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We show that the nonlinear optical response probed by two-dimensional coherent spectroscopy (2DCS) can discriminate between excitonic and lattice driven order. In the excitonic regime of a realistic model of Ta$_2$NiSe$_5$, the third order…

Strongly Correlated Electrons · Physics 2025-12-23 Jiyu Chen , Jernej Mravlje , Denis Golež , Philipp Werner

Transient responses of the electronic excitation and coherent soft phonon are investigated both above and below the ferroelectric phase transition temperature T$_{c}$ in Pb$_{1-x}$Ge$_{x}$Te by using an optical pump-probe technique. The…

Materials Science · Physics 2007-05-23 Rong Lu , Muneaki Hase , Masahiro Kitajima , Shinichi Nakashima , Shunji Sugai

Understanding the mechanism of structural phase transitions in rare-earth elements is a fundamental challenge in condensed matter physics, with significant implications for materials science applications. In this study, we present a…

The quasi-skutterudite superconductors $A_3T_4$Sn$_{13}$ ($A$=Sr, Ca; $T$=Ir, Rh, Co) are highly tunable featuring a structural quantum critical point. We construct a temperature-lattice constant phase diagram for these isovalent compounds,…

Excitonic insulators are electronically-driven phases of matter characterized by the spontaneous condensation of electron-hole pairs. Here we show that La$_3$Cd$_2$As$_6$ undergoes a transition at $T_{0}=278$ K to a highly insulating state…

The role of the crystal lattice for the electronic properties of cuprates and other high-temperature superconductors remains controversial despite decades of theoretical and experimental efforts. While the paradigm of strong electronic…

Time reversal symmetric topological insulators are generically robust with respect to weak local interaction, unless symmetry breaking transitions take place. Using dynamical mean-field theory we solve an interacting model of quantum spin…

Strongly Correlated Electrons · Physics 2025-08-19 A. Amaricci , G. Mazza , M. Capone , M. Fabrizio

Inelastic light scattering studies on single crystal of electron-doped Ca(Fe0.95Co0.05)2As2 superconductor, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at TSM ~ 140 K and superconducting…

Exciton-polaritons are light-matter hybrid quasi-particles that have emerged as a flexible platform for developing quantum technologies and engineering material properties. However, the fundamental mechanistic principles that govern their…

Soft phonons and diffuse scattering in insulating La$_{2-x}$Sr$_{x}$CuO$_4$ ($x=0.05$) have been studied by the neutron scattering technique. The X-point phonon softens from high temperature towards the structural transition temperature…

Superconductivity · Physics 2009-11-10 Shuichi Wakimoto , Seunghun Lee , Peter M. Gehring , Robert J. Birgeneau , Gen Shirane

The tunability of the interlayer coupling by twisting one layer with respect to another layer of two-dimensional materials provides a unique way to manipulate the phonons and related properties. We refer to this engineering of phononic…

Materials Science · Physics 2020-03-25 Indrajit Maity , Mit H. Naik , Prabal K Maiti , H. R. Krishnamurthy , Manish Jain

Using a microscopic model of lattice vibrations in the STO(001) substrate, an additional 50 mev longitudinal optical (LO) interface mode is identified. The soft mode propagating mainly in the first TiO2 layer ("O chains") has stronger…

Superconductivity · Physics 2019-08-28 Baruch Rosenstein , B. Ya. Shapiro

We have used a combination of ultrafast coherent phonon spectroscopy, ultrafast thermometry, and time-dependent Landau theory to study the inversion symmetry breaking phase transition at $T_c = 200$ K in the strongly spin-orbit coupled…

Strongly Correlated Electrons · Physics 2018-01-26 J. W. Harter , D. M. Kennes , H. Chu , A. de la Torre , Z. Y. Zhao , J. -Q. Yan , D. G. Mandrus , A. J. Millis , D. Hsieh

We study the zero-temperature phase diagram and fractional excitation when a thin film of 3D topological insulator has two competing masses: T- symmetric exciton condensation and T- breaking Zeeman effect. Two topologically distinct phases…

Strongly Correlated Electrons · Physics 2013-05-29 Gil Young Cho , Joel E. Moore

Optical control of structure-driven magnetic order offers a platform for magneto-optical terahertz devices. We control the magnetic phases of $d^1$ Mott insulating titanates using nonlinear phononics to transiently perturb the atomic…

Materials Science · Physics 2018-07-18 Mingqiang Gu , James M. Rondinelli

Using light to manipulate materials into desired states is one of the goals in condensed matter physics, since light control can provide ultrafast and environmentally-friendly photonics devices. However, it is generally difficult to realise…

We present a new high-resolution angle-resolved photoemission study of 1\textit{T}-TiSe$_{2}$ in both, its room-temperature, normal phase and its low-temperature, charge-density wave phase. At low temperature the photoemission spectra are…

Strongly Correlated Electrons · Physics 2009-11-13 H. Cercellier , C. Monney , F. Clerc , C. Battaglia , L. Despont , M. G. Garnier , H. Beck , L. Patthey , H. Berger , P. Aebi

Using a variational approach, the binding energies $E_b$ of the lowest bound excitons in Xenes under varying electric field are investigated. The internal exciton motion is described both by Dirac electron dispersion and in effective-mass…

Materials Science · Physics 2023-07-12 Olivia Pulci , Paola Gori , Davide Grassano , Marco D'Alessandro , Friedhelm Bechstedt

We use inelastic light scattering to study Sr$_{1-x}$Na$_x$Fe$_2$As$_2$ ($x\approx0.34$), which exhibits a robust tetragonal magnetic phase that restores the four-fold rotation symmetry inside the orthorhombic magnetic phase. With cooling,…

Superconductivity · Physics 2017-11-22 Li Yue , Xiao Ren , Tingting Han , Jianqing Guo , Zhicheng Wu , Yan Zhang , Yuan Li

An excitonic insulator (EI) phase is a consequence of collective many-body effects where an optical band gap is formed by the condensation of electron-hole pairs or excitons. We report pressure-dependent optical pump optical probe…

Materials Science · Physics 2024-11-28 Vikas Arora , Victor S Muthu , Arijit Sinha , Luminita Harnagea , U V Waghmare , A K Sood
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