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Context. The spatial distribution of molecules around starless cores is a powerful tool for studying the physics and chemistry governing the earliest stages of star formation. Aims. Our aim is to study the chemical differentiation in…

Astrophysics of Galaxies · Physics 2020-11-04 S. Spezzano , P. Caselli , J. E. Pineda , L. Bizzocchi , D. Prudenzano , Z. Nagy

Recently, the extremely sensitive torsion-rotation transitions in methanol have been used to set a tight constraint on a possible variation of the proton-to-electron mass ratio over cosmological time scales. In order to improve this…

Hydrogen sulfide (H$_2$S) is thought to be efficiently formed on grain surfaces through the successive hydrogenation of S atoms. Its non-detection so far in astronomical observations of icy dust mantles thus indicates that effective…

Astrophysics of Galaxies · Physics 2023-08-17 Julia C. Santos , Harold Linnartz , Ko-Ju Chuang

Physical conditions in dense and cold regions of interstellar clouds favour the formation of ice mantles on the surfaces of interstellar grains. It is predicted that most of the gaseous species heavier than H2 or He will adsorb onto the…

Astrophysics of Galaxies · Physics 2015-06-12 Oscar Morata , Tatsuhiko I. Hasegawa

We have investigated the hydrogen-bonded structures in liquid methanol and a 7:3 mole fraction aqueous solution using classical Molecular Dynamics simulations at 298K and ambient pressure. We find that, in contrast to recent predictions…

Soft Condensed Matter · Physics 2009-11-10 Susan K. Allison , Joseph P. Fox , Rowan Hargreaves , Simon P. Bates

Ethanol (CH3CH2OH) has been detected in interstellar ices within regions associated with the early stages of star and planet formation. Its solid-phase pathways can lead to diverse conditions that can significantly influence its…

Astrophysics of Galaxies · Physics 2026-04-08 J. A. DeVine , J. Terwisscha van Scheltinga , S. Ioppolo , K. -J. Chuang , E. F. van Dishoeck , T. Lamberts

Grain surface chemistry and its treatment in gas-grain chemical models is an area of large uncertainty. Whilst laboratory experiments are making progress, there is still much that is unknown about grain surface chemistry. Further, the…

Astrophysics of Galaxies · Physics 2018-12-04 Jonathan Holdship , Niall Jeffrey , Antonios Makrymallis , Serena Viti , Jeremy Yates

The expression of chirality in adsorption phenomena constitutes an important topic, not only relevant to asymmetric transformations involving solid surfaces, but also to the emergence of homochirality in both terrestrial and…

We report the first detection of triply-deuterated methanol, with 12 observed transitions, towards the low-mass protostar IRAS 16293-2422, as well as multifrequency observations of 13CH3OH, used to derive the column density of the main…

Astrophysics · Physics 2007-05-23 B. Parise , A. Castets , E. Herbst , E. Caux , C. Ceccarelli , I. Mukhopadhyay , A. G. G. M. Tielens

Context. In dense clouds, hydrogenation reactions on icy dust grains are key in the formation of molecules, like formaldehyde, methanol, and complex organic molecules (COMs). These species form through the sequential hydrogenation of CO…

Solar and Stellar Astrophysics · Physics 2018-09-28 K. -J. Chuang , G. Fedoseev , D. Qasim , S. Ioppolo , E. F. van Dishoeck , H. Linnartz

A magnetohydrodynamic model of a steady, transverse C-type shock in a dense molecular cloud is presented. A complete gas-grain chemical network is taken into account: the gas-phase chemistry, the adsorption of gas species on dust grains,…

Astrophysics of Galaxies · Physics 2018-06-12 A. V. Nesterenok

The association reaction S + CO {\to} OCS + hnu has been identified as being particularly important for the prediction of gas-phase OCS abundances by chemical models of dark clouds. We performed detailed ab-initio calculations for this…

Astrophysics of Galaxies · Physics 2015-06-03 Jean-Christophe Loison , Philippe Halvick , Astrid Bergeat , Kevin M. Hickson , Valentine Wakelam

Three structural isomers of the C2H4O2 molecule, namely, methyl formate (MF; HCOOCH3), acetic acid (AA; CH3COOH), and glycol aldehyde (GA; HOCH2CHO), have attracted considerable attention as targets for understanding pathways towards…

Astrophysics of Galaxies · Physics 2021-11-17 A. Ishibashi , H. Hidaka , Y. Oba , A. Kouchi , N. Watanabe

The methanol molecule CH3OH has a complex microwave spectrum with a large number of very strong lines. This spectrum includes purely rotational transitions as well as transitions with contributions of the internal degree of freedom…

Cosmology and Nongalactic Astrophysics · Physics 2013-06-12 S. A. Levshakov , M. G. Kozlov , D. Reimers

Hydroxylamine (NH2OH) is one of the potential precursors of complex pre-biotic species in space. Here we present a detailed experimental study of hydroxylamine formation through nitric oxide (NO) surface hydrogenation for astronomically…

Astrophysics of Galaxies · Physics 2017-05-26 Gleb Fedoseev , Sergio Ioppolo , Thanja Lamberts , Junfeng Zhen , Herma M. Cuppen , Harold Linnartz

Methanol (CH$_{3}$OH) is a key complex organic molecule (COM) in the interstellar medium, widely used as a tracer of dense gas and hot molecular cores (HMCs). Using high-resolution ALMA observations from the ATOMS survey, we investigate the…

Methanol lines observations of a sample of low mass Class 0 protostars are presented. Using a 1D radiative transfer model, I show that several protostars have large abundance jumps in the inner hot and dense region of envelopes, probably…

Astrophysics · Physics 2007-05-23 S. Maret

At low concentrations of methanol in ethanol-methanol binary system, the molecular interactions are seen to be uniquely complex. It is observed that the ethanol aggregates are not strictly hydrogen-bonded complexes; dispersion forces also…

Chemical Physics · Physics 2016-11-21 K Nilavarasi , Thejus R Kartha , V Madhurima

Complex organic molecules are only detected toward a fraction of high-mass protostars. The goal of this work is to investigate whether high-mass disks can explain the lack of methanol emission from some massive protostellar systems. We…

Astrophysics of Galaxies · Physics 2023-03-15 P. Nazari , B. Tabone , G. P. Rosotti

The formation and decomposition of methane hydrates, particularly in porous media such as subsea sediments, have attracted significant research interest due to their implications for energy production, storage, and safety in deep-sea…

Applied Physics · Physics 2024-10-01 Yuze Wang , Jianyu Yang , Pengfei Wang , Jinlong Zhu , Yongshun John Chen
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