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The negatively charged nitrogen-vacancy (NV-) center in diamond has realized new frontiers in quantum technology. Here, the center's optical and spin resonances are observed under hydrostatic pressures up to 60 GPa. Our observations…

We demonstrate optical coupling between a single tin-vacancy (SnV) center in diamond and a free-standing photonic crystal nanobeam cavity. The cavities are fabricated using quasi-isotropic etching and feature experimentally measured quality…

There is a continuous search for solid-state spin qubits operating at room temperature with excitation in the IR communication bandwidth. Recently we have introduced the photoelectric detection of magnetic resonance (PDMR) to read the…

Materials Science · Physics 2018-06-20 E. Londero , E. Bourgeois , M. Nesladek , A. Gali

The nitrogen-vacancy (NV) color center in diamond is an atom-like system in the solid-state which specific spin properties can be efficiently used as a sensitive magnetic sensor. An external magnetic field induces Zeeman shifts of the NV…

Mesoscale and Nanoscale Physics · Physics 2015-07-17 M. Chipaux , A. Tallaire , J. Achard , S. Pezzagna , J. Meijer , V. Jacques , J. -F. Roch , T. Debuisschert

The negatively charged tin-vacancy (SnV-) center in diamond has emerged as a promising platform for quantum computing and quantum networks. To connect SnV- qubits in large networks, in-situ tuning and stabilization of their optical…

We introduce an advanced material system for the production and spectroscopy of single silicon vacancy (SiV) color centers in diamond. We use microwave plasma chemical vapor deposition to synthesize heteroepitaxial nanodiamonds of approx.…

Materials Science · Physics 2011-11-16 Elke Neu , Martin Fischer , Stefan Gsell , Matthias Schreck , Christoph Becher

The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

Using pulsed photoionization the coherent spin manipulation and echo formation of ensembles of NV- centers in diamond are detected electrically realizing contrasts of up to 17 %. The underlying spin-dependent ionization dynamics are…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Florian M. Hrubesch , Georg Braunbeck , Martin Stutzmann , Friedemann Reinhard , Martin S. Brandt

Although the spin properties of superficial shallow nitrogen-vacancy (NV) centers have been the subject of extensive scrutiny, considerably less attention has been devoted to studying the dynamics of NV charge conversion near the diamond…

Mesoscale and Nanoscale Physics · Physics 2018-07-03 Siddharth Dhomkar , Harishankar Jayakumar , Pablo R. Zangara , Carlos A. Meriles

The spatial resolution and fluorescence signal amplitude in stimulated emission depletion (STED) microscopy is limited by the photostability of available fluorophores. Here, we show that negatively-charged silicon vacancy (SiV) centers in…

Optics · Physics 2019-10-25 Yaser Silani , Forrest Hubert , Victor M. Acosta

In diamond, nitrogen defects like the substitutional nitrogen defect (Ns) or the nitrogen-vacancy-hydrogen complex (NVH) outnumber the nitrogen vacancy (NV) defect by at least one order of magnitude creating a dense spin bath. While neutral…

The NV$^-$ color center in diamond has been extensively investigated for quantum sensing, computation, and communication applications. Nonetheless, charge-state decay from the NV$^-$ to its neutral counterpart the NV$^0$ detrimentally…

Materials Science · Physics 2023-12-22 Rodrick Kuate Defo , Alejandro W. Rodriguez , Steven L. Richardson

We investigate spin and optical properties of individual nitrogen-vacancy centers located within 1-10 nm from the diamond surface. We observe stable defects with a characteristic optically detected magnetic resonance spectrum down to lowest…

Mesoscale and Nanoscale Physics · Physics 2012-08-27 B. K. Ofori-Okai , S. Pezzagna , K. Chang , M. Loretz , R. Schirhagl , Y. Tao , B. A. Moores , K. Groot-Berning , J. Meijer , C. L. Degen

Recent advancements in quantum technology have highlighted the potential of nitrogen-vacancy (NV) centers in diamond. However, fully realizing this potential requires addressing challenges related to the size, complexity, and cost of…

Nitrogen-vacancy (NV) centers in diamond are optically addressable spin defects with great potential for nanoscale quantum sensing. A key application of NV centers is the detection of external spins at the diamond surface. Among metals,…

The efficiency of collecting photons from optically active defect centres in bulk diamond is greatly reduced by refraction and reflection at the diamond-air interface. We report on the fabrication and measurement of a geometrical solution…

The negatively charged nitrogen-vacancy defect (NV)$^-$ in diamond has attracted much attention in recent years in qubit and biological applications. The negative charge is donated from nearby nitrogen donors that could limit or stem the…

Materials Science · Physics 2009-02-16 Adam Gali

Isolated, micro-meter sized diamonds are grown by micro-wave plasma chemical vapour deposition technique on Si(001) substrates. Each diamond is uniquely identified by markers milled in the Si substrate by Ga+ focused ion beam. The…

We study features in the optically detected magnetic resonance (ODMR) signals associated with negatively charged nitrogen-vacancy (NV) centers coupled to other paramagnetic impurities in diamond. Our results are important for understanding…

We demonstrate fully three-dimensional and patterned localization of nitrogen-vacancy (NV) centers in diamond with coherence times in excess of 1 ms. Nitrogen {\delta}-doping during CVD diamond growth vertically confines nitrogen to 4 nm…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Claire A. McLellan , Bryan A. Myers , Stephan Kraemer , Kenichi Ohno , David D. Awschalom , Ania C. Bleszynski Jayich