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Related papers: Multiorbital processes rule the Nd$_{1-x}$Sr$_x$Ni…

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Using density functional based LDA+U method and linear-response theory, we study the magnetic exchange interactions of the superconductor Nd{1-x}Sr{x}NiO2. Our calculated nearest-neighbor exchange constant J1=82 meV is large, weakly…

Strongly Correlated Electrons · Physics 2021-02-17 Xiangang Wan , Vsevolod Ivanov , Giacomo Resta , Ivan Leonov , Sergey Y. Savrasov

Understanding the electronic behavior of Ni$^{2+}$ in a square planar environment of oxygen is the key to unravel the origin of the recently discovered superconductivity in the hole doped nickelate Nd$_{0.8}$Sr$_{0.2}$NiO$_2$. To identify…

The search for oxide materials with physical properties similar to the cuprate high Tc superconductors, but based on alternative transition metals such as nickel, has grown and evolved over time. The recent discovery of superconductivity in…

Employing combination of first-principles calculations, low-energy model construction, and variational Monte Carlo solution of the ab-initio derived Hubbard model, we study the effect of hydrogenation in the electronic structure and…

Superconductivity · Physics 2025-06-17 Manoj Gupta , Arun Kumar Maurya , Amal Medhi , Tanusri Saha Dasgupta

High-T$_c$ superconductivity has recently been discovered in Ruddlesden-Popper phase nickelates under pressure, where the low-energy electronic structure is dominated by Ni $d_{x^2 - y^2}$ and $d_{z^2}$ orbitals. However, the respective…

We study magnetism in the electron-doped infinite-layer nickelate NdNiO$_2$. We perform an unrestricted Hartree-Fock calculation for a tight-binding model which contains both nickel and neodymium orbitals. We reproduce the self-doping…

Strongly Correlated Electrons · Physics 2025-09-25 Adam Kłosiński , Roman Drachynskyi , Krzysztof Wohlfeld , Wojciech Brzezicki

The discovery that Nd$_{1-x}$Sr$_x$NiO$_2$, with the CaCuO$_2$ infinite-layer structure, superconducts up to 15 K around the hole-doping level $x$=0.2 raises the crucial question of its fundamental electronic and magnetic processes. The…

Superconductivity · Physics 2020-09-22 Mi-Young Choi , W. E. Pickett , K. -W. Lee

The discovery of superconductivity in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ [1] introduced a new family of layered nickelate superconductors that has now been extended to include a range of Sr-doping [2, 3], Pr or La in place of Nd [4-6], and the…

We report a determinant quantum Monte Carlo study of a two-band model, inspired by infinite-layer nickelates, focusing on the influence of interlayer hybridization between $3d_{x^2-y^2}$ orbitals derived from Ni (or Ni and O) in one layer…

Strongly Correlated Electrons · Physics 2024-06-10 Fangze Liu , Cheng Peng , Edwin W. Huang , Brian Moritz , Chunjing Jia , Thomas P. Devereaux

After the significant discovery of the hole-doped nickelate compound Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, an analysis of the electronic structure, orbital components, Fermi surfaces and band topology could be helpful to understand the mechanism of…

Materials Science · Physics 2021-03-18 Jiacheng Gao , Zhijun Wang , Chen Fang , Hongming Weng

The fundamental properties of infinite-layer rare-earth nickelates (RNiO2) are carefully revisited and compared with those of CaCuO2 and RNiO3 perovskites. Combining first-principles and finite-temperature second-principles calculations, we…

Materials Science · Physics 2022-01-04 Yajun Zhang , Jingtong Zhang , Xu He , Jie Wang , Philippe Ghosez

The recent discovery of superconductivity in Sr-doped NdNiO$_2$, with a critical temperature of $10-15$ K suggests the possibility of a new family of nickel-based high-temperature superconductors (HTS). NdNiO$_{2}$ is the $n=\infty$ member…

Strongly Correlated Electrons · Physics 2021-09-15 Harrison LaBollita , Antia S. Botana

Motivated by the recently reported signatures of superconductivity in trilayer La$_4$Ni$_3$O$_{10}$ under pressure, we comprehensively study this system using {\it ab initio} and random-phase approximation techniques. Without electronic…

Superconductivity · Physics 2024-09-24 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

In this work, we investigate collective electronic fluctuations and, in particular, the possibility of the charge density wave ordering in an infinite-layer NdNiO$_2$. We perform advanced many-body calculations for the ab-initio…

Strongly Correlated Electrons · Physics 2024-06-03 Evgeny A. Stepanov , Matteo Vandelli , Alexander I. Lichtenstein , Frank Lechermann

The discovery of superconductivity in infinite-layer nickelates has added a new family of materials to the fascinating growing class of unconventional superconductors. By incorporating the strongly correlated multi-orbital nature of the…

Superconductivity · Physics 2022-08-15 Andreas Kreisel , Brian M. Andersen , Astrid T. Rømer , Ilya M. Eremin , Frank Lechermann

We present a comparative density-functional theory plus dynamical mean-field theory (DFT+DMFT) study of the two known superconducting members of the rare-earth (R) layered nickelate family: hole-doped RNiO$_{2}$ ($n=\infty$) and…

Strongly Correlated Electrons · Physics 2022-03-01 Harrison LaBollita , Antia S. Botana

The discovery of superconductivity in hole-doped infinite layer nickelates, RNiO2 (R = Nd, Pr, La) has garnered sustained interest in the field. A definitive picture of low-energy many-body states has not yet emerged. We provide new…

Strongly Correlated Electrons · Physics 2023-03-28 Gheorghe Lucian Pascut , Lucian Cosovanu , Kristjan Haule , Khandker F. Quader

The recent observation of superconductivity in thin film infinite-layer nickelates$^{1-3}$ offers a different angle to investigate superconductivity in layered oxides$^{4}$. A wide range of candidate models have been proposed$^{5-10}$,…

We perform a comparative $2 \times 2$ real space cluster DMFT study on minimal models for NdNiO$_2$ and CaCuO$_2$ obtained from downfolding DFT states, using a Nambu formalism that allows for both superconducting and antiferromagnetic…

Strongly Correlated Electrons · Physics 2022-06-01 Jonathan Karp , Alexander Hampel , Andrew J. Millis

The minimal model for infinite-layer nickelates remains under debate, particularly regarding the hybridization between itinerant interstitial-$s$ and the correlated Ni-3$d_{x^2-y^2}$ orbitals, as well as the interaction between…

Strongly Correlated Electrons · Physics 2025-07-15 Hongbin Qu , Guang-Ming Zhang , Gang Li