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We demonstrate two solid-state sources of indistinguishable single photons. High resolution laser spectroscopy and optical microscopy were combined at T = 1.4 K to identify individual molecules in two independent microscopes. The Stark…

Quantum Physics · Physics 2009-11-13 R. Lettow , V. Ahtee , R. Pfab , A. Renn , E. Ikonen , S. Gotzinger , V. Sandoghdar

Isolating single molecules in the solid state has allowed fundamental experiments in basic and applied sciences. When cooled down to liquid helium temperature, certain molecules show transition lines, that are tens of megahertz wide,…

The Stark effect provides a powerful method to shift the spectra of molecules, atoms and electronic transitions in general, becoming one of the simplest and most straightforward way to tune the frequency of quantum emitters by means of a…

We propose a novel method to control the frequency of semiconductor lasers. The new technique allows fabricating three-terminal lasers with fast frequency tuning and the possibility to implement intrinsically the linearization of laser…

Applied Physics · Physics 2025-01-07 B. Laikhtman , G. Belenky , S. Suchalkin

We report on the triggered generation of indistinguishable photons by solid-state single-photon sources in two separate cryogenic laser scanning microscopes. Organic fluorescent molecules were used as emitters and investigated by means of…

Quantum Physics · Physics 2009-11-13 V. Ahtee , R. Lettow , R. Pfab , A. Renn , E. Ikonen , S. Götzinger , V. Sandoghdar

An array of radiatively coupled emitters is an exciting new platform for generating, storing, and manipulating quantum light. However, the simultaneous positioning and tuning of multiple lifetime-limited emitters into resonance remains a…

Quantum Physics · Physics 2024-02-23 Christian Lange , Emma Daggett , Valentin Walther , Libai Huang , Jonathan D. Hood

We employ heterodyne interferometry to investigate the effect of a single organic molecule on the phase of a propagating laser beam. We report on the first phase-contrast images of individual molecules and demonstrate a single-molecule…

Quantum Physics · Physics 2015-05-27 M. Pototschnig , Y. Chassagneux , J. Hwang , G. Zumofen , A. Renn , V. Sandoghdar

We demonstrate by time-resolved resonance fluorescence measurements on a single self-assembled quantum dot an internal photo-effect that emits electrons from the dot by an intra-band excitation. We find a linear dependence of the optically…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Pia Lochner , Jens Kerski , Annika Kurzmann , Andreas D. Wieck , Arne Ludwig , Martin Geller , Axel Lorke

A semiconductor quantum dot mimics a two-level atom. Performance as a single photon source is limited by decoherence and dephasing of the optical transition. Even with high quality material at low temperature, the optical linewidths are a…

Mesoscale and Nanoscale Physics · Physics 2015-09-09 Andreas V. Kuhlmann , Jonathan H. Prechtel , Julien Houel , Arne Ludwig , Dirk Reuter , Andreas D. Wieck , Richard J. Warburton

Colloidal semiconductor quantum dots are robust emitters implemented in numerous prototype and commercial optoelectronic devices. However, active fluorescence color tuning, achieved so far by electric-field induced Stark effect, has been…

Mesoscale and Nanoscale Physics · Physics 2023-05-16 Yonatan Ossia , Adar Levi , Yossef E. Panfil , Somnath Koley , Einav Scharf , Nadav Chefetz , Sergei Remennik , Atzmon Vakahi , Uri Banin

Collective coherent scattering of laser light by an ensemble of polarizable point particles creates long range interactions, whose properties can be tailored by choice of injected laser powers, frequencies and polarizations. We use a…

Quantum Physics · Physics 2015-06-17 Stefan Ostermann , Matthias Sonnleitner , Helmut Ritsch

We demonstrate two-photon interference using two remote single molecules as bright solid-state sources of indistinguishable photons. By varying the transition frequency and spectral width of one molecule, we tune and explore the effect of…

Quantum Physics · Physics 2015-05-14 R. Lettow , Y. L. A. Rezus , A. Renn , G. Zumofen , E. Ikonen , S. Goetzinger , V. Sandoghdar

Using a master-equation approach for the description of coherent and incoherent dynamics in `artificial atoms and molecules', we present a theoretical analysis of situations where intense laser fields lead to pronounced renormalizations of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Ulrich Hohenester , Filippo Troiani , Elisa Molinari

We study single-photon ionization of aligned H$_2^+$ in a high-frequency low-intensity laser field. We focus on the case where the laser frequency is not far larger than the ionization potential of the target. The calculated photoelectron…

Atomic Physics · Physics 2022-12-02 F. B. Zhang , J. Y. Che , W. Y. Li , C. Chen , Y. J. Chen

Single semiconductor quantum dots have been widely studied within devices that can apply an electric field. In the most common system, the low energy offset between the InGaAs quantum dot and the surrounding GaAs material limits the…

Quantum Physics · Physics 2012-03-28 R. B. Patel , A. J. Bennett , I. Farrer , C. A. Nicoll , D. A. Ritchie , A. J. Shields

A mechanism is explored whereby intense laser radiation induces an optical force between the constituent atoms of a molecule. In the case of a diatomic molecule the effect results in a modification of the vibrational potential, and using…

Optics · Physics 2007-05-23 D. L. Andrews R. G. Crisp

Scalability and miniaturization are hallmarks of solid-state platforms for photonic quantum technologies. Still a main challenge is two-photon interference from distinct emitters on chip. This requires local tuning, integration and novel…

Quantum Physics · Physics 2022-01-19 R. Duquennoy , M. Colautti , R. Emadi , P. Majumder , P. Lombardi , C. Toninelli

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

We analyze a scheme to manipulate quantum states of neutral atoms at individual sites of optical lattices using focused laser beams. Spatial distributions of focused laser intensities induce position-dependent energy shifts of hyperfine…

Quantum Physics · Physics 2009-11-13 Chuanwei Zhang , S. L. Rolston , S. Das Sarma

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

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