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We present a simple and efficient approximation to the electron-phonon scattering rate suitable for high-throughput screening of candidate materials for thermoelectric devices, based on electronic transport. The method is applied to…

Materials Science · Physics 2015-11-30 Georgy Samsonidze , Boris Kozinsky

We present a method to compute the intrinsic spin Hall conductivity from first principles using an interpolation scheme based on maximally-localized Wannier functions. After obtaining the relevant matrix elements among the ab initio Bloch…

Mesoscale and Nanoscale Physics · Physics 2019-06-18 Ji Hoon Ryoo , Cheol-Hwan Park , Ivo Souza

We present a comprehensive ab initio study of the influence of band structure corrections, particularly the electron effective mass, on the phonon-limited electron drift and Hall mobilities of GaAs. Our approach is based on the DFT+$U$…

The coupling between the intramolecular vibrational modes and the doped conduction electrons in $M_3C_{60}$ is studied by a calculation of the electronic contributions to the phonon self energies. The calculations are carried out for an…

Condensed Matter · Physics 2009-10-22 M. S. Deshpande , E. J. Mele , M. J. Rice , H-Y Choi

Charge transport plays a crucial role in manifold potential applications of two-dimensional materials, including field effect transistors, solar cells, and transparent conductors. At most operating temperatures, charge transport is hindered…

Materials Science · Physics 2023-05-03 Samuel Poncé , Miquel Royo , Massimiliano Stengel , Nicola Marzari , Marco Gibertini

The possibility of superconducting pairing of electrons in doped graphene due to in-plane and out-of-plane phonons is studied. Quadratic coupling of electrons with out-of-plane phonons is considered in details, taking into account both…

Mesoscale and Nanoscale Physics · Physics 2010-05-27 Yu. E. Lozovik , A. A. Sokolik

The phonon-assisted interband optical absorption spectrum of silicon is calculated at the quasiparticle level entirely from first principles. We make use of the Wannier interpolation formalism to determine the quasiparticle energies, as…

By means of the first-principles density-functional theory calculation and Wannier interpolation, electron-phonon coupling and superconductivity are systematically explored for boron-doped LiBC (i.e. LiB$_{1+x}$C$_{1-x}$), with $x$ between…

Superconductivity · Physics 2018-06-29 Qi-Zhi Li , Xun-Wang Yan , Miao Gao , Jun Wang

We describe an approach for calculations of phonon contributions to the electron spectral function, including both quasiparticle properties and satellites. The method is based on a cumulant expansion for the retarded one-electron Green's…

Materials Science · Physics 2015-06-22 S. M. Story , J. J. Kas , F. D. Vila , M. J. Verstraete , J. J. Rehr

We propose a fully $ \textit{ab initio} $ approach to predicting thermal attenuation in elastic helium atom scattering amplitudes, validated through strong agreement with experiments on Nb(100) and (3$\times$1)-O/Nb(100) surfaces. Our…

Materials Science · Physics 2024-12-17 Cristóbal Méndez , C. J. Thompson , M. F. Van Duinen , S. J. Sibener , Tomás A. Arias

We have performed a comprehensive computational study of the vibrational properties and electron-phonon couplings in the three known polymorphs of pentacene. Vibrational patterns and electron-phonon interactions were calculated at several…

Materials Science · Physics 2025-07-08 Luca Gnoli , Elisabetta Venuti , Matteo Masino , Patrizio Graziosi

Light-mass bipolarons in off-diagonally coupled electron-phonon systems provide a potential route to bipolaronic high-Tc superconductivity. While there has been numerical progress in the physically relevant limit of slow phonons, more…

Superconductivity · Physics 2023-08-28 Martin Grundner , Tizian Blatz , John Sous , Ulrich Schollwöck , Sebastian Paeckel

We investigate the interplay of the electron-phonon and the spin fluctuation interaction for the superconducting state of YBa$_2$Cu$_3$O$_{7}$. The spin fluctuations are described within the nearly antiferromagnetic Fermi liquid theory,…

Superconductivity · Physics 2009-10-31 T. S. Nunner , J. Schmalian , K. H. Bennemann

We report first principles analysis of electron-phonon coupling in molecular devices under external bias voltage and during current flow. Our theory and computational framework are based carrying out density functional theory within the…

Materials Science · Physics 2009-11-11 N. Sergueev , D. Roubtsov , Hong Guo

The Bethe-Salpeter formalism represents the most accurate method available nowadays for computing neutral excitation energies and optical spectra of crystalline systems from first principles. Bethe-Salpeter calculations yield very good…

Materials Science · Physics 2016-05-04 Yannick Gillet , Matteo Giantomassi , Xavier Gonze

We combine the fully anisotropic Migdal-Eliashberg theory with electron-phonon interpolation based on maximally-localized Wannier functions, in order to perform reliable and highly accurate calculations of the anisotropic…

Superconductivity · Physics 2015-06-12 E. R. Margine , F. Giustino

When the electron-phonon coupling is quadratic in the phonon coordinates, electrons can pair to form bipolarons due to phonon zero-point fluctuations, a purely quantum effect. We study superconductivity originating from this pairing…

Superconductivity · Physics 2024-09-18 Zhaoyu Han , Steven A. Kivelson , Pavel A. Volkov

We study (inverse) photoemission from systems with strong coupling of doped carriers to phonons. Using an adiabatic approximation, we develop a method for calculating spectra. This method is particularly simple for systems where the…

Strongly Correlated Electrons · Physics 2007-05-23 O. Rösch , O. Gunnarsson

We develop a method for calculating the electron-phonon vertex in polar semiconductors and insulators from first principles. The present formalism generalizes the Fr\"ohlich vertex to the case of anisotropic materials and multiple phonon…

Materials Science · Physics 2015-10-22 Carla Verdi , Feliciano Giustino

We develop a first-principles scheme to calculate adiabatic and non-adiabatic phonon frequencies in the full Brillouin zone. The method relies on the variational properties of a force-constants functional with respect to the first-order…

Materials Science · Physics 2015-05-19 Matteo Calandra , Gianni Profeta , Francesco Mauri