Related papers: Plasmonic Purcell Effect in Organic Molecules
We develop a theory for spontaneous decay of a quantum emitter (QE) situated near metal-dielectric structure supporting localized surface plasmons. If plasmon resonance is tuned close to the QE emission frequency, the emission is enhanced…
The optical properties of molecules close to plasmonic nanostructures greatly differ from their isolated molecule counterparts. To theoretically investigate such systems in a Quantum Chemistry perspective, one has to take into account that…
Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced…
We extend the model of exciton-plasmon materials to include a ro-vibrational structure of molecules using wave-packet propagations on electronic potential energy surfaces. The new model replaces conventional two-level emitters with more…
We review the studies of a wide range of optical phenomena resulting from near-field coupling between excitons and localized surface plasmon-polaritons in hybrid nanostructures. Modern physical approaches and theoretical models reported…
Controlling the light emitted by individual molecules is instrumental to a number of novel nanotechnologies ranging from super-resolution bio-imaging and molecular sensing to quantum nanophotonics. Molecular emission can be tailored by…
The Purcell effect describes the enhancement of the spontaneous emission rate of an emitter near a resonant structure. However, evaluating the Purcell factor quantitatively and empirically is difficult due to the difficulties in measuring…
Recent experiments have shown that highly efficient energy transfer can take place in organic nanocrystals at extremely low acceptor densities. This striking phenomenon has been ascribed to the formation of exciton polaritons thanks to the…
Plasmonic nanopatch antennas that incorporate dielectric gaps hundreds of picometers to several nanometers thick have drawn increasing attention over the past decade because they confine electromagnetic fields to grossly sub-diffraction…
The microscopic processes underlying electro-optic sampling of quantum-vacuum fluctuations are discussed, leading to the interpretation of these experiments in terms of an exchange of virtual photons. With this in mind it is shown how one…
We investigate the spontaneous emission rate of a two-level quantum emitter next to a composite medium made of randomly distributed metallic inclusions embedded in a dielectric host matrix. In the near-field, the Purcell factor can be…
We study numerically the effect of mode mixing and direct dipole-dipole interactions between gain molecules on spasing in a small composite nanoparticles with a metallic core and a dye-doped dielectric shell. By combining Maxwell-Bloch…
We model a dye-doped polymeric nanosphere as an ensemble of quantum emitters and use it to investigate the localized exciton-polaritons supported by such a nanosphere. By determining the time evolution of the density matrix of the…
Spontaneous emission of quantum emitters can be modified by engineering their optical environment. This allows a resonant nanoantenna to significantly modify the radiative properties of a quantum emitter. In this article, we go beyond the…
Nanoscale semiconductor lasers have been developed recently using either metal, metallo-dielectric or photonic crystal nanocavities. While the technology of nanolasers is steadily being deployed, their expected performance for on-chip…
The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely…
Based on the reciprocity theorem, we present a formalism to calculate the power emitted by a dipole source into a particular propagating mode leaving an open optical system. The open system is completely arbitrary and the approach can be…
The Purcell effect is defined as the modification of spontaneous decay in the presence of a resonator, and in plasmonics it is usually associated with the large local-field enhancement in "hot spots" due to surface plasmon polaritons. Here…
An emitter in the vicinity of a metal nanostructure is quenched by its decay through non-radiative channels, leading to the belief in a zone of inactivity for emitters placed within $<$10nm of a plasmonic nanostructure. Here we demonstrate…
Engineering the local density of states with nanophotonic structures is a powerful tool to control light-matter interactions via the Purcell effect. At optical frequencies, control over the electric field density of states is typically used…