Related papers: Large molasses-like cooling forces for molecules u…
We study a single incoherently pumped atom moving within an optical high-Q resonator in the strong coupling regime. Using a semiclassical description for the atom and field dynamics, we derive a closed system of differential equations to…
We demonstrate laser cooling of barium monofluoride (138BaF) molecules. We use serrodynes to synthesize time-sequenced optical spectra that can be precisely tailored to the hyperfine structure of this heaviest non-radioactive alkaline earth…
We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…
We suggest a protocol for the sympathetic cooling of a molecular asymmetric top rotor co-trapped with laser-cooled atomic ions, based on resonant coupling between the molecular ion's electric dipole moment and a common normal mode of the…
Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…
Molecular predissociation is the spontaneous, nonradiative bond breaking process that can occur upon excitation. In the context of laser cooling, predissociation is an unwanted consequence of molecular structure that limits the ability to…
We propose to repeatedly load laser-cooled molecules into optical tweezers, and transfer them to storage states that are rotationally excited by two additional quanta. Collisional loss of molecules in these storage states is suppressed, and…
We present a novel approach to precisely synthesize arbitrary polarization states of light with a high modulation bandwidth. Our approach consists of superimposing two laser light fields with the same wavelength, but with opposite circular…
An important effort is currently underway to extend optical cycling and laser cooling to more molecular species. Significant challenges arise in particular when multiple nuclear spins give rise to complex, resolved hyperfine spectra, as is…
We study laser cooling of atomic gases by collisional redistribution of fluorescence. In a high pressure buffer gas regime, frequent collisions perturb the energy levels of alkali atoms, which allows for the absorption of a far red detuned…
Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…
Recently, the spectral manipulation of single photons has been achieved through spatial-temporal modulation of the optical refractive index. Here, we generalize this mechanism to massive particles, i.e. realizing the acceleration or…
Some of us have recently reported in Science 321 232 (2008) vibrational cooling of translationally cold Cs_2 molecules into the lowest vibrational level v=0 of the singlet X 1Sigma_g ground electronic state. Starting from a sample of cold…
Laser cooling of large, complex molecules is a long-standing goal, instrumental for enabling new quantum technology and precision measurements. A primary consideration for the feasibility of laser cooling, which determines the efficiency…
We demonstrate sub-Doppler cooling of 40K on the D_1 atomic transition. Using a gray molasses scheme, we efficiently cool a compressed cloud of 6.5x10^8 atoms from ~ 4\mK to 20uK in 8 ms. After transfer in a quadrupole magnetic trap, we…
A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…
Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…
The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…
We report optical trapping of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH molecules from a magneto-optical trap are sub-Doppler laser cooled to $20(3)~\mu\text{K}$ in free space and loaded into an optical dipole trap. We…
We analyzed bichromatic and polychromatic stimulated forces for laser cooling and trapping of Yb atoms using only the narrow $^1S_0\rightarrow^3P_1$ transition. Our model is based on numerical solutions of optical Bloch equations for…