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We investigate the ultrafast magnetization dynamics of an interlayer-exchange-coupled Co/Mn/Co trilayer system after excitation with an ultrafast optical pump. We probe element- and time-resolved ferromagnetic order by X-ray magnetic…

We study the ultrafast demagnetization of Ni/NiMn and Co/NiMn ferromagnetic/antiferromagnetic bilayer systems after excitation by a laser pulse. We probe the ferromagnetic order of Ni and Co using magnetic circular dichroism in…

Manipulating spin in antiferromagnetic (AFM) materials has great potential in AFM opto-spintronics. Laser pulses can induce a transient ferromagnetic (FM) state in AFM metallic systems, but have never been proven in two-dimensional (2D) AFM…

Materials Science · Physics 2022-03-11 Shuo Li , Junjie He , Thomas Frauenheim

Resonant absorption of a photon by bound electrons in a solid can promote an electron to another orbital state or transfer it to a neighboring atomic site. Such a transition in a magnetically ordered material could affect the magnetic…

We investigate theoretically the dynamic multiferroic response of coupled ferroelectric/ferromagnetic composites upon excitation by a photo-induced acoustic strain pulse. Two magnetoelectric mechanisms are considered: interface strain- and…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 Chenglong Jia , Ning Zhang , Alexander Sukhov , Jamal Berakdar

Atomically engineered oxide heterostructures provide a fertile ground for creating novel states. For example, a two-dimensional electron gas at the interface between two oxide insulators, giant thermoelectric Seebeck coefficient, emergent…

Femtosecond reflection spectroscopy was performed on a perovskite-type manganite, Gd0.55Sr0.45MnO3, with the short-range charge and orbital order (CO/OO). Immediately after the photoirradiation, a large increase of the reflectivity was…

Ultrafast optical pump-probe spectroscopy is used to reveal the coexistence of coupled antiferromagnetic/ferroelectric and ferromagnetic orders in multiferroic TbMnO3 films through their time domain signatures. Our observations are…

Strongly Correlated Electrons · Physics 2015-06-05 J. Qi , L. Yan , H. D. Zhou , J. -X. Zhu , S. A. Trugman , A. J. Taylor , Q. X. Jia , R. P. Prasankumar

Ultrafast heating of FeRh by a femtosecond laser pulse launches a magneto-structural phase transition from an antiferromagnetic to a ferromagnetic state. Aiming to reveal the ultrafast kinetics of this transition, we studied magnetization…

Optically-induced phase transitions of the manganite $\rm Pr_{1/3}Ca_{2/3}MnO_3$ have been simulated using a model Hamiltonian, that captures the dynamics of strongly correlated charge, orbital, lattice, and spin degrees of freedom. Its…

Strongly Correlated Electrons · Physics 2020-12-01 Sangeeta Rajpurohit , Liang Z. Tan , Christian Jooss , P. E. Blöchl

We use transient absorption spectroscopy with circularly polarized x-rays to detect laser-excited hole states below the Fermi level and compare their dynamics with that of unoccupied states above the Fermi level in ferromagnetic [Co/Pd]…

By using intense coherent electromagnetic radiation, it may be possible to manipulate the properties of quantum materials very quickly, or even induce new and potentially useful phases that are absent in equilibrium. For instance, ultrafast…

Strongly Correlated Electrons · Physics 2023-03-30 Jonathan B. Curtis , Ankit Disa , Michael Fechner , Andrea Cavalleri , Prineha Narang

We have performed a two-color time-resolved magneto-optical Kerr effect (MOKE) study of a ferromagnetic InMnAs/GaSb heterostructure. We observed ultrafast photo-induced changes in the MOKE signal induced by a large density of spin-polarized…

Materials Science · Physics 2007-05-23 J. Wang , G. A. Khodaparast , J. Kono , T. Slupinski , A. Oiwa , H. Munekata

Precession of magnetization induced by pulsed optical excitation is observed in a ferromagnetic semiconductor (Ga,Mn)As by time-resolved magneto-optical measurements. It appears as complicated oscillations of polarization plane of…

Materials Science · Physics 2009-11-13 Y. Hashimoto , H. Munekata

Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Junhua Zhang , Joerg Schmalian , Tianqi Li , Jigang Wang

We investigate the demagnetization dynamics of the cycloidal and sinusoidal phases of multiferroic TbMnO$_3$ by means of time-resolved resonant soft x-ray diffraction following excitation by an optical pump. Using orthogonal linear x-ray…

Understanding how fast short-range interactions build up long-range order is one of the most intriguing topics in condensed matter physics. FeRh is a test specimen for studying this problem in magnetism, where the microscopic spin-spin…

We study ultrafast magnetization quenching of ferromagnetic iron following excitation by an optical vs a terahertz pump pulse. While the optical pump (photon energy of 3.1 eV) induces a strongly nonthermal electron distribution, terahertz…

We theoretically study photoinduced magnetic phase transitions and their dynamical processes in the Kondo-lattice model on a cubic lattice. It is demonstrated that light irradiation gives rise to magnetic phase transitions from the…

Strongly Correlated Electrons · Physics 2025-04-18 Ryo Hamano , Masahito Mochizuki

The ultrafast manipulation of magnetic order due to optical excitation is governed by the intricate flow of energy and momentum between the electron, lattice and spin subsystems. While various models are commonly employed to describe these…

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