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The simultaneous ordering of different degrees of freedom in complex materials undergoing spontaneous symmetry-breaking transitions often involves intricate couplings that have remained elusive in phenomena as wide ranging as stripe…

Femtosecond time-resolved core-level photoemission spectroscopy with a free-electron laser is used to measure the atomic-site specific charge-order dynamics in the charge-density-wave/Mott insulator 1T-TaS2. After strong photoexcitation, a…

The strong coupling between lattice modes and charges which leads to the formation of charge density waves in materials such as the transition-metal dichalcogenides may also give rise to superconductivity in the same materials, mediated by…

Superconductivity · Physics 2015-06-29 Jasper van Wezel , Paul Nahai-Williamson , Siddarth S. Saxena

The electronic structure of a new charge-density-wave/ superconductor system, 1T-CuxTiSe2, has been studied by photoemission spectroscopy. A correlated semiconductor band structure is revealed for the undoped case. With Cu doping, the…

Strongly Correlated Electrons · Physics 2009-11-11 J. F. Zhao , H. W. Ou , G. Wu , B. P. Xie , Y. Zhang , D. W. Shen , J. Wei , L. X. Yang , J. K. Dong , M. Arita , H. Namatame , M. Taniguchi , X. H. Chen , D. L. Feng

We study the charge-density wave phase in $\textup{TiSe}_2$ by using first principle calculations. We show that, regardless of the local functional used and as long as the cell parameters are in agreement with the experiment,…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 Raffaello Bianco , Matteo Calandra , Francesco Mauri

Revealing the interactions binding electronic and lattice components of cooperative quantum order is central to sculpting new states of matter. This challenge is epitomized by the charge density wave material 1T-TiSe$_2$, where…

At low temperature TiSe2 undergoes a charge density wave instability. Superconductivity is stabilized either by pressure or by Cu intercalation. We show that the pressure phase diagram of TiSe2 is well described by first-principles…

Materials Science · Physics 2015-05-27 Matteo Calandra , Francesco Mauri

Complex materials encompassing different phases of matter can display new photoinduced metastable states differing from those attainable under equilibrium conditions. These states can be realized when energy is injected in the material…

Strongly Correlated Electrons · Physics 2024-06-27 Wibke Bronsch , Manuel Tuniz , Denny Puntel , Alessandro Giammarino , Fulvio Parmigiani , Yang-hao Chan , Federico Cilento

The ultrafast electronic structures of the charge density wave material 1T-TiSe$_2$ were investigated by high-resolution time- and angle-resolved photoemission spectroscopy. We found that the quasiparticle populations drove ultrafast…

Strongly Correlated Electrons · Physics 2023-06-02 Shaofeng Duan , Wei Xia , Chaozhi Huang , Shichong Wang , Lingxiao Gu , Haoran Liu , Dao Xiang , Dong Qian , Yanfeng Guo , Wentao Zhang

The origin of charge density waves (CDW) in TiSe$_2$ has long been debated, mainly due to the difficulties in identifying the timescales of how and when the excitonic pairing and electron-phonon coupling (EPC) come into play. Without a…

Mesoscale and Nanoscale Physics · Physics 2020-01-07 Chao Lian , Sheng-Jie Zhang , Shi-Qi Hu , Meng-Xue Guan , Sheng Meng

The correlation between electronic and crystal structures of 1T-TiSe2 in the charge density wave (CDW) state is studied by x-ray diffraction. Three families of reflections are used to probe atomic displacements and the orbital asymmetry in…

A number of intriguing phenomena, including exciton condensation, orbital ordering, and emergence of chirality, have been proposed to accompany charge-density-wave (CDW) formation in the layered transition metal dichalcogenide…

Strongly Correlated Electrons · Physics 2025-02-18 Wei Wang , Patrick Liu , Lijun Wu , Jing Tao , Genda Gu , Alfred Zong , Yimei Zhu

The Bose-Einstein condensation of excitons continues to garner immense attention as a prototypical example for observing emergent properties from many-body quantum effects. In particular, Titanium Diselenide (TiSe$_2$) is a promising…

Materials Science · Physics 2019-12-06 Chao Lian , Zulfikhar A. Ali , Bryan M. Wong

In low-dimensional metallic systems, lattice distortion is usually coupled to a density-wave-like electronic instability due to Fermi surface nesting (FSN) and strong electron-phonon coupling. However, the ordering of other electronic…

Strongly Correlated Electrons · Physics 2018-12-26 D. W. Song , J. Li , D. Zhao , L. K. Ma , L. X. Zheng , S. J. Li , L. P. Nie , X. G. Luo , Z. P. Yin , T. Wu , X. H. Chen

Charge density waves (CDWs) underpin the electronic properties of many complex materials. Near-equilibrium CDW order is linearly coupled to a periodic, atomic-structural distortion, and the dynamics is understood in terms of amplitude and…

We study the non-equilibrium structural dynamics of the incommensurate and nearly-commensurate charge-density wave phases in 1T-TaS$_2$. Employing ultrafast low-energy electron diffraction (ULEED) with 1 ps temporal resolution, we…

Recent experiments suggest that excitonic degrees of freedom play an important role in precipitating the charge density wave (CDW) transition in $1T$-$\mathrm{TiSe}_2$. Through systematic calculations of the electronic and phonon spectrum…

Mesoscale and Nanoscale Physics · Physics 2018-12-03 Chuan Chen , Bahadur Singh , Hsin Lin , Vitor M. Pereira

Time-resolved elastic neutron scattering combined with rapid laser heating was used to probe the charge density wave (CDW) state in 1T-TiSe$_2$, capturing both the melting and reformation of the CDW on long timescales and providing clues on…

Materials Science · Physics 2025-09-22 K. Dharmasiri , S. S. Philip , D. Louca , S. A. Chen , M. D. Frontzek , Z. J. Morgan , C. Hua

Layered 1$T$-TiSe$_{2}$ has attracted much interest for the competition of charge density wave (CDW) and superconductivity in its bulk and even monolayer forms. Here we perform first-principles calculations of the electronic structure,…

Superconductivity · Physics 2018-08-01 Bao-Tian Wang , Peng-Fei Liu , Jing-Jing Zheng , Wen Yin , Fangwei Wang

We explore the interplay of a charge density wave (CDW) order and s-wave superconductivity (sSC) in a disordered system. Recent experiments on 1T-TiSe_2, where the pristine sample has a commensurate CDW order and the superconductivity…

Superconductivity · Physics 2018-10-03 Anurag Banerjee , Arti Garg , Amit Ghosal
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