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We show that the standard perturbative (i.e., cubic) description of the thermal nonlinear response of small metal nanospheres to intense continuous wave illumination is insufficient already beyond temperature rises of a few tens of degrees.…

Optics · Physics 2017-07-19 I. Gurwich , Y. Sivan

We solve the Maxwell and heat equations self-consistently for metal nanoparticles under intense continuous wave (CW) illumination. Unlike previous studies, we rely on {\em experimentally}-measured data for the metal permittivity for…

Optics · Physics 2016-07-13 Yonatan Sivan , Shi-Wei Chu

Understanding the intricate relation between illumination and temperature in metallic nano-particles is crucial for elucidating the role of illumination in various physical processes which rely on plasmonic enhancement but are also…

Chemical Physics · Physics 2023-03-31 Ieng-Wai Un , Yonatan Dubi , Yonatan Sivan

We study the thermal response of a single spherical metal nanoparticle to continuous wave illumination as a function of its size. We show that the particle temperature increases non-monotonically as the particle size increases, indicating…

Optics · Physics 2020-01-08 Ieng-Wai Un , Yonatan Sivan

Plasmonic absorption of light can lead to significant local heating in metallic nanostructures, an effect that defines the sub-field of thermoplasmonics and has been leveraged in diverse applications from biomedical technology to…

Mesoscale and Nanoscale Physics · Physics 2014-02-21 Joseph B. Herzog , Mark W. Knight , Douglas Natelson

We investigate the nonlinear optical response of suspended 1D photonic crystal nanocavities fabricated on a silicon nitride chip. Strong thermo-optical nonlinearities are demonstrated for input powers as low as $2\,\mu\text{W}$ and a…

Thermal and photothermal effects play an increasing role at the nanoscale due to the general decrease of thermal conductances and to the increasing role of interfaces. Here we present a non-contact optomechanical analysis of the thermal and…

Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in…

Recently, there has been a growing interest in the usage of mm-scale composites of plasmonic nanoparticles for enhancing the rates of chemical reactions; the effect was shown recently to be predominantly associated with the elevated…

Applied Physics · Physics 2023-03-31 Ieng-Wai Un , Yonatan Sivan

A theory of weakly-nonlinear low-temperature relaxational absorption of acoustic and electromagnetic waves in dielectric and metallic glasses is developed. Basing upon the model of two-level tunneling systems we show that the nonlinear…

Disordered Systems and Neural Networks · Physics 2009-10-30 M. Kirkengen , Yu. M. Galperin

Nonlinear highly multimode photonic systems are ubiquitous in optics. Yet, the sheer complexity arising from the action of nonlinearity in multimode environments has posed theoretical challenges in describing these systems. In this work, we…

The optical response of materials based on gold nanoparticle assemblies depends on many parameters regarding both material morphology and light excitation characteristics. In this paper, the interplay between the optical and thermal…

Quantum dots are useful model systems for studying quantum thermoelectric behavior because of their highly energy-dependent electron transport properties, which are tunable by electrostatic gating. As a result of this strong energy…

Mesoscale and Nanoscale Physics · Physics 2016-06-17 Artis Svilans , Adam M. Burke , Sofia Fahlvik Svensson , Martin Leijnse , Heiner Linke

Promising applications in photonics are driven by the ability to fabricate crystal-quality metal thin films of controlled thickness down to a few nanometers. In particular, these materials exhibit a highly nonlinear response to optical…

Mesoscale and Nanoscale Physics · Physics 2023-08-21 A. Rodríguez Echarri , F. Iyikanat , S. Boroviks , N. Asger Mortensen , Joel D. Cox , F. Javier García de Abajo

Leveraging strong optoelectronic responses to external stimuli, such as temperature and electric fields, is central to the development of advanced photonic technologies, including adaptive photodetectors and reconfigurable photovoltaic…

Materials Science · Physics 2026-02-25 Pol Benítez , Cibrán López , Edgardo Saucedo , Claudio Cazorla

We investigate, theoretically and numerically, the dependence of a material's nonlinear-optical response on the linear relative electric permittivity $\epsilon$ and magnetic permeability $\mu$. The conversion efficiency of low-order…

Optics · Physics 2025-09-24 Diego M. Solís , Robert W. Boyd , Nader Engheta

We investigate the polarization dependence of optical nonlinearity enhancement for a uniaxial anisotropic composite of metal nanocrystals in a dielectric host. Three cases are distinguished depending on whether the polarization is parallel,…

Soft Condensed Matter · Physics 2007-05-23 K. P. Yuen , M. F. Law , K. W. Yu , Ping Sheng

Silicon photonics has attracted significant interest in recent years due to its potential in integrated photonics components (1,2) as well as all-dielectric meta-optics elements.(3) Strong photon-photon interactions, aka optical…

Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light-matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of…

Optics · Physics 2023-04-20 Y. Sivan , I. W. Un , I. Kalyan , K. -Q. Lin , J. M. Lupton , S. Bange

The pulsed photothermal phenomenon due to optically absorbed energy, result from non-radiative decay mechanisms, which in nature, these imply the temporal change in the local free energy and thus a temporary change in the local temperature.…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 M. Rodríguez-Matus , C. Garcia-Segundo , Jean-Parick Connerade
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