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The organic terahertz (THz) generation crystal BNA has recently gained traction as a valuable source to produce broadband THz pulses. Even when pumped with 800-nm light, thin BNA crystals can produce relatively high electric fields with…

We are reporting on terahertz generation from organic crystal BNA using a 1.15 to 1.55 um near infrared pump. We observed a very large emission spectrum extending up to 7 THz, compared to 2.5 THz from Ti:Sa pump in previous reports. The…

Materials Science · Physics 2019-07-24 Hang Zhao , Yong Tan , Tong Wu , Gunther Steinfeld , Yan Zhang , Cunlin Zhang , Liangliang Zhang , Mostafa Shalaby

The generation of tunable narrowband pulses is increasingly being pursued in terahertz science, for example to study the nonlinear response of individual modes of solids and molecules. Here, we extend the chirp-and-delay method to achieve…

Optics · Physics 2025-10-28 D. Pavicevic , M. Nishida , J. Song , M. Buzzi , A. Cavalleri

We report on high energy terahertz pulses by optical rectification (OR) in the organic crystal N-benzyl-2-methyl-4-nitroaniline (BNA) directly pumped by a conventional Ti:Sapphire (Ti:Sa) amplifier. The simple scheme provides an optical to…

We demonstrate a 13.3 MHz repetition rate, broadband THz source with milliwatt-average power, obtained by collinear optical rectification of a high-power Yb-doped thin-disk laser in the organic crystal BNA…

We demonstrate efficient optical rectification in the organic crystal BNA (N-benzyl-2-methyl-4-nitroaniline), driven by a temporally compressed, commercially available industrial Yb-laser system operating at 540 kHz repetition rate. Our THz…

In this work, we demonstrate BNAs high potential for efficient generation of high power THz using ytterbium laser wavelengths. We study the generation theoretically and experimentally using laser wavelength of 960-1150 nm. Broadband pulses…

Optics · Physics 2021-09-10 Hovan Lee , Claudia Gollner , Jiaqi Nie , Yan Zhang , Cedric Weber , Mostafa Shalaby

Increasing the average power of broadband, few-cycle terahertz (THz) sources is currently a topic of intense investigation, fueled by recent immense progress in high average power femtosecond laser driving sources at 1030 nm. However, many…

We report the full characterization of a new organic nonlinear optical (NLO) crystal for intense THz generation: PNPA ((E)-4-((4-nitrobenzylidene)amino)-N-phenylaniline). We discuss crystal growth and structural characteristics. We present…

Organic nonlinear optical (NLO) crystals have emerged as efficient room-temperature emitters of broadband THz radiation with high electric field strengths. Although initially confined to high-pulse-energy excitation in the millijoule range…

Optics · Physics 2024-08-07 Lukasz A. Sterczewski , Jakub Mnich , Jaroslaw Sotor

We present a high power and broadband THz-TDS setup utilizing the nonlinear organic crystal MNA both as emitter and detector. The THz source is based on optical rectification of near infra-red laser pulses at a central wavelength of 1036 nm…

We present a terahertz time-domain spectroscopy (THz-TDS) system which accesses a broadband spectrum, efficiently covering the so-called "new THz gap" between 5 and 15 THz and extending beyond 25 THz. The system exploits nonlinear…

The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses…

Optics · Physics 2023-03-08 Yuxuan Wei , Jiaming Le , Chuanshan Tian

The terahertz spectral regime, ranging from about 0.1 to 15 THz, is one of the least explored yet most technologically transformative spectral regions. One current challenge is to develop efficient and compact terahertz emitters/detectors…

Mesoscale and Nanoscale Physics · Physics 2019-03-12 Liang Luo , Ioannis Chatzakis , Jigang Wang , Fabian B. P. Niesler , Martin Wegener , Thomas Koschny , Costas M. Soukoulis

We report on extensive experimental investigation of novel barium chalcogenides (BaGa4Se7, BaGa2GeSe6 and BaGa2GeS6) for generation of a strong narrowband terahertz (THz) radiation. The Ba-containing compounds demonstrate the large bandgap…

Optics · Physics 2026-03-03 D. Z. Suleimanova , E. A. Migal , D. V. Badikov , F. V. Potemkin

Sensitive detection of terahertz (THz) radiation is fundamental to progress in spectroscopy, advanced wireless communication, and the realization of emerging quantum technologies. However, the intrinsically low photon energies in the THz…

As high-average power ultrafast lasers become increasingly available for nonlinear conversion, the temperature dependence of the material properties of nonlinear crystals becomes increasingly relevant. Here, we present temperature-dependent…

Optics · Physics 2023-08-29 Samira Mansourzadeh , Tim Vogel , Mostafa Shalaby , Clara J. Saraceno

Terahertz (THz) radiation is a powerful probe of low-energy excitations in all phases of matter. However, it remains a challenge to find materials that efficiently generate THz radiation in a broad range of frequencies following optical…

We demonstrate high-energy terahertz generation from a large-aperture (75 mm diameter) lithium niobate wafer by using a femtosecond laser with energy up to 2 J. This scheme utilizes optical rectification in a bulk lithium niobate crystal,…

Optics · Physics 2020-01-08 Dogeun Jang , Chul Kang , Seong Ku Lee , Jae Hee Sung , Chul-sik Kee , Ki-yong Kim

Using a canonical pump-probe experimental technique, we studied the terahertz (THz) waves generation and detection via optical rectification and mixing in Czochralski-grown periodically poled Mg:Y:LiNbO3 (PPLN) crystals. THz waves with…

Optics · Physics 2009-11-11 G. H. Ma , G. Kh. Kitaeva , I. I. Naumova , S. H. Tang
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