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In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek

Exciton binding energies of hundreds of meV and strong light absorption in the optical frequency range make transition metal dichalcogenides (TMDs) promising for novel optoelectronic nanodevices. In particular, atomically thin TMDs can be…

Mesoscale and Nanoscale Physics · Physics 2018-04-24 Simon Ovesen , Samuel Brem , Christopher Linderälv , Mikael Kuisma , Paul Erhart , Malte Selig , Ermin Malic

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. While optical signatures of excitons have been studied extensively, experimental access to the excitonic…

The optical properties of semiconducting transition metal dichalcogenides are dominated by both neutral excitons (electron-hole pairs) and charged excitons (trions) that are stable even at room temperature. While trions directly influence…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Kai Hao , Lixiang Xu , Philipp Nagler , Akshay Singh , Kha Tran , Chandriker Kavir Dass , Christian Schüller , Tobias Korn , Xiaoqin Li , Galan Moody

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and…

Mesoscale and Nanoscale Physics · Physics 2022-11-02 Raul Perea-Causin , Daniel Erkensten , Jamie M. Fitzgerald , Joshua J. P. Thompson , Roberto Rosati , Samuel Brem , Ermin Malic

Atomically thin transition metal dichalcogenides (TMDs) are direct-gap semiconductors with strong light-matter and Coulomb interaction. The latter accounts for tightly bound excitons, which dominate the optical properties of these…

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 Dinh Van Tuan , Hanan Dery

Starting from the single-particle Dirac Hamiltonian for charge carriers in monolayer transition metal dichalcogenides (TMDs), we construct a four-band Hamiltonian describing interlayer excitons consisting of an electron in one TMD layer and…

Mesoscale and Nanoscale Physics · Physics 2018-09-05 M. Van der Donck , F. M. Peeters

The physics of excitons, electron-hole pairs that are bound together by their mutual Coulomb attraction, can to great extent be understood in the framework of the quantum-mechanical hydrogen model. This model has recently been challenged by…

Mesoscale and Nanoscale Physics · Physics 2017-09-15 Maxim Trushin , Mark Oliver Goerbig , Wolfgang Belzig

Two-dimensional group-VI transition metal dichalcogenide semiconductors, such as MoS2, WSe2 and others, exhibit strong light-matter coupling and possess direct band gaps in the infrared and visible spectral regimes, making them potentially…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Thomas Mueller , Ermin Malic

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

Monolayer transition metal dichalcogenides (TMDs) exhibit a remarkably strong Coulomb interaction that manifests in tightly bound excitons. Due to the complex electronic band structure exhibiting several spin-split valleys in the conduction…

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

Mesoscale and Nanoscale Physics · Physics 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

Exciton-polaritons - coherently hybridized states of excitons and photons - are instrumental for solid-state nonlinear optics and quantum simulations. To enable engineered polariton energy landscapes and interactions, local control over the…

Monolayer transition metal dichalcogenides (1L-TMDs) have tremendous potential as atomically thin, direct bandgap semiconductors that can be used as convenient building blocks for quantum photonic devices. However, the short exciton…

We develop a stochastic theory that treats time-dependent exciton-exciton s-wave scattering and that accounts for dynamic Coulomb screening, which we describe within a mean-field limit. With this theory, we model excitation-induced…

Chemical Physics · Physics 2020-10-26 Ajay Ram Srimath Kandada , Hao Li , Félix Thouin , Eric R. Bittner , Carlos Silva

Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…

Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and…

Monolayer transition metal dichalcogenides feature tightly bound bright excitons at the degenerate valleys, where electron-hole Coulomb exchange interaction strongly couples the valley pseudospin to the momentum of exciton. Placed on…

Mesoscale and Nanoscale Physics · Physics 2022-06-01 Xu-Chen Yang , Hongyi Yu , Wang Yao