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Particle tracking passive microrheology in 8CB liquid crystals is used to redefine the precessional motion of the orientation of nematic director in liquid crystals. Physical origin of tumbling director in presence of presmectic clusters…

Soft Condensed Matter · Physics 2015-04-02 Balaji Yendeti , Ashok Vudayagiri

Recently, a new class of smectic liquid crystal phases (SmCP phases) characterized by the spontaneous formation of macroscopic chiral domains from achiral bent-core molecules has been discovered. We have carried out Monte Carlo simulations…

Statistical Mechanics · Physics 2009-11-07 Yves Lansac , Prabal K. Maiti , Noel A. Clark , Matthew A. Glaser

The structure of nematic liquid crystals formed by bent-core mesogens (BCMs) is studied in the context of Monte Carlo simulations of a simple molecular model that captures the symmetry, shape and flexibility of achiral BCMs. The results…

Soft Condensed Matter · Physics 2013-09-10 Stavros D. Peroukidis , Alexandros G. Vanakaras , Demetri J. Photinos

The bent-core liquid crystals (LCs) are highly regarded as the next-generation materials for electro-optic devices. The nematic (N) phase of these LCs possesses highly ordered smectic-like cybotactic clusters which are promising in terms of…

Soft Condensed Matter · Physics 2019-02-06 Sourav Patranabish , Yiwei Wang , Aloka Sinha , Apala Majumdar

The effects of dipolar interactions and molecular flexibility on the structure and phase behavior of bent-core molecular fluids are studied using Monte Carlo computer simulations. Some calculations of flexoelectric coefficients are also…

Soft Condensed Matter · Physics 2007-05-23 Alastair Dewar , Philip J. Camp

Chiral liquid crystals often exhibit periodic modulations in the molecular director; in particular, thin films of the smectic-C* phase show a chiral striped texture. Here, we investigate whether similar chiral modulations can occur in the…

Soft Condensed Matter · Physics 2009-10-31 J. V. Selinger , J. Xu , R. L. B. Selinger , B. R. Ratna , R. Shashidhar

By molecular modeling we demonstrate that the nematic long-range order discovered in bent-core liquid crystal systems should reveal further spatially homogeneous phases. Two of them are identified as a tetrahedratic nematic ($N_T$) phase…

Soft Condensed Matter · Physics 2009-04-30 Lech Longa , Grzegorz Pająk , Thomas Wydro

Comprehensive x-ray scattering studies have characterized the smectic ordering of octylcyanobiphenyl (8CB) confined in the hydrogen-bonded silica gels formed by aerosil dispersions. For all densities of aerosil and all measurement…

Soft Condensed Matter · Physics 2009-11-07 R. L. Leheny , S. Park , R. J. Birgeneau , J. -L. Gallani , C. W. Garland , G. S. Iannacchione

We carry out Monte Carlo simulations to investigate the effect of molecular shape on liquid-crystal order. In our approach, each model mesogen consists of several soft spheres bonded rigidly together. The arrangement of the spheres may be…

Soft Condensed Matter · Physics 2009-11-07 J. Xu , R. L. B. Selinger , J. V. Selinger , R. Shashidhar

Using Monte Carlo simulation methods, we explore the role of molecular shape in the phase behavior of liquid crystals and the electroclinic effect. We study a "bent-rod" mesogen shaped like the letter Z, composed of seven soft spheres…

Soft Condensed Matter · Physics 2009-10-31 J. Xu , R. L. B. Selinger , J. V. Selinger , B. R. Ratna , R. Shashidhar

Colloidal rods immersed in a thermotropic liquid-crystalline solvent are at the basis of so-called hybrid liquid crystals which are characterized by tunable nematic fluidity with symmetries ranging from conventional uniaxial nematic or…

Soft Condensed Matter · Physics 2021-07-28 B. Senyuk , H. Mundoor , I. I. Smalyukh , H. H. Wensink

A high-resolution calorimetric study has been carried out on nano-colloidal dispersions of aerosils in the liquid crystal 4-\textit{n}-pentylphenylthiol-4'-\textit{n}-octyloxybenzoate ($\bar{8}$S5) as a function of aerosil concentration and…

Soft Condensed Matter · Physics 2009-11-11 A. Roshi , G. S. Iannacchione , P. S. Clegg , R. J. Birgeneau , M. E. Neubert

We explore the phase behavior and structure of orthogonal smectic liquid crystals consisting of bent-core molecules (BCMs) by means of Monte Carlo molecular simulations. A simple athermal molecular model is introduced that describes the…

Soft Condensed Matter · Physics 2016-07-26 Stavros D. Peroukidis , Alexandros G. Vanakaras , Demetri J. Photinos

We use lattice Boltzmann simulations of the Beris--Edwards formulation of nematodynamics to probe the response of a nematic liquid crystal with conflicting anchoring at the boundaries under shear and Poiseuille flow. The geometry we focus…

Soft Condensed Matter · Physics 2009-11-10 D. Marenduzzo , E. Orlandini , J. M. Yeomans

The possible symmetries of the biaxial nematic phase are examined against the implications of the presently available experimental results. Contrary to the widespread notion that biaxial nematics have orthorhombic symmetry, our study shows…

Soft Condensed Matter · Physics 2010-04-15 Panagiota K. Karahaliou , Alexandros G. Vanakaras , Demetri J. Photinos

Optical birefringence measurements on a rod-like liquid crystal (8OCB), imbibed in silica channels (7 nm diameter), are presented and compared to the thermotropic bulk behavior. The orientational and positional order of the confined liquid…

Soft Condensed Matter · Physics 2015-05-20 Andriy V. Kityk , Patrick Huber

Recent liquid-crystalline (LC) research is focused on structurally new molecular systems distinct from simple nematic or smectic phases. Sophisticated molecular shape may reveal structural complexity, combining helicity and polarity.…

We study the layer-to-layer diffusion in smectic-A liquid crystals of colloidal hard rods with different length-to-diameter ratios using computer simulations. The layered arrangement of the smectic phase yields a hopping-type diffusion due…

Soft Condensed Matter · Physics 2010-06-16 Alessandro Patti , Djamel El Masri , René van Roij , Marjolein Dijkstra

Nematic liquid crystals exhibit both crystal-like and fluid-like features. In particular, the propagation of an acoustic wave shows an unexpected occurrence of some of the solid-like features at the hydrodynamic level, namely, the…

Soft Condensed Matter · Physics 2017-01-04 Stefano S. Turzi

A number of highly polar three ring rod-shaped compounds with a terminal thiophene ring have been synthesized and the physical properties of a subset are reported in detail. On cooling from the isotropic fluid, they directly transition to a…

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