English
Related papers

Related papers: Electrostatic interactions in water: nonlocal elec…

200 papers

Understanding the response of the surface of metallic solids to external electric field sources is crucial to characterize electrode-electrolyte interfaces. Continuum electrostatics offer a simple description of the induced charge density…

Chemical Physics · Physics 2021-12-14 Giovanni Pireddu , Laura Scalfi , Benjamin Rotenberg

Hydrodynamic equations for a one-component plasma are derived as a generalization of the Euler equations to include the effects of the long-range Coulomb interaction. By using a variational principle, these equations self-consistently unify…

Plasma Physics · Physics 2024-03-20 Daniels Krimans , Seth Putterman

The nonlocal dielectric properties of liquid water are studied in the context of {\it ab initio} molecular dynamics simulations based on density functional theory. We calculate the dielectric response from the charge structure factor of the…

The electrostatic interaction between pairs of spherical or macroscopically long, parallel cylindrical colloids trapped at fluid interfaces is studied theoretically for the case of small inter-particle separations. Starting from the…

Soft Condensed Matter · Physics 2018-11-30 Arghya Majee , Markus Bier , S. Dietrich

The Multiparticle Collision Dynamics technique (MPC) for hydrodynamics simulations is generalized to binary fluid mixtures and multiphase flows, by coupling the particle-based fluid dynamics to a Ginzburg-Landau free-energy functional for…

Soft Condensed Matter · Physics 2024-06-03 Thomas Eisenstecken , Raphael Hornung , Roland G. Winkler , Gerhard Gompper

We examine the effective force between two nanometer scale solutes in water by Molecular Dynamics simulations. Macroscopic considerations predict a strong reduction of the hydrophobic attraction between solutes when the latter are charged.…

Statistical Mechanics · Physics 2009-11-10 J. Dzubiella , J. -P. Hansen

We have used molecular simulation and methods of importance sampling to study the thermodynamics and kinetics of ionic charge separation at a liquid water-metal interface. We have considered this process using canonical examples of two…

Chemical Physics · Physics 2022-06-08 John A. Kattirtzi , David T. Limmer , Adam P. Willard

Using molecular dynamics simulations, we reveal emergent properties of hydrated electrode interfaces that while molecular in origin are integral to the behavior of the system across long times scales and large length scales. Specifically,…

Materials Science · Physics 2015-05-20 David T. Limmer , Adam P. Willard

Macroscopic field quantization is presented for a nondispersive photonic dielectric environment, both in the absence and presence of guest atoms. Starting with a minimal-coupling Lagrangian, a careful look at functional derivatives shows…

Quantum Physics · Physics 2007-10-31 Martijn Wubs , L. G. Suttorp , A. Lagendijk

The structure of an aqueous solution of sodium chloride at a planar electrode is investigated by integral equation techniques. With the central force water model the aqueous electrolyte is modelled as a mixture of sodium and chloride ions…

chem-ph · Physics 2009-10-28 M. Vossen , F. Forstmann

Charge-stabilized colloidal spheres dispersed in deionized water are supposed to repel each other. Instead, artifact-corrected video microscopy measurements reveal an anomalous long-ranged like-charge attraction in the interparticle pair…

Soft Condensed Matter · Physics 2009-11-11 Marco Polin , David G. Grier , Yilong Han

On a basis of a two-length scale description of hydrophobic interactions we develop a continuous self-consistent theory of solute-water interactions which allows to determine a hydrophobic layer of a solute molecules of any geometry with…

Soft Condensed Matter · Physics 2007-05-23 G. Sitnikov , S. Nechaev , M. Taran , A. Muryshev

We construct a boundary integral representation for the low-Reynolds-number flow in a channel in the presence of freely-suspended particles (or droplets) of arbitrary size and shape. We demonstrate that lubrication theory holds away from…

Fluid Dynamics · Physics 2018-01-17 Itzhak Fouxon , Zhouyang Ge , Luca Brandt , Alexander Leshansky

We derive hydrodynamic equations from Vicsek-style dry active matter models in three dimensions (3D), building on our experience on the 2D case using the Boltzmann-Ginzburg-Landau approach. The hydrodynamic equations are obtained from a…

Soft Condensed Matter · Physics 2020-03-17 Benoît Mahault , Aurelio Patelli , Hugues Chaté

Based on the thermodynamic perturbation theory (TPT) and the Random phase approximation (RPA), we present a statistical theory of solutions of electrically neutral soft molecules, every of which is modelled as a set of sites that interact…

Soft Condensed Matter · Physics 2019-03-12 Yu. A. Budkov

In this paper, we consider the numerical approximation for a diffuse interface model of the two-phase incompressible inductionless magnetohydrodynamics problem. This model consists of Cahn-Hilliard equations, Navier-Stokes equations and…

Numerical Analysis · Mathematics 2022-02-01 Xiaorong Wang , Xiaodi Zhang

The free motion of charged colloids within ionic solutions and in the vicinity of charged boundaries, is a phenomenon that occurs in various natural, biological and industrial settings. Here, we develop an electrohydrodynamic lubrication…

Soft Condensed Matter · Physics 2026-04-29 Anirban Chatterjee , Yacine Amarouchene , Thomas Salez

The aggregation of clay particles in aqueous solution is a ubiquitous everyday process of broad environmental and technological importance. However, it is poorly understood at the all-important atomistic level since it depends on a complex…

In this paper we study the electrostatic properties of `Janus' spheres with unequal charge densities on both hemispheres. We introduce a method to compare primitive-model Monte Carlo simulations of the ionic double layer with predictions of…

Soft Condensed Matter · Physics 2012-09-18 Joost de Graaf , Niels Boon , Marjolein Dijkstra , René van Roij

We investigate the system constituted by a polarizable atom near a nanosphere under the influence of an external electrostatic field, showing that the attractive dispersive force between them can be overcome by the electrostatic…

Quantum Physics · Physics 2021-08-26 P. P. Abrantes , V. Pessanha , Reinaldo de Melo e Souza , C. Farina