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Attosecond spectroscopy is currently restricted to photon energies around 100 eV. We show that under these conditions, electron-electron scatterings, as the photoelectrons leave the metal give rise to a tail of secondary electrons with…

Other Condensed Matter · Physics 2015-05-13 Jan Conrad Baggesen , Lars Bojer Madsen

A calculation of the high-harmonic generation (HHG) in $\alpha$-quartz using the time-dependent density functional theory is reported. The inter-band process is attributed to the dominant in HHG above the band gap. The photon energy is set…

Optics · Physics 2017-01-04 T. Otobe

We explore with ab-initio theory high harmonic generation (HHG) from a series of gas-phase fullerenes (from C$_{20}$ to C$_{60}$, including isomers) under varying laser conditions (different ellipticities, angular orientations, intensities…

Optics · Physics 2026-02-27 Km Akanksha Dubey , Ofer Neufeld

Non-perturbative high-harmonic generation (HHG) has recently been observed in the liquid phase, where it was demonstrated to have a different physical mechanism compared to gas and solid phases of matter. The currently best physical picture…

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics…

Atomic Physics · Physics 2009-11-13 P. Koval , F. Wilken , D. Bauer , C. H. Keitel

We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2025-04-23 A. A. Gunyaga , M. V. Durnev , S. A. Tarasenko

It is shown that electron backscattering can enhance high-harmonic generation in periodic systems with broken translational symmetry. Paradigmatically, we derive for a finite chain of atoms the harmonic cutoff due to electrons backscattered…

Atomic Physics · Physics 2022-04-13 Chuan Yu , Ulf Saalmann , Jan M. Rost

We demonstrated nonperturbative high harmonics induced by intense mid-infrared light up to 18th order that well exceed the material bandgap in monolayer transition metal dichalcogenides. The intensities of the even-order high-harmonic…

Mesoscale and Nanoscale Physics · Physics 2019-08-20 Naotaka Yoshikawa , Kohei Nagai , Kento Uchida , Yuhei Takaguchi , Shogo Sasaki , Yasumitsu Miyata , Koichiro Tanaka

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…

Atomic Physics · Physics 2017-11-29 Kenneth K. Hansen , Tobias Deffge , Dieter Bauer

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

Atomic Physics · Physics 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

We extend the semi-classical trajectory description for the high-order harmonic generation~(HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semi-classical trajectory model with a one-dimensional…

We analyzed the energy and momentum distributions of laser-induced high-energy photoelectrons of alkali and rare gas atoms. For the plateau electrons with energies above $4U_p$, ($U_p$ is the ponderomotive energy), in the tunneling…

Atomic Physics · Physics 2008-04-24 Zhangjin Chen , Anh-Thu Le , Toru Morishita , C. D. Lin

Considering C$_{60}$ as a model system for describing field emission from the extremity of a carbon nanotip, we explore electron emission from this fullerene excited by an intense, near-infrared, few-cycle laser pulse…

Atomic and Molecular Clusters · Physics 2016-03-23 Cong-Zhang Gao , Phuong Mai Dinh , Peter Kluepfel , Chris Meier , Paul-Gerhard Reinhard , Eric Suraud

Understanding how light interacts at the nanoscale with metals, semiconductors, or ordinary dielectrics is pivotal if one is to properly engineer nano-antennas, filters and, more generally, devices that aim to harness the effects of new…

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

In frequently studied two-band models for solid-state high-harmonic generation, interband harmonics in principle can range from the minimum to the maximum bandgap. However, it is known that a laser-intensity dependent cutoff exists that may…

Optics · Physics 2024-03-13 Lina Bielke , Hannah Jürß , Vincent Burgtorf , Dieter Bauer
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