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Strong coupling of molecules to the vacuum field of micro cavities can modify the potential energy surfaces opening new photophysical and photochemical reaction pathways. While the influence of laser fields is usually described in terms of…

Quantum Physics · Physics 2016-02-08 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

Mesoscale and Nanoscale Physics · Physics 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl

The capability of optical resonators to extend the effective radiation-matter interaction length originates from a multipass effect, hence is intrinsically limited by the resonator quality factor. Here, we show that this constraint can be…

Optics · Physics 2016-07-05 P. Malara , C. E. Campanella , A. Giorgini , S. Avino , P. De Natale , G. Gagliardi

Achieving strong coupling between light and matter is usually a challenge in Cavity Quantum Electrodynamics (cQED), especially in solid state systems. For this reason is useful taking advantage of alternative approaches to reach this…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 J. E. Ramírez-Muñoz , J. P. Restrepo Cuartas , H. Vinck-Posada

The ultrafast non-radiative relaxation of a molecular ensemble coupled to a cavity mode is considered theoretically and by real-time quantum dynamics. For equal coupling strength of single molecules to the cavity mode, the non-radiative…

Chemical Physics · Physics 2018-12-26 Oriol Vendrell

Intermixed light-matter quasiparticles - polaritons - possess unique optical properties owned to their compositional nature. These intriguing hybrid states have been extensively studied over the past decades in a wide range of realizations…

The increased decay rate of a two-level system weakly coupled to an optical cavity, known as the Purcell effect, is a cornerstone of cavity QED. However, the effect of cavity coupling is not well understood if the two-level system is…

Quantum Physics · Physics 2023-06-19 Charlie Nation , Valentina Notararigo , Alexandra Olaya-Castro

We theoretically investigate the optical response of a one-dimensional array of strongly nonlinear optical microcavities. When the optical nonlinearity is much larger than both losses and inter-cavity tunnel coupling, the non-equilibrium…

Other Condensed Matter · Physics 2013-05-29 Iacopo Carusotto , Dario Gerace , Hakan Tureci , Simone De Liberato , Cristiano Ciuti , Atac Imamoglu

We investigate a hybrid optomechanical system in which a membrane oscillator is coupled to a collective spin of ground states of an intracavity $\Lambda$-type three-level atomic medium. The cavity field response is greatly modified by…

Optics · Physics 2015-06-22 Haibin Wu , Min Xiao

Recent experiments have demonstrated that molecular polaritons, hybrid states of light and matter formed by the strong coupling between molecular electronic or vibrational excitations and an optical cavity, can substantially modify the…

Chemical Physics · Physics 2021-07-08 Nguyen Thanh Phuc

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

We study a system of a transition metal dichalcogenide (TMD) monolayer placed in an optical resonator, where strong light-matter coupling between excitons and photons is achieved. We present quantitative theory of the nonlinear optical…

Mesoscale and Nanoscale Physics · Physics 2020-10-09 V. Shahnazaryan , V. K. Kozin , I. A. Shelykh , I. V. Iorsh , O. Kyriienko

Very efficient amplification of light-matter waves (polaritons), that are a superposition of cavity photons and excitons [1] has recently been reported[2-11]. The optical gain curve versus the pump power shows a threshold and then saturates…

Materials Science · Physics 2007-05-23 S. Savasta , O. Di Stefano , R. Girlanda

Polariton emission from optical cavities integrated with various luminophores has been extensively studied recently due to the wide variety of possible applications in photonics, particularly promising in terms of fabrication of…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Dmitriy Dovzhenko , Maksim Lednev , Konstantin Mochalov , Ivan Vaskan , Pavel Samokhvalov , Yury Rakovich , Igor Nabiev

Strong light-matter coupling provides a versatile and novel means to manipulate chemical processes. Here we develop a theoretical framework to investigate the spectroscopy and dynamics of a molecular ensemble embedded in an optical cavity…

Quantum Physics · Physics 2023-06-16 Bing Gu

When light and matter interact strongly, the resulting hybrid system inherits properties from both constituents, allowing one to modify material behavior by engineering the surrounding electromagnetic environment. This concept underlies the…

We discuss theoretically the light-matter coupling in a microcavity containing a quantum well with a two-dimensional electron gas. The high density limit where the bound exciton states are absent is considered. The matrix element of…

Mesoscale and Nanoscale Physics · Physics 2007-12-01 N. S. Averkiev , M. M. Glazov

The central theme of cavity quantum electrodynamics is the coupling of a single optical mode with a single matter excitation, leading to a doublet of cavity polaritons which govern the optical properties of the coupled structure. Especially…

The enormous progress in controlling quantum optical and atomic systems has prompted ideas for new experimental realizations of strongly correlated many-body systems operating with light. These systems consist of photons confined in optical…

Other Condensed Matter · Physics 2015-03-17 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

Two dimensional (2D) atomic crystals of graphene, and transition metal dichalcogenides have emerged as a class of materials that show strong light-matter interaction. This interaction can be further controlled by embedding such materials…

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