplored…

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