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The surface free energy, or surface tension, of a liquid interface gives rise to a pressure jump when the interface is curved. Here we show that a similar capillary pressure arises at the interface of soft solids. We present experimental…

Fluid Dynamics · Physics 2015-06-03 Antonin Marchand , Siddhartha Das , Jacco H. Snoeijer , Bruno Andreotti

We have developed a simulation model to describe particle adsorption to and desorption from liquid interfaces. Using this model we formulate a closed interfacial equation of state for repulsive elastic spheres. The effect of a long-range…

Soft Condensed Matter · Physics 2011-02-24 Robert D. Groot , Simeon D. Stoyanov

We study, using Monte Carlo simulations, the interaction between charged colloidal particles confined to the air-water interface. The dependence of force on ionic strength and counterion valence is explored. For 1:1 electrolyte, we find…

Soft Condensed Matter · Physics 2018-02-05 Matheus Girotto , Alexandre P. dos Santos , Yan Levin

Using fluorescence microscopy we study the adsorption of single latex microparticles at a water/water interface between demixing aqueous solutions of polymers, generally known as a water-in-water emulsion. Similar microparticles at the…

Soft Condensed Matter · Physics 2018-05-23 Louis Keal , Carlos E. Colosqui , Hans Tromp , Cecile Monteux

Within a general theoretical framework we study the effective, deformation-induced interaction between two colloidal particles trapped at a fluid interface in the regime of small deformations. In many studies, this interaction has been…

Soft Condensed Matter · Physics 2010-06-18 Alvaro Dominguez , Martin Oettel , Siegfried Dietrich

Soft particles at fluid interfaces play an important role in many aspects of our daily life, such as the food industry, paints and coatings, and medical applications. Analytical methods are not capable of describing the emergent effects of…

Computational Physics · Physics 2019-09-25 Maarten Wouters , Othmane Aouane , Timm Krueger , Jens Harting

Although the dynamics of colloids in the vicinity of a solid interface has been widely characterized in the past, experimental studies of Brownian diffusion close to an air-water interface are rare and limited to particle-interface gap…

Soft Condensed Matter · Physics 2022-11-11 Stefano Villa , Christophe Blanc , Abdallah Daddi-Moussa-Ider , Antonio Stocco , Maurizio Nobili

We investigate excluded-volume effects in a bidisperse colloidal suspension near a flexible interface. Inspired by a recent experiment by Dinsmore et al. (Phys. Rev, Lett. 80, 409 (1998)), we study the adsorption of a mesoscopic bead on the…

Soft Condensed Matter · Physics 2009-11-10 Thomas Bickel

The influence of the external pressure and surface energy on the wetting transition at nanotextured interfaces is studied using molecular dynamics and continuum simulations. The surface roughness of the composite interface is introduced via…

Soft Condensed Matter · Physics 2018-07-12 Bishal Bhattarai , Nikolai V. Priezjev

Thermocapillary convection is particularly effective for the control of thin liquid film topography or for the actuation of microparticles at the liquid-air interface. Experiments with water are challenging, however, as its interface is…

Soft Condensed Matter · Physics 2024-11-25 Thomas Bickel

In biomimetic and biological systems, interactions between surfaces are often mediated by adhesive molecules, nanoparticles, or colloids dispersed in the surrounding solution. We present here a general, statistical-mechanical model for two…

Soft Condensed Matter · Physics 2009-11-13 Bartosz Rozycki , Reinhard Lipowsky , Thomas R. Weikl

The idea of working with a near-critical phase-separated liquid mixture whereby the surface tension becomes weak, has recently made the field of laser manipulation of liquid interfaces a much more convenient tool in practice. The…

Optics · Physics 2009-11-10 Aslak Hallanger , Iver Brevik , Skjalg Haaland , Roger Sollie

We use confocal microscopy to study an equilibrated crystal-liquid interface in a colloidal suspension. Capillary waves roughen the surface, but locally the intrinsic interface is sharply defined. We use local measurements of the structure…

Soft Condensed Matter · Physics 2009-09-28 Jessica Hernández-Guzmán , Eric R. Weeks

The efficiency of soft particles to stabilize emulsions is examined by measuring their desorption free energy, i.e., the mechanical work required to detach the particle from a fluid interface. Here, we consider rubber-like elastic as well…

Soft Condensed Matter · Physics 2020-08-20 Hadi Mehrabian , Jacco H. Snoeijer , Jens Harting

Several model fluids in contact with planar, spherical, and cylindrical walls are investigated for small number densities within density functional theory. The dependence of the solid-fluid interfacial tension on the curvature of spherical…

Statistical Mechanics · Physics 2015-05-05 Andreas Reindl , Markus Bier , S. Dietrich

Hypothesis: The collective dynamics and self-assembly of colloids floating at a fluid/fluid interface is a balance between deterministic lateral interaction forces, viscous resistance to colloid motion along the surface and thermal…

Soft Condensed Matter · Physics 2022-10-05 Archit Dani , Mohsen Yeganeh , Charles Maldarelli

Solid interfaces have intrinsic elasticity. However, in most experiments, this is obscured by bulk stresses. Through microscopic observations of the contact-line geometry of a partially wetting droplet on an anisotropically stretched…

Soft Condensed Matter · Physics 2017-11-29 Qin Xu , Robert W. Style , Eric R. Dufresne

The dynamics of colloid-size particles trapped at a liquid interface is an extensively studied problem owing to its relevance to a wide range of engineering applications. Here we investigate the impact of interfacial deformations on the…

Soft Condensed Matter · Physics 2024-10-15 Zhi Zhou , Petia M. Vlahovska , Michael J. Miksis

The effects of contact-line pinning are well-known in macroscopic systems, but are only just beginning to be explored at the microscale in colloidal suspensions. We use digital holography to capture the fast three-dimensional dynamics of…

Soft Condensed Matter · Physics 2017-09-13 Anna Wang , W. Benjamin Rogers , Vinothan N. Manoharan

Measurements of the surface diffusivity of colloidal spheres translating along a vapor/liquid inter- face show an unexpected decrease in diffusivity, or increase in surface drag (from the Stokes-Einstein relation) when the particles situate…

Soft Condensed Matter · Physics 2016-07-08 Joel Koplik , Charles Maldarelli