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Revealing hidden non-radiative (dark) of resonant nanostructures using optical methods such as dark-field spectroscopy often becomes a sophisticated problem due to a weak coupling of these modes with a far-field radiation, whereas methods…

We introduce a novel method for creating a high-quality, sharply defined, non-diffracting optical bottle beam by focusing a Bessel beam propagating through a flat multi-level diffractive lens (MDL). This study highlights the impact of the…

Raman spectroscopy is a valuable characterization tool for two-dimensional materials. Starting from model Hamiltonians for Chern insulators and magnetized monolayers of transition metal dichalcogenides, we theoretically predict two…

Mesoscale and Nanoscale Physics · Physics 2025-01-29 Selçuk Parlak , Ion Garate

Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…

Chemical Physics · Physics 2015-05-13 X. G. Xu , S. O. Konorov , J. W. Hepburn , V. Milner

Raman microspectroscopy was used to characterize amorphous silica plastic behavior. Using a correlation between Raman spectrum and density, a map of the local residual indentation-induced densification is obtained. The existence of a…

We demonstrate dark-field x-ray microtomography in a compact, laboratory-based system capable of resolving attenuation, phase, and anisotropic scattering signals with micrometer-scale resolution across centimetre-scale samples. The method…

Nonlinear optical processes are used in biological microscopy to surpass the diffraction limit on resolution, image deeper into brain tissues, and identify biomolecules without exogenous labels. These techniques typically require high…

Efficient multilayer optics for radiation in the water window range are difficult to manufacture due to extremely small layer thicknesses and severe intermixing of elements between the layers. Therefore, adequate analytics and short…

We use vortex photon fields with orbital and spin angular momentum to probe chiral fluctuations within liquid crystals. In the regime of iridescence with a well-defined pitch length of chirality, we find low energy Raman scattering that can…

Soft Condensed Matter · Physics 2023-08-21 Silvia Müllner , Florian Büscher , Angela Möller , Peter Lemmens

Coherent Anti Stokes Raman Scattering (CARS) offers many advantages for nonlinear bio-imaging, thanks to its sub-cellular spatial resolution and unique chemical specificity. Its working principle requires two incident pulsed laser beams…

Peat, a crucial component in whisky production, imparts distinctive and irreplaceable flavours to the final product. However, the extraction of peat disrupts ancient ecosystems and releases significant amounts of carbon, contributing to…

Computer Vision and Pattern Recognition · Computer Science 2024-05-06 Yijun Yan , Jinchang Ren , Barry Harrison , Oliver Lewis , Yinhe Li , Ping Ma

The scattering of lattice excitations (phonons) with the photoexcited charge carriers is of a major concern in optoelectronic devices. Here, the resonant Raman scattering will be utilized to study an exciton-phonon interaction in GaN…

Near-field enhanced, nano-Raman spectroscopy has been successfully used to probe the surface chemistry of silicon prepared using standard wafer cleaning and processing techniques. The results demonstrate the utility of this measurement for…

Materials Science · Physics 2010-02-16 P. G. Spizzirri , J. -H. Fang , S. Rubanov , E. Gauja , S. Prawer

Raman spectroscopy in combination with machine learning has significant promise for applications in clinical settings as a rapid, sensitive, and label-free identification method. These approaches perform well in classifying data that…

Machine Learning · Computer Science 2021-11-12 Yaroslav Balytskyi , Justin Bendesky , Tristan Paul , Guy Hagen , Kelly McNear

We demonstrate state detection based on coherent Raman repumping and a two-color Raman state transfer. The Raman coupling during detection selectively eliminates unwanted dark states in the fluorescence cycle without compromising the…

Quantum Physics · Physics 2011-05-05 Boon Leng Chuah , Nick C. Lewty , Murray D. Barrett

Phonon modes found in low frequency Raman scattering from $CdS_{1-x}Se_x$ nanocrystals embedded in borosilicate glass arising from confined acoustic phonons are investigated. In addition to the breathing modes and quadrupolar modes, two…

Materials Science · Physics 2008-03-10 Sanjeev K. Gupta , Satyaprakash Sahoo , Prafulla K. Jha , A. K. Arora , Y. M. Azhniuk

Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…

Optics · Physics 2021-08-20 Hongli Ni , Peng Lin , Yifan Zhu , Meng Zhang , Yuying Tan , Yuewei Zhan , Ji-Xin Cheng

Images taken through window glass are often degraded by contaminants adhered to the glass surfaces. Such contaminants cause occlusions that attenuate the incoming light and scatter stray light towards the camera. Most of existing deep…

Computer Vision and Pattern Recognition · Computer Science 2025-09-03 Qiang Li , Yuanming Cao

Raman spectroscopy's capability to provide meaningful composition predictions is heavily reliant on a pre-processing step to remove insignificant spectral variation. This is crucial in biofluid analysis. Widespread adoption of diagnostics…

Signal Processing · Electrical Eng. & Systems 2019-04-05 Emily E Storey , Amr S. Helmy

The cerebrospinal fluid (CSF) of 19 subjects who received a clinical diagnosis of Alzheimer's disease (AD) as well as of 5 pathological controls have been collected and analysed by Raman spectroscopy (RS). We investigated whether the raw…