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We report on an inelastic (Raman) light scattering study of the local structure of amorphous GeTe films. A detailed analysis of the temperature-reduced Raman spectra has shown that appreciable structural changes occur as a function of…

Materials Science · Physics 2009-11-11 K. S. Andrikopoulos , S. N. Yannopoulos , G. A. Voyiatzis , A. V. Kolobov , M. Ribes , J. Tominaga

The nature of enhanced photoemission in disordered and amorphous solids is an intriguing open question. A point in case is light emission in silicon, which occurs when the material is porous or nanostructured, but the effect is absent in…

Bulk glass formation occurs over a very small part of phase space, and "good" glasses (which form even at low quench rates ~ 10K/sec) select an even smaller part of that accessible phase space. An axiomatic theory provides the physical…

Soft Condensed Matter · Physics 2009-11-13 P. Boolchand , Mingji Jin , D. I. Novita , S. Chakravarty

Near-bandgap Raman scattering was used to induce and study photostructural changes in AsxS100-x bulk glasses revealing a new photoinduced polymerization effect. Raman spectra were recorded also in off-resonant conditions allowing for a…

Materials Science · Physics 2009-11-13 F. Kyriazis , S. N. Yannopoulos

The anharmonic lattice dynamics of oxide and halide perovskites play a crucial role in their mechanical and optical properties. Raman spectroscopy is one of the key methods used to study these structural dynamics. However, despite decades…

A synopsis of the various photoinduced changes of rheological, mechanical and elastic properties is presented in the first part of the article. After a critical appraisal of a large body of experimental data it suggested that the…

Materials Science · Physics 2009-08-13 S. N. Yannopoulos , M. L. Trunov

Systematic Raman experiments performed on water and water-ethanol samples, stored in different containers (fused silica, polypropylene, soda-lime glass type III) for several hours, have shown that the luminescence contribution to the Raman…

Raman spectra from silicon nanostructures, recorded using excitation laser power density of 1.0 kW/cm^2, is employed here to reveal the dominance of thermal effects at temperatures higher than the room temperature. Room temperature Raman…

Mesoscale and Nanoscale Physics · Physics 2012-01-25 Rajesh Kumar , Vivek Kumar , A. K. Shukla

Inelastic light scattering is an intensively used tool in the study of electronic properties of solids. Triggered by the discovery of high temperature superconductivity in the cuprates and by new developments in instrumentation, light…

Strongly Correlated Electrons · Physics 2009-11-11 T. P. Devereaux , R. Hackl

The effects of plasticization of poly(methyl methacrylate) glass on the boson peaks observed by Raman and neutron scattering are compared. In plasticized glass the cohesion heterogeneities are responsible for the neutron boson peak and…

Condensed Matter · Physics 2007-05-23 E. Duval , L. Saviot , A. Mermet , L. David , S. Etienne , V. Bershtein , A. J. Dianoux

Atomic scale computer simulations on structures and photo induced volume changes of flatly and obliquely deposited amorphous selenium films have been carried out in order to understand how the properties of chalcogenide glasses are…

Materials Science · Physics 2009-11-13 Rozalia Lukacs , Jozsef Hegedus , Sandor Kugler

We use vortex photon fields with orbital and spin angular momentum to probe chiral fluctuations within liquid crystals. In the regime of iridescence with a well-defined pitch length of chirality, we find low energy Raman scattering that can…

Soft Condensed Matter · Physics 2023-08-21 Silvia Müllner , Florian Büscher , Angela Möller , Peter Lemmens

Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…

Optics · Physics 2021-08-10 Xiao Liu , Zelin Ma , Aku Antikainen , Siddharth Ramachandran

Propagation of light in a highly scattering medium is among the most fascinating optical effect that everyone experiences on an everyday basis and possesses a number of fundamental problems which have yet to be solved. Conventional wisdom…

Raman spectra of thin solid electrolyte films obtained by sputtering a lithium sulfate target in nitrogen plasma are measured and compared to ab initio electronic structure calculations for clusters composed of 28 atoms. Agreement between…

Materials Science · Physics 2009-11-13 Christian Muller , Patrik Johansson , Maths Karlsson , Philipp Maass , Aleksandar Matic

An important source of opacity in exoplanet atmospheres at short visible and near-UV wavelengths is Rayleigh scattering of light on molecules. It is accompanied by a related, albeit weaker process -- Raman scattering. We analyze the…

Earth and Planetary Astrophysics · Physics 2016-11-23 Antonija Oklopčić , Christopher M. Hirata , Kevin Heng

Diagnostic potential of the spectral signatures of Raman scattering imprinted in planetary albedo spectra at short optical wavelengths has been demonstrated in research on Solar System planets and has recently been proposed as a probe of…

Earth and Planetary Astrophysics · Physics 2017-09-13 Antonija Oklopčić , Christopher M. Hirata , Kevin Heng

Pressure-dependent, low temperature inelastic light (Raman) scattering measurements of KCuF$_3$ show that applied pressure above $P^{*} \sim$ 7 kbar suppresses a previously observed structural phase transition temperature to zero…

Strongly Correlated Electrons · Physics 2015-05-28 S. Yuan , M. Kim , J. Seeley , S. Lal , P. Abbamonte , S. L. Cooper

The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…

Materials Science · Physics 2021-07-07 Guru Khalsa , Nicole A. Benedek , Jeffrey Moses

We report a Raman study of the effect of temperature on the self-energies of optical phonons in a number of transition metals with hexagonal-close-packed structure. Anisotropic softening of phonon energies and narrowing of phonon linewidths…

Materials Science · Physics 2017-01-04 Yu. S. Ponosov , S. V. Streltsov
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