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Related papers: Coupling and Decoupling of Polaritonic States in M…

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Polaritonic chemistry offers the possibility of modifying molecular properties and even influencing chemical reactivity through strong coupling between vibrational transitions and confined light modes in optical cavities. Despite…

Chemical Physics · Physics 2025-05-16 Thomas Schnappinger , Markus Kowalewski

We demonstrate that collective vibrational strong coupling of molecules in thermal equilibrium can give rise to significant local electronic polarizations in the thermodynamic limit. We do so by first showing that the full non-relativistic…

Cavity quantum electrodynamics has been studied as a potential approach to modify free charge carrier generation in donor-acceptor heterojunctions because of the delocalization and controllable energy level properties of hybridized…

Chemical Physics · Physics 2022-11-02 Weijun Wu , Andrew E. Sifain , Courtney A. Delpo , Gregory D. Scholes

Polaritonic chemistry exploits strong light-matter coupling between molecules and confined electromagnetic field modes to enable new chemical reactivities. In systems displaying this functionality, the choice of the cavity determines both…

Optics · Physics 2022-08-25 Jacopo Fregoni , Francisco J. García-Vidal , Johannes Feist

In a circuit quantum eletrodynamic system, a chain of N qubits inhomogeneously coupled to a cavity field forms a mesoscopic quasi-lattice, which is characterized by its degree of deformation from a normal lattice. This deformation is a…

Quantum Physics · Physics 2014-04-23 Hou Ian , Yu-xi Liu

I investigate the tunneling decay rate of a polaritonic system formed by a strong coupling between a vacuum cavity mode and $N$ metastable systems. Using a simple model potential, I find the instanton solutions controlling the…

Quantum Physics · Physics 2023-01-25 Kalle S. U. Kansanen

The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…

Materials Science · Physics 2020-10-09 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir

Quantum control of a system requires the manipulation of quantum states faster than any decoherence rate. For mesoscopic systems, this has so far only been reached by few cryogenic systems. An important milestone towards quantum control is…

Quantum Physics · Physics 2021-02-01 Andrés de los Ríos Sommer , Nadine Meyer , Romain Quidant

Motivated by the dramatic success of realizing cavity exciton-polariton condensation in experiment we consider the formation of polaritons from cavity photons and the amplitude or Higgs mode of a superconductor. Enabled by the recently…

Superconductivity · Physics 2020-02-19 Zachary M. Raines , Andrew A. Allocca , Mohammad Hafezi , Victor M. Galitski

The features of superfluid-Mott insulator phase transition in the array of dissipative nonlinear cavities are analyzed. We show analytically that the coupling to the bath can be reduced to renormalizing the eigenmodes of atom-cavity system.…

Quantum Physics · Physics 2014-12-16 Ke Liu , Lei Tan , C. -H Lv , W. M. Liu

Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Maxime Dherbécourt , Joël Bellessa , Clémentine Symonds , Guillaume Weick , David Hagenmüller

Molecular strong coupling offers exciting prospects in physics, chemistry and materials science. Whilst attention has been focused on developing realistic models for the molecular systems, the important role played by the entire photonic…

Band engineering stands as an efficient route to induce strongly correlated quantum many-body phenomena. Besides inspiring analogies among diverse physical fields, tuning on demand the group velocity is highly attractive in photonics…

Cavity exciton--polaritons are quasiparticles that form when quantum well excitons hybridize with a cavity mode. Here, we carry out photon correlation measurements under continuous wave resonant laser excitation to demonstrate quantum…

Inspired by the recent experimental observation of strongly coupled polaritons in a Moir\'e heterobilayer, we study a model of dipole-interacting excitons localized on sites of a lattice and coupled to planar cavity photons. We calculate…

Strongly Correlated Electrons · Physics 2022-03-25 Alexander Edelman , Peter B. Littlewood

In most theoretical descriptions of collective strong coupling of organic molecules to a cavity mode, the molecules are modeled as simple two-level systems. This picture fails to describe the rich structure provided by their internal…

Quantum Physics · Physics 2015-11-11 Javier Galego , Francisco J. Garcia-Vidal , Johannes Feist

A remote energy transfer pathway from electronic to vibrational degrees of freedom is identified inside an infrared optical cavity under vibrational strong coupling conditions. This mechanism relies on the dynamical Casimir effect, whereby…

Quantum Physics · Physics 2024-03-19 Tao E. Li

Collective strong coupling of molecular ensembles to optical cavities opens a route to modifying matter through genuinely collective electronic correlations. Yet even in the absence of a cavity, Coulomb correlations are notoriously…

Quantum Physics · Physics 2026-05-05 Dominik Sidler , Michael Ruggenthaler , Angel Rubio

When molecular transitions strongly couple to photon modes, they form hybrid light-matter modes called polaritons. Collective vibrational strong coupling is a promising avenue for control of chemistry, but this can be deterred by the large…

We study an atom-cavity system in which the cavity has several degenerate transverse modes. Mode-resolved cavity transmission spectroscopy reveals well-resolved atom-cavity resonances for several cavity modes, a signature of collective…

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