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We present a simultaneous investigation of coherent spin dynamics in both localized and itinerant carriers in Fe/GaAs heterostructures using ultrafast and spin-resolved pump-probe spectroscopy. We find that for excitation densities that…

Mesoscale and Nanoscale Physics · Physics 2018-10-31 Yu-Sheng Ou , N. J. Harmon , Patrick Odenthal , R. K. Kawakami , M. E. Flatté , E. Johnston-Halperin

The use of advanced X-ray sources plays a key role in the study of dynamic processes in magnetically ordered materials. The progress in X-ray free electron lasers enables the direct and simultaneous observation of the femtosecond evolution…

Transition metals with their densely confined and strongly coupled valence electrons are key constituents of many materials with unconventional properties, such as high-Tc superconductors, Mott insulators and transition-metal…

Atomic Physics · Physics 2020-01-08 M. Volkov , S. A. Sato , F. Schlaepfer , L. Kasmi , N. Hartmann , M. Lucchini , L. Gallmann , A. Rubio , U. Keller

Quantum many-body systems driven far from equilibrium can exhibit chaos, entanglement, and non-classical correlations, yet directly observing these phenomena in large, closed quantum systems remains challenging. Here we realize the Dicke…

The interference of the directly emitted photoelectron wave and the wave scattered coherently by neighboring atoms gives holographic fringes in the photoelectron emission intensity $I(\hat{\bf R})$. In the electron emission holography…

Condensed Matter · Physics 2016-08-31 Eddy Timmermans , G. T. Trammell , J. P. Hannon

We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

We have recently proposed a mechanism of photon-axion oscillations as a way of rendering supernovae dimmer without cosmic acceleration. Subsequently, it has been argued that the intergalactic plasma may interfere adversely with this…

High Energy Physics - Phenomenology · Physics 2009-09-17 Csaba Csaki , Nemanja Kaloper , John Terning

The excitation of the spin degrees of freedom of an adsorbed atom by tunneling electrons is computed using a strong coupling theory. The excitation process is shown to be a sudden switch between the initial state determined by the…

Mesoscale and Nanoscale Physics · Physics 2009-04-29 Nicolás Lorente Jean-Pierre Gauyacq

The photoinduced switching of Fe(II)-based spin-crossover complexes from singlet to quintet takes place at ultrafast time scales. This a priori spin-forbidden transition triggered numerous time-resolved experiments of solvated samples to…

Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the…

Shape resonances in photoionization of atoms and molecules arise from a particular geometry of the ionic potential which traps the receding photoelectron in a quasi-bound state in a particular partial wave. This mechanism allows us to…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets , Stephen Catsamas

We present the extension of the time-dependent configuration interaction singles (TDCIS) method to the computation of the electron kinetic-energy spectrum in photoionization processes. Especially for strong and long ionizing light pulses…

Atomic Physics · Physics 2014-04-17 Antonia Karamatskou , Stefan Pabst , Yi-Jen Chen , Robin Santra

Measurements of the single photoionization cross section of Cu-like Zn$^+$ ions are reported in the energy (wavelength) range 17.5 eV (709 \AA) to 90 eV (138 \AA). The measurements on this {\it trans}-Fe element were performed at the…

We present coincidence measurements of two-photon double-ionization (TPDI) of argon driven by femtosecond pulses tunable around 26.5 eV photon energy, which are obtained from a high-harmonic generation source. The measured photoelectron…

The attosecond ultrafast ionization dynamics of correlated two- or many-electron systems have, so far, been mainly addressed investigating atomic systems. In the case of single ionization, it is well known that electron-electron correlation…

We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter…

Atomic Physics · Physics 2016-09-21 Martin Huppert , Inga Jordan , Denitsa Baykusheva , Aaron von Conta , Hans Jakob Wörner

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

We report the coherent coupling of two electron spins at a distance via virtual microwave photons. Each spin is trapped in a silicon double quantum dot at either end of a superconducting resonator, achieving spin-photon couplings up to…

Mesoscale and Nanoscale Physics · Physics 2022-05-13 Patrick Harvey-Collard , Jurgen Dijkema , Guoji Zheng , Amir Sammak , Giordano Scappucci , Lieven M. K. Vandersypen

Electron-boson coupling in unconventional superconductors is one of the key parameters in understanding the superconducting pairing symmetry. Here, we report definitive photoemission evidence of electron-spin exciton coupling in the…

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