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Quantum tunneling of the magnetization is a major obstacle to the use of single-molecule magnets (SMMs) as basic constituents of next-generation storage devices. In this context, phonons are often only considered (perturbatively) as…

Strongly Correlated Electrons · Physics 2020-08-12 K. Irländer , J. Schnack

Tunneling between the two lowest energy levels of single molecule magnets with Ising type anisotropy, accompanied by the emission or absorption of phonons, is considered. Quantitatively accurate calculations of the rates for such tunneling…

Mesoscale and Nanoscale Physics · Physics 2015-10-05 Yun Liu , Anupam Garg

This chapter takes a microscopic view of quantum tunneling of magnetization (QTM) in single-molecule magnets (SMMs), focusing on the interplay between exchange and anisotropy. Careful consideration is given to the relationship between…

Mesoscale and Nanoscale Physics · Physics 2013-03-04 Junjie Liu , Enrique del Barco , Stephen Hill

We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…

Strongly Correlated Electrons · Physics 2009-11-11 C. Romeike , M. R. Wegewijs , H. Schoeller

Magnetothermal transport in various frustrated magnets exhibits striking field-dependent anomalies that deviate from conventional magnon or phonon transport. To understand such anomalies, we derive an effective spin-phonon Hamiltonian in…

Strongly Correlated Electrons · Physics 2026-04-14 Haoting Xu , Antoine Matar , Hae-Young Kee

Within a wide class of ferromagnetic and antiferromagnetic systems, quantum tunneling of magnetization direction is spin-parity dependent: it vanishes for magnetic particles with half-integer spin, but is allowed for integer spin. A…

Condensed Matter · Physics 2009-01-23 Daniel Loss , David P. DiVincenzo , G. Grinstein

Indirect long range interactions between localized magnetic moments are in metals mediated by itinerant electrons. In insulators and semi-conductor, such interactions need to be small, if not negligible, due to the absence of mediating…

Other Condensed Matter · Physics 2026-04-17 J. Fransson

We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…

Condensed Matter · Physics 2007-05-23 Igor Tupitsyn , Bernard Barbara

Highly symmetric magnetic environments have been suggested to stabilize the magnetic information stored in magnetic adatoms on a surface. Utilized as memory devices such systems are subjected to electron tunneling and external magnetic…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Christoph Hübner , Benjamin Baxevanis , Alexander Ako Khajetoorians , Daniela Pfannkuche

Magnetic order typically emerges due to the short-range exchange interaction between the constituent electronic spins. Recent discoveries have found a crucial role for spin-phonon coupling in various phenomena from optical ultrafast…

Mesoscale and Nanoscale Physics · Physics 2024-05-16 Petros Andreas Pantazopoulos , Johannes Feist , Francisco J. García-Vidal , Akashdeep Kamra

Multifunctional properties in quantum systems require the interaction between different degrees of freedom. As such, spin-phonon coupling emerges as an ideal mechanism to tune multiferroicity, magnetism, and magnetoelectric response. In…

The magnon-phonon coupling has received growing attention in recent years due to its central role in spin caloritronics and the emerging field of acoustic spintronics. At resonance, this magnetoelastic interaction drives the formation of…

Mathematical Physics · Physics 2021-11-02 Tor Jonas Sjöstrand , Ferdi Aryasetiawan

We derive a semiclassical quantization for a spin, study it for not too small a spin quantum number (S>5), and compute the 2S+1 eigenvalues of a Hamiltonian exhibiting resonant tunnelling as the magnetic field parallel to the anisotropy…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. L. van Hemmen , A. Suto

The prospect of developing magnetic qubits is discussed. The first part of the article makes suggestions on how to achieve the coherent quantum superposition of spin states in small ferromagnetic clusters, weakly uncompensated…

Statistical Mechanics · Physics 2007-05-23 Eugene M. Chudnovsky

Magnetophononics, the modulation of magnetic interactions by driving infrared-active lattice excitations, is emerging as a key mechanism for the ultrafast dynamical control of both semiclassical and quantum spin systems by coherent light.…

Strongly Correlated Electrons · Physics 2023-05-15 M. Yarmohammadi , M. Krebs , G. S. Uhrig , B. Normand

Anisotropic open shell 4f ions have magnetic moments that can be read and written as atomic bits. If it comes to qbits where the phase of the wave function has to be written, controlled and read, it is of advantage to rely on more than one…

Quantum Physics · Physics 2024-03-14 Thomas Greber

We study the effects of phonons on the tunneling of an atom between two surfaces. In contrast to an atom tunneling in the bulk, the phonons couple very strongly, and qualitatively change the tunneling behavior. This is the first example of…

Condensed Matter · Physics 2009-10-22 Ard A. Louis , James P. Sethna

Strong hyperfine coupling in a 0.2% Holmium doped LiYF_4 single crystal induces staircaselike hysteresis loops of the magnetization at very low temperatures. The field sweep rate dependence of hysteresis loops allows the study of two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. Giraud , W. Wernsdorfer , A. M. Tkachuk , D. Mailly , B. Barbara

Tunneling two-level systems are ubiquitous in amorphous solids, and form a major source of noise in systems such as nano-mechanical oscillators, single electron transistors, and superconducting qubits. Occurance of defect tunneling despite…

Mesoscale and Nanoscale Physics · Physics 2017-07-10 P. Nalbach , M. Schechter

We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru
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