Related papers: Large optical nonlinearity enhancement under elect…
We investigate the resonant quantum dynamics of a laser-pumped real or artificial two-level single-atom system embedded in a leaking microcavity. We found that for stronger laser-atom-cavity couplings the generated microcavity photons…
We report on Kerr nonlinearity and dispersive optical bistability of a Fabry-Perot optical resonator due to the displacement of ultracold atoms trapped within. In the driven resonator, such collective motion is induced by optical forces…
Nonlinear imaging systems can surpass the limits of linear optics, but to date they have all relied on physical media (e.g. crystals) to work. These materials are all constrained by their physical properties, such as frequency selectivity,…
Strong optical nonlinearities at the few-photon level are a central goal for quantum photonics, yet they remain difficult to realize in solid-state systems. In doped two-dimensional semiconductors, coupling between excitons and a degenerate…
We demonstrate a cooperative optical non-linearity caused by dipolar interactions between Rydberg atoms in an ultra-cold atomic ensemble. By coupling a probe transition to the Rydberg state we map the strong dipole-dipole interactions…
There are a variety of nonlinear optical effects including higher harmonic generations, photovoltaic effects, and nonlinear Kerr rotations. They are realized by the strong light irradiation to materials that results in nonlinear…
The intimate interaction between phase-matched parametric amplification and strong nonlinear mode coupling in a multimode optical fiber results in a saturable spatial mode conversion that appears to violate the conservation of momentum. We…
We consider parametric interactions of laser pulses in a coherent macroscopic ensemble of resonant atoms, which are possible in the strong coupling regime of light-matter interaction. The spectrum condensation (lasing at collective vacuum…
Several years ago, it was shown that strong coupling between an electronic transition in organic molecules and a resonant photonic structure can modify the electronic landscape of the molecules and affect their chemical behavior. Since…
In this article, we show that the collective light-matter strong coupling regime, where $N$ molecular emitters couple to the photon mode of an optical cavity, can be mapped to a quantum impurity model where the photon is the impurity that…
We utilize the generation of large atomic coherence to enhance the resonant nonlinear magneto-optic effect by several orders of magnitude, thereby eliminating power broadening and improving the fundamental signal-to-noise ratio. A…
We propose a new method of resonant enhancement of optical Kerr nonlinearity using multi-level atomic coherence. The enhancement is accompanied by suppression of the other linear and nonlinear susceptibility terms of the medium. We show…
The nonlinear optical response of an excitonic insulator coupled to lattice degrees of freedom is shown to depend in strong and characteristic ways on whether the insulating behavior originates primarily from electron-electron or…
A coherent coupling among different energy photons provided by nonlinear optical interaction is regarded as a photonic version of the Rabi oscillation. Cavity enhancement of the nonlinearity reduces energy requirement significantly and…
Recent investigations on optical nonlinearities of plasmonic materials suggest their responses may be even beyond the usual perturbative description. To better understand these surprisingly strong responses, we develop here a simple but…
We predict theoretically and demonstrate experimentally an ellipticity-dependent nonlinear magneto-optic rotation of elliptically-polarized light propagating in a coherent atomic medium. We show that this effect results from a hexadecapole…
Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice systems. The magnitude of the THG at the 10 percent doping increases by the factor about 10^2 from that of the neutral…
We show that an ensemble of organic dye molecules with permanent electric dipole moments embedded in a microcavity can lead to strong optical nonlinearities at the single photon level. The strong long-range electrostatic interaction between…
Fabry-P\'erot (FP) cavities are fundamental and ubiquitous optical elements frequently used in various sensing applications. Here, we introduce a general theoretical framework to study arbitrary light-cavity mode interactions for planar FPs…
Realizing strong interactions between individual photons is a cornerstone for advancing photonic quantum computing and quantum nonlinear optics. Here, we experimentally demonstrate strong interactions between counter-propagating photons…