Related papers: Laplacian-Level Quantum Hydrodynamic Theory for Pl…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…
In this paper we study global existence of weak solutions for the Quantum Hydrodynamics System in 2-D in the space of energy. We do not require any additional regularity and/or smallness assumptions on the initial data. Our approach…
Plasmon excitations in metallic nanostructures can decay directly into dynamic electron-hole pairs (EHPs), exploitable for photocurrent generation. This approach has extensively been employed to develop nanoplasmonic light-sensing devices…
Quantum-electrodynamical density-functional theory (QEDFT) provides a first-principles framework for describing materials coupled to quantized electromagnetic fields. While QEDFT has successfully captured cavity-induced modifications of…
In this paper we consider the one dimensional quantum hydrodynamics (QHD) system, with a genuine hydrodynamic approach. The global existence of weak solutions with large data has been obtained in [2, 3], in several space dimensions, by…
We study theoretically the optical response of a nanohybrid comprising a symmetric quantum dimer emitter coupled to a metal nanoparticle (MNP). The interactions between the exitonic transitions in the dimer and the plasmons in the MNP lead…
The rapid progress of nanophotonics demands theoretical frameworks capable of predicting the resonant behavior of complex systems comprising constituents of varying nature, operating beyond the weak-coupling, high-Q regime where classical…
Group 4 transition metal nitride (TMN) nanoparticles (NPs) display strong plasmonic responses in the visible and near-infrared regimes, exhibit high melting points and significant chemical stability and thus are potential earth-abundant…
Highly lossy nature of metals has severely limited the scope of practical applications of plasmonics. The conventional approach to circumvent this limitation has been to search for new materials with more favorable dielectric properties…
Our conventional understanding of optical responses in metals has been based on the Drude theory. In recent years, however, it has become possible to prepare ultrapure metallic samples where the electron-electron scattering becomes the most…
Tho-photon absorption holds potential for many practical applications. We theoretically investigate the onset of this phenomenon in a semiconductor quantum dot -- metallic nanoshell composite subjected to a resonant CW excitation.…
To make relevant predictions about observable emission, hydrodynamical simulation codes must employ schemes that account for radiative losses, but the large dimensionality of accurate radiative transfer schemes is often prohibitive.…
Quantum hydrodynamics is a formulation of quantum mechanics based on the probability density and flux (current) density of a quantum system. It can be used to define trajectories which allow for a particle-based interpretation of quantum…
Performing electronic structure calculations for large systems, such as nanoparticles or metal clusters, via orbital based Hartree-Fock or Kohn-Sham theories is computationaly demanding. To study such systems, therefore, we have taken…
Nanoparticle surface structure and geometry generally dictate where chemical transformations occur, with the low-coordination-number, high-radius-of-curvature sites being energetically-preferred. Here, we show how optical excitation of…
We calculate the x-ray absorption spectra of liquid water at ambient conditions and of hexagonal ice close to melting, using a static GW approach that includes approximately local field effects. Quantum dynamics of the nuclei is taken into…
The plasmonic properties of sphere-like bcc Na nanoclusters ranging from Na$_{15}$ to Na$_{331}$ have been studied by real-time time-dependent local density approximation calculations. The optical absorption spectrum, density response…
Surface lattice resonance supported on plasmonic nanoparticle arrays enhances light-matter interactions for applications such as photoluminescence enhancement. The photoluminescence process is enhanced through confining light beyond the…
Orbital-free density functional theory (OF-DFT) constitutes a computationally highly effective tool for modeling electronic structures of systems ranging from room-temperature materials to warm dense matter. Its accuracy critically depends…
We develop an approximate quasi-static theory describing the low-frequency plasmonic resonances of slender nanometallic rings and configurations thereof. First, we use asymptotic arguments to reduce the plasmonic eigenvalue problem…