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We provide theoretical and numerical tools to quantitatively study the impact of nonlocality arising from free electrons in metals on the optical properties of metallo-dielectric multilayers. Though effects due to nonlocality are in general…

We generalize the concept of charge regulation of ionic solutions, and apply it to complex fluids with mobile macro-ions having internal non-electrostatic degrees of freedom. The suggested framework provides a convenient tool for…

Soft Condensed Matter · Physics 2018-01-17 Tomer Markovich , David Andelman , Rudi Podgornik

The electric microfield distribution at charged particles is studied for two-component electron-ion plasmas using molecular dynamics simulation and theoretical models. The particles are treated within classical statistical mechanics using…

Plasma Physics · Physics 2009-11-11 H. B. Nersisyan , C. Toepffer , G. Zwicknagel

The effects of ion temperature are discussed in a two-ion electron plasma and for a model applicable to the oscillating sheath theory that has recently been much in the focus of researchers. The differences between the fluid and kinetic…

Plasma Physics · Physics 2009-11-13 J. Vranjes , B. P. Pandey , M. Y. Tanaka , S. Poedts

We formulate a general mean-field theory of a flat electric double layer in ionic liquids and electrolyte solutions with ions possessing static polarizability and a permanent dipole moment on a charged electrode. We establish a new…

Statistical Mechanics · Physics 2021-08-17 Yu. A. Budkov , S. V. Zavarzin , A. L. Kolesnikov

Nanoscopic heterogeneities in composition and structure are quintessential for the properties of electrocatalyst materials. Here, we present a semiclassical model to study the electrochemical properties of supported electrocatalyst…

Materials Science · Physics 2025-02-27 Yufan Zhang , Tobias Binninger , Jun Huang , Michael Eikerling

In this thesis we study the lateral electrostatic interaction between a pair of non-identical, moderately charged colloidal particles trapped at an electrolyte interface in the limit of short inter-particle separations. Using a simplified…

Soft Condensed Matter · Physics 2017-10-17 Timo Schmetzer

The motion of the charged particles in graphen in the frame of the quantum non-local hydrodynamic description is considered. It is shown as results of the mathematical modeling that the mentioned motion is realizing in the soliton forms.…

General Physics · Physics 2012-11-28 Boris V. Alexeev , Irina V. Ovchinnikova

The electrostatic screening properties of ionic fluids are of paramount importance in countless physical processes. Yet, the behavior of ionic conductors out of thermal equilibrium has to date mainly been studied in the context of…

Statistical Mechanics · Physics 2023-04-19 Andrea Grisafi , Federico Grasselli

Electrochemical devices often consist of multicomponent electrolyte solutions. Two processes influence the overall dynamics of these devices: the formation of electrical double layers and chemical conversion due to redox reactions. However,…

Chemical Physics · Physics 2022-06-20 Nathan Jarvey , Filipe Henrique , Ankur Gupta

The two-fluid model is a phenomenological description of the gradual change of the itinerant and local characters of the f-electrons with temperature and other tuning parameters and has been quite successful in explaining many unusual and…

Strongly Correlated Electrons · Physics 2016-06-01 Yi-feng Yang

In recent years, ionic microgels have garnered much attention due to their unique properties, especially their stimulus-sensitive swelling behavior. The tunable response of these soft, permeable, compressible, charged colloidal particles is…

Soft Condensed Matter · Physics 2023-12-18 Mohammed O. Alziyadi , Alan R. Denton

We develop a consistent quantum description of surface plasmons interacting with quantum emitters and external electromagnetic field. Within the framework of macroscopic electrodynamics in dispersive and absorptive medium, we derive, in the…

Mesoscale and Nanoscale Physics · Physics 2021-01-21 Tigran V. Shahbazyan

Nonlocal effects have been shown to be responsible for a variety of non-trivial optical effects in small-size plasmonic nanoparticles, beyond classical electrodynamics. However, it is not clear whether optical mode descriptions can be…

We propose a nonlocal Poisson-Fermi model for ionic solvent that includes ion size effects and polarization correlations among water molecules in the calculation of electrostatic potential. It includes the previous Poisson-Fermi models as…

Chemical Physics · Physics 2016-08-03 Dexuan Xie , Jinn-Liang Liu , Bob Eisenberg , L. Ridgway Scott

Polymer electrolytes are intensely investigated for use as solid electrolytes in next generation lithium-ion and lithium-metal batteries. However, little is known about the structural and dynamical properties of polymer electrolytes close…

Soft Condensed Matter · Physics 2021-12-02 Andreas Thum , Diddo Diddens , Andreas Heuer

Historically, the field of plasmonics has been relying on the framework of classical electrodynamics, with the local-response approximation of material response being applied even when dealing with nanoscale metallic structures. However,…

The classical Poisson-Boltzmann (PB) theory of electrolytes assumes a dilute solution of point charges with mean-field electrostatic forces. Even for very dilute solutions, however, it predicts absurdly large ion concentrations (exceeding…

Chemical Physics · Physics 2007-05-23 Mustafa Sabri Kilic , Martin Z. Bazant , Armand Ajdari

The nonlinear electrokinetic response of ionic solutions is important in nanofluidics. However, quantitatively understanding the mechanisms is still a challenging problem because of a lack of analytic approaches. Here, a general framework…

Fluid Dynamics · Physics 2023-05-26 Yuki Uematsu

Thermodynamics and dynamics of a classical two-dimensional system with dipole-like isotropic repulsive interactions are studied systematically using extensive molecular dynamics (MD) simulations supplemented by appropriate theoretical…

Soft Condensed Matter · Physics 2018-03-02 Sergey Khrapak , Nikita Kryuchkov , Stanislav Yurchenko