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Upcoming high-intensity laser systems will be able to probe the quantum-induced nonlinear regime of electrodynamics. So far unobserved QED phenomena such as the discovery of a nonlinear response of the quantum vacuum to macroscopic…

High Energy Physics - Phenomenology · Physics 2009-10-29 Holger Gies

Spectroscopy is the most important method for probing the structure of molecules. However, predicting molecular spectra on classical computers is computationally expensive, with the most accurate methods having a cost that grows…

Quantum Physics · Physics 2025-10-06 Liam P. Flew , Ivan Kassal

Calculation of the coherent nonlinear response of a system is essential to correctly interpret results from advanced techniques such as two-dimensional coherent spectroscopy (2DCS). Usually, even for the simplest systems, such calculations…

We start a series of studies of the excitation of an optical target by quantum light. In this first part, we introduce the problematic and address the first case of interest, that of exciting the quantum harmonic oscillator, corresponding…

Quantum Physics · Physics 2017-02-15 J. C. López Carreño , F. P. Laussy

Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission…

Quantum Physics · Physics 2020-08-10 Akihito Ishizaki

We explore how the Jaynes-Cummings ladder transpires in the emitted spectra of a two-level system in strong coupling with a single mode of light. We focus on the case of very strong coupling, that would be achieved with systems of…

Mesoscale and Nanoscale Physics · Physics 2009-07-09 Fabrice P. Laussy , Elena del Valle

Conical intersections (CIs) have been widely studied using spectroscopic techniques. However, CIs have mainly been identified by rapid internal conversion transitions that take place after the photoexcitation. Such identifications cannot…

Chemical Physics · Physics 2018-12-26 Hazem Daoud , Loic Joubert-Doriol , Artur F. Izmaylov , R. J. Dwayne Miller

We present a full microscopic many-body calculation of a recently-proposed nonlinear two-dimensional spectroscopy for Fermi polarons, and show that the quantum coherence between the attractive and repulsive polarons, which has never been…

Quantum Gases · Physics 2022-08-04 Jia Wang , Hui Hu , Xia-Ji Liu

A detailed analysis of the process of two photon emission by an electron scattered from a high-intensity laser pulse is presented. The calculations are performed in the framework of strong-field QED and include exactly the presence of the…

High Energy Physics - Phenomenology · Physics 2013-02-13 F. Mackenroth , A. Di Piazza

The quantum vacuum constitutes a fascinating medium of study, in particular since near-future laser facilities will be able to probe the nonlinear nature of this vacuum. There has been a large number of proposed tests of the low-energy,…

High Energy Physics - Theory · Physics 2010-04-23 Mattias Marklund , Joakim Lundin

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…

Optics · Physics 2017-01-24 Jonathan Tollerud , Jeffrey Davis

Recent interest in the role of quantum mechanics in the primary events of photosynthetic energy transfer has led to a convergence of nonlinear optical spectroscopy and quantum optics on the topic of energy-transfer dynamics in…

Quantum Physics · Physics 2014-01-23 Agata M. Branczyk , Daniel B. Turner , Gregory D. Scholes

Phase-sensitive pump-probe hyperspectral imaging is a precise technique for absolute two-beam measurements of the optical Kerr coefficient ($n_2$). The irradiance profile is characterized and background effects are rejected by rastering the…

Optics · Physics 2026-04-14 J. K. Wahlstrand , C. D. Cruz

Two-level systems (TLS) of unclear physical origin are a major contributor to decoherence in superconducting qubits. The interactions of individual TLS with a qubit can be detected via various spectroscopic methods, most of which have…

A survey of physical parameters and of a ladder of various regimes of laser-matter interactions at extreme intensities is given. Special emphases is made on three selected topics: (i) qualitative derivation of the scalings for probability…

Optics · Physics 2016-12-08 Alexander Fedotov

Coupled laser arrays exhibit rich and complex physical properties, making them powerful tools for exploring a wide range of phenomena. They enable efficient ground-state optimization of complex landscapes, solve computational problems,…

Optics · Physics 2025-02-10 Simon Mahler

We apply quantum field theory to study the excitation spectrum of doped two-leg ladders. It follows from our analysis that throughout most of the phase diagram the spectrum consists of degenerate quartets of kinks and anti-kinks and a…

Strongly Correlated Electrons · Physics 2009-11-11 D. Controzzi , A. M. Tsvelik

We present a comprehensive study of the optical transitions and selection rules of variably charged single self-assembled InAs/GaAs quantum dots. We apply high resolution polarization sensitive photoluminescence excitation spectroscopy to…

Mesoscale and Nanoscale Physics · Physics 2012-08-28 Y. Benny , Y. Kodriano , E. Poem , T. A. Truong , P. M. Petroff , D. Gershoni

We consider a non-relativistic quantum particle interacting with a singular potential supported by two parallel straight lines in the plane. We locate the essential spectrum under the hypothesis that the interaction asymptotically…

Spectral Theory · Mathematics 2014-06-12 Sylwia Kondej , David Krejcirik