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The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…

The mid-infrared spectral range (2 to 20 \mu m) is of particular importance for chemistry, biology and physics as many molecules exhibit strong ro-vibrational fingerprints. Frequency combs - broad spectral bandwidth coherent light sources…

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

Optical frequency combs have emerged as a cornerstone for a wide range of areas, including spectroscopy, ranging, optical clocks, time and frequency transfer, waveform synthesis, and communications. However, quantum mechanical fluctuations…

Quantum Physics · Physics 2024-12-30 Abdulkarim Hariri , Shuai Liu , Haowei Shi , Quntao Zhuang , Xudong Fan , Zheshen Zhang

A train of periodic optical pulses gives an optical frequency "comb" that acts as a precise ruler for light measurement due to its equally spaced frequencies. Today, such pulses last millionths of a billionth of a second (Femtoseconds/fs)…

Optics · Physics 2026-05-22 Tushar Malica

Dual comb spectroscopy (DCS) is a powerful technique for broadband spectroscopy with high precision and fast data acquisition. High-frequency resolution requires long data acquisition times, limiting the temporal resolution in time-resolved…

Optics · Physics 2022-12-06 Sutapa Ghosh , Gadi Eisenstein

The method of Doppler - free comb - spectroscopy for dipole transitions was proposed. The calculations for susceptibility spectrum for moving two-level atoms driving by strong counter propagating combs have been done. The used theoretical…

Optics · Physics 2014-03-07 S. A. Pulkin , A. Kalinichev , V. Arnautov , S. V. Uvarova , S. Savel'eva

We report a high-energy, bidirectional, dissipative soliton mode-locked fiber laser operating in the 1550 nm normal-dispersion regime. By leveraging intracavity dispersion management and a Lyot filtering mechanism, the laser achieves…

Optics · Physics 2026-02-17 Mingjun Wang , Zhangru Shi , Anshuang Wang , Bowen Li

We demonstrate coherent dual frequency-comb spectroscopy for detecting variations in greenhouse gases. High signal-to-noise spectra are acquired spanning 5990 to 6260 cm^-1 (1600 to 1670 nm) covering ~700 absorption features from CO2, CH4,…

To meet the challenges of high-resolution molecular spectroscopy, increasingly sophisticated spectroscopic techniques were developed. For a long time FTIR and laser-based spectroscopies were used for these studies. The recent development of…

We explore the advantages of a free-form dual-comb spectroscopy (DCS) platform based on time-programmable frequency combs for real-time, penalty-free apodized scanning. In traditional DCS, the fundamental spectral resolution, which equals…

Molecular spectroscopy in the mid-infrared portion of the electromagnetic spectrum (3--25 um) has been a cornerstone interdisciplinary analytical technique widely adapted across the biological, chemical, and physical sciences. Applications…

Instrumentation and Detectors · Physics 2018-09-18 Abijith S. Kowligy , Henry Timmers , Alex Lind , Ugaitz Elu , Flavio C. Cruz , Peter G. Schunemann , Jens Biegert , Scott A. Diddams

The noise of a device under test (DUT) is measured simultaneously with two instruments, each of which contributes its own background. The average cross power spectral density converges to the DUT power spectral density. This method enables…

Instrumentation and Detectors · Physics 2010-03-02 Enrico Rubiola , Francois Vernotte

On-chip spectroscopy that could realize real-time fingerprinting with label-free and high-throughput detection of trace molecules is one of the 'holy grails" of sensing. Such miniaturized spectrometers would greatly enable applications in…

Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

Laser dynamics underpin a broad range of modern photonic technologies and continue to reveal rich nonlinear behaviors. However, existing spectroscopic tools, most notably time-stretched dispersive Fourier transform spectroscopy (TS-DFT),…

Photodetector nonlinearity, the main limiting factor in terms of optical power in the detection chain, is corrected to improve the signal-to-noise ratio of a short-time measurement in dual-comb spectroscopy. An iterative correction…

Instrumentation and Detectors · Physics 2021-09-08 Philippe Guay , Nicolas Bourbeau Hébert , Alex Tourigny-Plante , Vincent Michaud-Belleau , Jérôme Genest

Broadband, high resolution and rapid measurement of dual-comb spectroscopy (DCS) generates a large amount of data stream. We numerically demonstrate significant data compression of DCS spectra by using a compressive sensing technique. Our…

Signal Processing · Electrical Eng. & Systems 2025-05-06 Akira Kawai , Takahiro Kageyama , Ryoichi Horisaki , Takuro Ideguchi

While being invented for precision measurement of single atomic transitions, frequency combs have also become a versatile tool for broadband spectroscopy in the last years. In this paper we present a novel and simple approach for broadband…

For the first time to our knowledge, a dual-comb laser based on thin-disk technology and its application to direct frequency comb spectroscopy are presented. The peak power (0.6 MW) and the average power (12 W) of our Yb:YAG thin-disk…

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