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Disordered systems like liquids, gels, glasses, or granular materials are not only ubiquitous in daily life and in industrial applications but they are also crucial for the mechanical stability of cells or the transport of chemical and…

Disordered Systems and Neural Networks · Physics 2019-04-30 Zhen Zhang , Walter Kob

The conventional wisdom is that liquids are completely disordered and lack non-trivial structure beyond nearest-neighbor distances. Recent observations have upended this view and demonstrated that the microstructure in liquids is…

Soft Condensed Matter · Physics 2023-02-13 Navneet Singh , Zhen Zhang , A. K. Sood , Walter Kob , Rajesh Ganapathy

An efficient description of the structures of liquids and, in particular, the structural changes that happen with liquids on supercooling remains to be a challenge. The systems composed of soft particles are especially interesting in this…

Soft Condensed Matter · Physics 2020-09-09 V. A. Levashov , R. E. Ryltsev , N. M. Chtchelkatchev

The paper continues a series of publications devoted to the 3D nonlinear localized coherent structures on the surface of vertically falling liquid films. The work is primarily focussed on experimental investigations. We study: (i)…

Fluid Dynamics · Physics 2015-05-18 E. A. Demekhin , E. N. Kalaidin , A. S. Selin

We propose the new method of fluid structure investigation which is based on numerical analytical continuation of structural correlation functions with Pade approximants. The method particularly allows extracting hidden structural features…

Materials Science · Physics 2016-06-29 N. M. Chtchelkatchev , B. A. Klumov , R. E. Ryltsev , R. M. Khusnutdinoff , A. V. Mokshin

In this paper the amorphous/solid to disorder liquid structural phase transitions of an anomalous confined fluid is analyzed using their local fractal dimension. The model is a system of particles interacting through a two length scales…

Soft Condensed Matter · Physics 2016-02-17 Elsa M. de la Calleja-Mora , Leandro B. Krott , Marcia C. Barbosa

Silica is the paradigmatic network glass-former and understanding its response to pressure is essential for comprehending the mechanical properties of silica-based materials and the behavior of silicate melts in the Earth's interior. While…

Disordered Systems and Neural Networks · Physics 2025-10-16 Zhen Zhang , Zhencheng Xie , Walter Kob

There are at least three fundamental states of matter, depending upon temperature and pressure: gas, liquid, and solid (crystal). These states are separated by first-order phase transitions between them. In both gas and liquid phases the…

Soft Condensed Matter · Physics 2013-07-03 Hajime Tanaka

Whereas knowledge of a crystalline material's unit cell is fundamental to understanding the material's properties and behavior, there are not obvious analogues to unit cells for disordered materials despite the frequent existence of…

Computational Geometry · Computer Science 2020-05-27 Benjamin Schweinhart , David Rodney , Jeremy Mason

A line of hard spheres confined by a transverse harmonic potential, with hard walls at its ends, exhibits a variety of buckled structures as it is compressed longitudinally. Here we show that these may be conveniently observed in a rotating…

Soft Condensed Matter · Physics 2019-09-24 Jens Winkelmann , Adil Mughal , Denis Weaire , Stefan Hutzler

We use the isoconfigurational (IC) ensemble to show the connection between emerging heterogeneities in the tetrahedral order parameter and the dynamic propensity in a mildly undercooled glass-forming liquid. We observe that spatially…

Soft Condensed Matter · Physics 2021-01-18 M Shajahan G Razul , Gurpreet S Matharoo , Balakrishnan Viswanathan

We report the structure of transient fluctuations in the liquid phase of a two-dimensional system that exhibits several ordered phases with different symmetries. The density-temperature phase diagram of the system studied, composed of…

Soft Condensed Matter · Physics 2018-07-04 Ari B. Roitman , Linsey M. Nowack , Chris Liepold , Binhua Lin , Stuart A. Rice

For almost a century, since Bernal\'s attempts at a molecular theory of liquid structure(Bernal [1]), correlation functions have been the bridge to compare theoretical calculations with experimental measurements in the study of disordered…

Structural organization and correlations are studied in very large packings of equally sized acrylic spheres, reconstructed in three-dimensions by means of X-ray computed tomography. A novel technique, devised to analyze correlations among…

Soft Condensed Matter · Physics 2007-09-19 Tomaso Aste

Using computed x-ray tomography we determine the three dimensional (3d) structure of binary hard sphere mixtures as a function of composition and size ratio of the particles, q. Using a recently introduced four-point correlation function we…

Soft Condensed Matter · Physics 2023-02-15 Houfei Yuan , Zhen Zhang , Walter Kob , Yujie Wang

We use a series of molecular dynamics simulations, and analytical theory, to demonstrate that a system of hard spheres confined to a narrow cylindrical channel exhibits a continuous phase transition from an isotropic fluid at low densities,…

Soft Condensed Matter · Physics 2014-09-18 Mahdi Zaeifi Yamchi , Richard K. Bowles

Specially synthesized silica colloidal spheres with fluorescent cores were used as model electrorheological fluids to experimentally explore structure formation and evolution under conditions of no shear. Using Confocal Scanning Laser…

Soft Condensed Matter · Physics 2009-10-31 U. Dassanayake , S. Fraden , A. van Blaaderen

We study numerically the crystallization of a hard-sphere mixture with 8\% polydispersity. Although often used as a model glass former, for small system sizes we observe crystallization in molecular dynamics simulations. This opens the…

Soft Condensed Matter · Physics 2016-09-05 Matteo Campo , Thomas Speck

Exploring structural order in disordered systems including liquids and glasses is an intriguing but challenging issue in condensed matter physics. Here we construct a new parameter based on the angular distribution function of particles and…

Soft Condensed Matter · Physics 2018-06-11 Xiunan Yang , Wei-Hua Wang , Ke Chen

Liquids and solids are two fundamental states of matter. However, due to the lack of direct experimental determination, our understanding of the 3D atomic structure of liquids and amorphous solids remained speculative. Here we advance…

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