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A high-throughput investigation of local epitaxy (called combinatorial substrate epitaxy) was carried out on Ca$_2$MnO$_4$ Ruddlesden-Popper thin films of six thicknesses (from 20 to 400 nm), all deposited on isostructural polycrystalline…

Materials Science · Physics 2015-07-29 M. Lacotte , A. David , G. S. Rohrer , P. A. Salvador , W. Prellier

We analyze the electronic structure of the recently synthesized higher-order nickelate Ruddlesden-Popper phases La$_{n+1}$Ni$_n$O$_{3n+1}$ ($n=4-6$) using first-principles calculations. For all materials, our results show large holelike…

Strongly Correlated Electrons · Physics 2022-03-08 Myung-Chul Jung , Jesse Kapeghian , Chase Hanson , Betül Pamuk , Antia S. Botana

Two-dimensional (2D) hybrid organic--inorganic perovskites (HOIPs) are promising candidates for next-generation optoelectronic and spintronic applications. This work systematically investigates the relationship between structural…

Materials Science · Physics 2026-04-10 Yue Zhao , Fu Li , Vikrant Chaudhary , Hongbin Zhang , Gaoyang Gou , Niuzhuang Yang , Yue Hao , Wenyi Liu

The temperature-dependent phase transitions in Ruddlesden-Popper oxides with perovskite bilayers have been under increased scrutiny in recent years due to the so-called hybrid improper ferroelectricity that some chemical compositions…

Materials Science · Physics 2021-12-08 Gabriel Clarke , Dominik Daisenberger , X. Luo , S. W. Cheong , Nicholas C. Bristowe , Mark S. Senn

The recent discovery of superconductivity in Ruddlesden-Popper bilayer nickelate, specifically La$_3$Ni$_2$O$_7$, has generated significant interest in the exploration of high-temperature superconductivity within this material family. In…

Superconductivity · Physics 2024-03-26 Haozhe Wang , Long Chen , Aya Rutherford , Haidong Zhou , Weiwei Xie

Compositionally complex solid solutions provide a unique route for engineering high-performance electrocatalysts, where the polyelemental surface composition can be seamlessly tuned to optimize activity, selectivity, and stability. However,…

The observation of low energy edge photoluminescence and its beneficial effect on the solar cell efficiency of Ruddlesden-Popper perovskites has unleashed an intensive research effort to reveal its origin. This effort, however, has been met…

The discovery of 80 K superconductivity in bilayer La$_3$Ni$_2$O$_7$ at pressures greater than 14 GPa presents a unique opportunity to study a novel class of high-temperature superconductors. Therefore, other bilayer nickelate following the…

Superconductivity · Physics 2024-06-19 Hasan Yilmaz , Kathrin Küster , Ulrich Starke , Oliver Clemens , Masahiko Isobe , Pascal Puphal

Ruddlesden-Popper nickelates offer a new route to high-temperature superconductivity beyond the cuprates and iron-pnictides. However, the electronic reorganization that enables superconductivity in bilayer nickelates remain unresolved,…

The realization of the stable structure of Heusler compounds and the study of different properties is an important step for their potential application in spintronics and magnetoelectronic devices. In this paper, using the plane-wave…

Using molecular dynamics simulation with an angle-dependent Lennard-Jones potential, we study orientational glass with quadrupolar symmetry in mixtures of elliptic particles and circular impurities in two dimensions. With a mild aspect…

Soft Condensed Matter · Physics 2015-07-24 Kyohei Takae , Akira Onuki

By high-throughput calculations based on the density functional theory, we construct a structure map for AB$_2$ type monolayers of 3844 compounds which are all the combinations of 62 elements selected from the periodic table. The structure…

Materials Science · Physics 2019-04-15 Masahiro Fukuda , Jingning Zhang , Yung-Ting Lee , Taisuke Ozaki

Van der Waals (vdW) materials provide a platform to study and control the physical properties of low-dimensional materials. While strategies developed for two-dimensional (2D) crystals are not directly transferable to one-dimensional (1D)…

Second magnetization peak (SMP) in hole-doped cuprates and iron pnictide superconductors has been widely explored. However, similar feature in the family of electron-doped cuprates is not common. Here, we report the vortex dynamics study in…

Superconductivity · Physics 2020-08-28 S. Salem-Sugui , P. V. Lopes , M. P. Kern , Shyam Sundar , Zhaoyu Liu , Shiliang Li , Huiqian Luo , L. Ghivelder

We present a theoretical study of classical Wigner crystals in two- and three-dimensional isotropic parabolic traps aiming at understanding and quantifying the configurational uncertainty due to the presence of multiple stable…

Plasma Physics · Physics 2012-04-27 Arūnas Radzvilavičius , Egidijus Anisimovas

We have discovered from first-principles an unusual polar state in the low n Sr$_{n+1}$Ti$_n$O$_{3n+1}$ Ruddlesden-Popper (RP) layered perovskites in which ferroelectricity is nearly degenerate with antiferroelectricity, a relatively rare…

Materials Science · Physics 2012-01-31 Turan Birol , Nicole A. Benedek , Craig J. Fennie

A chemical-free technique for fabricating submicron complex oxide structures has been developed based on selective epitaxial growth. The crystallinity and hence the conductivity of the complex oxide is inhibited by amorphous SrTiO3 (STO).…

Superconductivity · Physics 2007-05-23 P. Morales , M. DiCiano , J. Y. T. Wei

The discovery of high-temperature superconductivity in La3Ni2O7 and La4Ni3O10 under high pressure indicates that the Ruddlesden-Popper (RP) phase nickelates Rn+1NinO3n+1 (R = rare earth) is a new material family for high-temperature…

The field of high entropy oxides (HEOs) flips traditional materials science paradigms on their head by seeking to understand what properties arise in the presence of profound configurational disorder. This disorder, which originates from…

Materials Science · Physics 2024-10-30 Solveig S. Aamlid , Mohamed Oudah , Jörg Rottler , Alannah M. Hallas

The rare-earth nickelates possess a diverse set of collective phenomena including metal-to-insulator transitions, magnetic phase transitions, and, upon chemical reduction, superconductivity. Here, we demonstrate epitaxial stabilization of…

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