Related papers: Heteronuclear Rydberg molecules
We prepare and analyze Rydberg states with orbital quantum numbers $\ell \le 6$ using three-optical-photon electromagnetically-induced transparency (EIT) and radio-frequency (RF) dressing, and employ the high-$\ell$ states in electric-field…
Obtaining full control over the internal and external quantum states of molecules is the central goal of ultracold chemistry and allows for the study of coherent molecular dynamics, collisions and tests of fundamental laws of physics. When…
We report experimental results on Rydberg facilitation, whereby Rydberg levels can be excited off-resonantly in the presence of a nearby Rydberg atom because of Rydberg-Rydberg interactions, for high-lying $S$, $P$ and $D$ levels in…
The ability to control and tune interactions in ultracold atomic gases has paved the way towards the realization of new phases of matter. Whereas experiments have so far achieved a high degree of control over short-ranged interactions, the…
We show that transient supersolid quantum states of Rydberg-excitations can be created dynamically from a Mott insulator of ground state atoms in a 2D optical-lattices by irradiating it with short laser pulses. The structure of these…
The level structure of negative-ions near the electron detachment limit dictates the low-energy scattering of an electron with the parent neutral atom. We demonstrate that a single ultracold atom bound inside a Rydberg orbit forming an…
We present the direct measurements of electric-dipole moments for $5P_{3/2}\to nD_{5/2}$ transitions with $20<n<48$ for Rubidium atoms. The measurements were performed in an ultracold sample via observation of the Autler-Townes splitting in…
We present combined measurements of the spatially-resolved optical spectrum and the total excited-atom number in an ultracold gas of three-level atoms under electromagnetically induced transparency conditions involving high-lying Rydberg…
We observe that when an ultracold ground state cesium (Cs) atom becomes bound within the electronic cloud of an extended Cs electronic orbit, ultralong-range molecules with giant (kilo-Debye) permanent electric dipole moments form. Large…
Recent theoretical studies with alkali atoms A$^{\ast}$ excited to high Rydberg states predicted the existence of ultra long-range molecular bound states. Such excited dimers have large electric dipole moments which, in combination with…
We present a novel binding mechanism where a neutral Rydberg atom and an atomic ion form a molecular bound state at large internuclear distance. The binding mechanism is based on Stark shifts and level crossings which are induced in the…
We report measurements of the absolute excitation frequencies of $^{165}$Ho $4f^{11}6sns$ and $4f^{11}6snd$ odd-parity Rydberg series. The states are detected through depletion of a magneto-optical trap via a two-photon excitation scheme.…
The complex Rydberg structure of ytterbium atoms is shaped by multiple low-lying ion-core-excited states and strong channel interactions, which presents both opportunities and challenges for quantum information processing and precision…
Clusters of the electronically excited condensed matter Rydberg Matter (RM) are planar and six-fold symmetric with magic numbers N = 7, 19, 37, 61 and 91. The bond distances in the clusters are known with a precision of +- 5% both from…
We study Rydberg atoms modulated by strong radio-frequency (RF) fields with a frequency of 70 MHz. The Rydberg atoms are prepared in a room temperature cesium cell, and their level structure is probed using electromagnetically induced…
Vibrational properties of ultralong Rydberg Cs$_2$ molecules are investigated on corresponding potential curves obtained by perturbation theory. The Rydberg Cs$_2$ molecules are associated by a Rydberg Cs($nS/nP$) atom $(n=30-70)$ and a…
We demonstrate that through localised Rydberg excitation in a three-dimensional cold atom cloud atomic motion can be rendered directed and nearly confined to a plane, without spatial constraints for the motion of individual atoms. This…
We report the experimental observation of radiative recombination from Rydberg excitons in a two-dimensional semiconductor, monolayer WSe2, encapsulated in hexagonal boron nitride. Excitonic emission up to the 4s excited state is directly…
Rydberg atom-based sensors are a new type of radio frequency sensor that is inherently quantum mechanical. Several configurations of the sensor use a local oscillator to determine the properties of the target radio frequency field. We…
We calculate the potential energy curves, the permanent dipole moment curves, and the lifetimes of the ground and excited vibrational states of the heteronuclear alkali dimers XY (X, Y = Li, Na, K, Rb, Cs) in the X1{\Sigma}+ electronic…